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Hydro-, Carbo-, and Cycloalumination of Unsaturated Compounds

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Modern Organoaluminum Reagents

Part of the book series: Topics in Organometallic Chemistry ((TOPORGAN,volume 41))

Abstract

This chapter gives a survey and a systematic account of modern achievements in the synthesis of acyclic and cyclic organoaluminum compounds using thermal and catalytic hydro- and carboalumination of unsaturated compounds. Here we consider a new, versatile catalytic cycloalumination reaction of olefins, acetylenes, and 1,2-dienes of various structures with alkyl and halogen alkyl Al catalyzed by Zr and Ti complexes to give previously unknown classes of OACs: aluminacyclopropanes, aluminacyclopropenes, aluminacyclopentanes, aluminacyclopentenes, aluminacyclopentadienes, and aluminamacrocarbocycles. Much attention is given to applications of hydro-, carbo-, and cycloalumination reactions for the synthesis of practically important natural carbo- and heterocyclic compounds.

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Abbreviations

COD:

1,5-Cyclooctadienyl

Cp:

η5-Cyclopentadienyl, C5H5

Cp*:

η5-Pentamethylcyclopentadienyl, C5Me5

Hex:

n-C6H13

OAC:

Organoaluminum compound

ZACA:

Zr-catalyzed asymmetric carboalumination of alkenes

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Authors and Affiliations

  1. Laboratory of Catalytic Synthesis, Institute of Petrochemistry and Catalysis, Russian Academy of Sciences, 141 Prospekt Oktyabrya, Ufa, 450075, Russian Federation

    Usein M. Dzhemilev & Vladimir A. D’yakonov

Authors
  1. Usein M. Dzhemilev
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  2. Vladimir A. D’yakonov
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Correspondence to Vladimir A. D’yakonov .

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Editors and Affiliations

  1. , School of Chemistry, The University of Nottingham, University Park, Nottingham, NG7 2RD, United Kingdom

    Simon Woodward

  2. Laboratoire DECOMET, Institut Le Bel, Université de Strasbourg, 4 rue Blaise Pascal, Strasbourg, 67000, France

    Samuel Dagorne

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Dzhemilev, U.M., D’yakonov, V.A. (2012). Hydro-, Carbo-, and Cycloalumination of Unsaturated Compounds. In: Woodward, S., Dagorne, S. (eds) Modern Organoaluminum Reagents. Topics in Organometallic Chemistry, vol 41. Springer, Berlin, Heidelberg. https://doi.org/10.1007/3418_2012_38

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