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Rh(III)- and Ir(III)-Catalyzed C–C Bond Cross Couplings from C–H Bonds

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C-H Bond Activation and Catalytic Functionalization I

Part of the book series: Topics in Organometallic Chemistry ((TOPORGAN,volume 55))

Abstract

Over the recent years, dicationic [Cp*Ir(III)] and more particularly [Cp*Rh(III)] complexes have established themselves as extremely powerful catalysts enabling direct C–H activation of various aromatic and vinylic compounds. During such transformations, a common metallacyclic intermediate [Cp*M(C^X)] (M=Ir, Rh) is formed and undergoes further transformations, according to the nature of the coupling partner, to finally afford a myriad of valuable, often complex, and otherwise difficult to access scaffolds like heterocycles and polyunsaturated skeletons. The major advances achieved in this field clearly showcase the potential of these catalysts to functionalize latent C–H bonds under surprisingly mild reaction conditions. The aim of this chapter is to present the latest and most representative contributions in the field of Rh(III)- and Ir(III)-catalyzed C–H activation by focusing on the reactivity of the corresponding metallacyclic intermediates.

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Authors and Affiliations

  1. Laboratoire de Chimie Moléculaire (UMR CNRS 7509), Université de Strasbourg, ECPM, 25 Rue Becquerel, 67087, Strasbourg, France

    Joanna Wencel-Delord

  2. Technische Universität Kaiserslautern, Erwin-Schrödinger-Straße Geb. 52, 67663, Kaiserslautern, Germany

    Frederic W. Patureau

  3. Westälische Wilhelms-Universität Münster, International Graduate, School of Chemistry and Organisch-Chemisches Institut, Corrensstrasse 40, 48149, Münster, Germany

    Frank Glorius

Authors
  1. Joanna Wencel-Delord
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  2. Frederic W. Patureau
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  3. Frank Glorius
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Correspondence to Joanna Wencel-Delord .

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  1. Université de Rennes, Rennes, France

    Pierre H. Dixneuf

  2. Université de Rennes , Rennes, France

    Henri Doucet

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© 2015 Springer International Publishing Switzerland

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Wencel-Delord, J., Patureau, F.W., Glorius, F. (2015). Rh(III)- and Ir(III)-Catalyzed C–C Bond Cross Couplings from C–H Bonds. In: Dixneuf, P., Doucet, H. (eds) C-H Bond Activation and Catalytic Functionalization I. Topics in Organometallic Chemistry, vol 55. Springer, Cham. https://doi.org/10.1007/3418_2015_140

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