Abstract
We identify uncertainties and knowledge gaps of chemical risk assessment related to unconventional drillings and propose adaptations. We discuss how chemical risk assessment in the context of unconventional oil and gas (UO&G) activities differs from conventional chemical risk assessment and the implications for existing legislation. A UO&G suspect list of 1,386 chemicals that might be expected in the UO&G water samples was prepared which can be used for LC-HRMS suspect screening. We actualize information on reported concentrations in UO&G-related water. Most information relates to shale gas operations, followed by coal-bed methane, while only little is available for tight gas and conventional gas. The limited research on conventional oil and gas recovery hampers comparison whether risks related to unconventional activities are in fact higher than those related to conventional activities. No study analyzed the whole cycle from fracturing fluid, flowback and produced water, and surface water and groundwater. Generally target screening has been used, probably missing contaminants of concern. Almost half of the organic compounds analyzed in surface water and groundwater exceed TTC values, so further risk assessment is needed, and risks cannot be waived. No specific exposure scenarios toward groundwater aquifers exist for UO&G-related activities. Human errors in various stages of the life cycle of UO&G production play an important role in the exposure. Neither at the international level nor at the US federal and the EU levels, specific regulations for UO&G-related activities are in place to protect environmental and human health. UO&G activities are mostly regulated through general environmental, spatial planning, and mining legislation.
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Abbreviations
- AU:
-
Australia
- BMDL:
-
Benchmark dose
- CA:
-
Concentration addition
- DE:
-
Germany
- DWD:
-
Drinking Water Directive
- EC50:
-
Half maximal effective concentration
- EU:
-
European Union
- GA:
-
Glutaraldehyde
- GWD:
-
Groundwater Directive
- IARC:
-
International Agency for Research on Cancer
- IEA:
-
International Energy Agency
- Koc:
-
Soil organic carbon-water partition coefficient
- LC-HRMS:
-
Liquid chromatography high resolution mass spectrometry
- Log Kow:
-
n-octanol-water partition coefficient
- MS:
-
Mass Spectrometry
- NOAEL:
-
No adverse effect level
- PBT:
-
Persistent, bioaccumulative and toxic
- PEC:
-
Predicted environmental concentration
- PNEC:
-
Predicted no effect concentration
- RfD:
-
Reference dose
- RQ:
-
Risk quotient
- TDS:
-
Total dissolved solids
- TDI:
-
Tolerable daily intake
- TTC:
-
Threshold of toxicological concern
- UK:
-
United Kingdom
- UO&G:
-
Unconventional oil and gas
- USA:
-
United States of America
- WFD:
-
Water Framework Directive
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Acknowledgments
This work is part of the research program “Shale Gas & Water” with project number 859.14.001, which is financed by the Netherlands Organization for Scientific Research (NWO) and the drinking water companies Brabant Water, Oasen, and Waterleiding Maatschappij Limburg.
The authors declare that they have no conflict of interest.
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Faber, AH. et al. (2017). How to Adapt Chemical Risk Assessment for Unconventional Hydrocarbon Extraction Related to the Water System. In: de Voogt, P. (eds) Reviews of Environmental Contamination and Toxicology Volume 246. Reviews of Environmental Contamination and Toxicology, vol 246. Springer, Cham. https://doi.org/10.1007/398_2017_10
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