Skip to main content

Dynamics of Frustrated Magnetic Moments in Antiferromagnetically Ordered TbNiAl Probed by Spin Echo and Time-of-Flight Spectroscopy

  • Chapter
  • First Online:
Neutron Spin Echo Spectroscopy

Part of the book series: Lecture Notes in Physics ((LNP,volume 601))

Abstract

In this contribution we present a combined study of the dynamics of frustrated Tb spins in the intermetallic compound TbNiAl by means of neutron time-of-flight and spin echo spectroscopy. It is a remarkable and very unusual characteristic of TbNiAl that its afm phase (below T N = 47 K) contains regular long-range ordered spins as well as frustrated spins. The latter are identified by a strongly reduced moment measured by neutron diffraction. Our quasielastic measurements show that the frustrated moments relax on a time scale of 0.01 ns to 0.1 ns. Their auto-correlation function I(Q, t) is Q-independent and exponential in time.

This is a preview of subscription content, log in via an institution to check access.

Access this chapter

Chapter
USD 29.95
Price excludes VAT (USA)
  • Available as PDF
  • Read on any device
  • Instant download
  • Own it forever
eBook
USD 84.99
Price excludes VAT (USA)
  • Available as PDF
  • Read on any device
  • Instant download
  • Own it forever
Softcover Book
USD 109.99
Price excludes VAT (USA)
  • Compact, lightweight edition
  • Dispatched in 3 to 5 business days
  • Free shipping worldwide - see info
Hardcover Book
USD 109.99
Price excludes VAT (USA)
  • Durable hardcover edition
  • Dispatched in 3 to 5 business days
  • Free shipping worldwide - see info

Tax calculation will be finalised at checkout

Purchases are for personal use only

Institutional subscriptions

Preview

Unable to display preview. Download preview PDF.

Unable to display preview. Download preview PDF.

References

  1. R. Liebmann, Statistical Mechanics of Periodic Frustrated Ising Systems, (Springer, Berlin 1986)

    Google Scholar 

  2. H. T. Diep, Magnetic Systems with Competing Interactions: Frustrated Spin Systems, (World Scientific, Singapore 1994)

    Google Scholar 

  3. A. P. Ramirez, Annu. Rev. Mater. Sci. 24, 453 (1994)

    Article  ADS  Google Scholar 

  4. J. N. Reimers, A.J. Berlinsky, A.C. Shi, Phys. Rev. B 43, 865 (1991)

    Article  ADS  Google Scholar 

  5. G. H. Wannier, Phys. Rev. 79, 357 (1950)

    Article  MATH  ADS  MathSciNet  Google Scholar 

  6. I. Syozi, Prog. Theor. Phys. 6, 306 (1951)

    Article  MATH  ADS  MathSciNet  Google Scholar 

  7. J. N. Reimers, Phys. Rev. B 45, 7287 (1992)

    Article  ADS  Google Scholar 

  8. R. Moessner, J.T. Chalker, Phys. Rev. Lett. 80, 2929 (1998)

    Article  ADS  Google Scholar 

  9. R. Moessner, J.T. Chalker, Phys. Rev. B 58, 12049 (1998)

    Article  ADS  Google Scholar 

  10. A. Keren, Phys. Rev. Lett. 72, 3254 (1994)

    Article  ADS  Google Scholar 

  11. B. D. Gaulin, J.N. Reimers, T.E. Mason, J.E. Greedan, Z. Tun, Phys. Rev. Lett. 69, 3244 (1992)

    Article  ADS  Google Scholar 

  12. M. J. Harris, M.P. Zinkin, T. Zeiske, Phys. Rev. B 52, R707 (1995)

    Article  ADS  Google Scholar 

  13. S. H. Lee, C. Broholm, G. Aeppli, T.G. Perring, B. Hessen, A. Taylor, Phys. Rev. Lett. 76, 4424 (1996)

    Article  ADS  Google Scholar 

  14. M. P. Zinkin, M.J. Harris, T. Zeiske, Phys. Rev. B 56, 11786 (1997)

    Article  ADS  Google Scholar 

  15. H. Serrano-González, S.T. Bramwell, K.D.M. Harris, B.M. Kariuki, L. Nixon, I.P. Parkin, C. Ritter, Phys. Rev. B 59, 14451 (1999)

    Article  ADS  Google Scholar 

  16. J. S. Gardner, B.D. Gaulin, S.H. Lee, C. Broholm, N.P. Raju, J.E. Greedan, Phys. Rev. Lett. 83, 211 (1999)

    Article  ADS  Google Scholar 

  17. S. H. Lee, C. Broholm, T.H. Kim, W. Ratcliff II, S.W. Cheong, Phys. Rev. Lett. 84, 3718 (2000)

    Article  ADS  Google Scholar 

  18. A. Keren, K. Kojima, L.P. Le, G.M. Luke, W.D. Wu, Y.J. Uemura, M. Takano, H. Dabkowska, M.J.P. Gingras, Phys. Rev. B 53, 6451 (1996)

    Article  ADS  Google Scholar 

  19. J. S. Gardner, S.R. Dunsiger, B.D. Gaulin, M.J.P. Gingras, J.E. Greedan, R.F. Kie, M.D. Lumsden, W.A. MacFarlane, N.P. Raju, J.E. Sonier, I. Swainson, Z. Tun, Phys. Rev. Lett. 82, 1012 (1999)

    Article  ADS  Google Scholar 

  20. A. Keren, Y.J. Uemura, G. Luke, P. Mendels, M. Mekata, T. Asano, Phys. Rev. Lett. 84, 3450 (2000)

    Article  ADS  Google Scholar 

  21. S. R. Dunsiger, J.S. Gardner, J.A. Chakhalian, A.L. Cornelius, M. Jaime, R.F. Kiefl, R. Movshovich, W.A. MacFarlane, R.I. Miller, J.E. Sonier, B.D. Gaulin, Phys. Rev. Lett. 85, 3504 (2000)

    Article  ADS  Google Scholar 

  22. B. Martínez, A. Labarta, R. Rodríguez-Solía, X. Obradors, Phys. Rev. B 50, 15779 (1994)

    Article  ADS  Google Scholar 

  23. J. E. Greedan, N.P. Raju, A. Maignan, Ch. Simon, J.S. Pedersen, A.M. Niraimathi, E. Gmelin, M.A. Subramanian, Phys. Rev. B 54, 7189 (1996)

    Article  ADS  Google Scholar 

  24. M. J. P. Gingras, C.V. Stager, N.P. Raju, B.D. Gaulin, J.E. Greedan, Phys. Rev. Lett. 78, 947 (1997)

    Article  ADS  Google Scholar 

  25. N. P. Raju, J.E. Greedan, M.A. Subramanian, C.P. Adams, T.E. Mason, Phys. Rev. B 58, 5550 (1998)

    Article  ADS  Google Scholar 

  26. Y. K. Tsui, C.A. Burns, J. Snyder, P. Schiffer, Phys. Rev. Lett. 82, 3532 (1999)

    Article  ADS  Google Scholar 

  27. N. P. Raju, M. Dion, M.J.P. Gingras, T.E. Mason, J.E. Greedan, Phys. Rev. B 59, 14489 (1999)

    Article  ADS  Google Scholar 

  28. M. J. P. Gingras, B.C. den Hertog, M. Faucher, J.S. Gardner, S.R. Dunsiger, L.J. Chang, B.D. Gaulin, N.P. Raju, J.E. Greedan, Phys. Rev. B 62, 6496 (2000)

    Article  ADS  Google Scholar 

  29. A. E. Dwight, M.H. Mueller, R.A. Conner, Jr., J.W. Downey, H. Knott, Trans. Metall. Soc. AIME 242, 2075 (1968)

    Google Scholar 

  30. H. Oesterreicher, J. Less-Common Met. 30, 225 (1973)

    Article  Google Scholar 

  31. H. Maletta, V. Sechovský, J. Alloys Compd. 207–208, 234 (1994)

    Google Scholar 

  32. G. Ehlers, H. Maletta, Z. Phys. B 99, 145 (1996)

    Article  ADS  Google Scholar 

  33. P. Javorský, P. Burlet, V. Sechovský, A.V. Andreev, J. Brown, P. Svoboda, J. Magn. Magn. Mater. 166, 133 (1997)

    Article  ADS  Google Scholar 

  34. A. Dönni, G. Ehlers, H. Maletta, P. Fischer, H. Kitazawa, M. Zolliker, J. Phys: Condens. Matter 8, 11213 (1996)

    Article  ADS  Google Scholar 

  35. M. Dolores Núñez-Regueiro, C. Lacroix, B. Canals, Physica C 282–287 1885 (1997)

    Article  Google Scholar 

  36. S. A. M. Mentink, A. Drost, G.J. Nieuwenhuys, E. Frikkee, A.A. Menovsky, J.A. Mydosh, Phys. Rev. Lett. 73, 1031 (1994)

    Article  ADS  Google Scholar 

  37. S. A. M. Mentink, G.J. Nieuwenhuys, H. Nakotte, A.A. Menovsky, A. Drost, E. Frikkee, J.A. Mydosh, Phys. Rev. B 51, 11567 (1995)

    Article  ADS  Google Scholar 

  38. C. Lacroix, B. Canals, M.D. Núñez-Regueiro, Phys. Rev. Lett. 77, 5126 (1996)

    Article  ADS  Google Scholar 

  39. R. Movshovich, M. Jaime, S. Mentink, A.A. Menovsky, J.A. Mydosh, Phys. Rev. Lett. 83, 2065 (1999)

    Article  ADS  Google Scholar 

  40. B. Farago, Physica B 267–268, 270 (1999)

    Article  Google Scholar 

  41. F. Mezei, Neutron Spin Echo, Lecture Notes in Physics, Vol. 128, (Springer Verlag, Berlin, 1980)

    Book  Google Scholar 

  42. O. Schärpf, H. Capellmann, Phys. Status Solidi A 135, 359 (1993)

    Article  ADS  Google Scholar 

  43. R. E. Lechner, F. Volino, A.J. Dianoux, F. Douchin, H. Hervet, G.C. Stirling, Internal ILL report 73L85 (ILL, Grenoble 1973), see also Chapter 3.2.1 in M. Bée, Quasielastic Neutron Scattering (Adam Hilger, Bristol, 1988) pp. 81–85

    Google Scholar 

  44. R. E. Lechner, Neutron News 7, No. 4, 9 (1996)

    Article  Google Scholar 

  45. R. E. Lechner, in Proceedings of ICANS-XI, KEK Report 90-25, ed. by M. Misawa, M. Furusaka, H. Ikeda, N. Watanabe (Nat. Lab. for High Energy Physics, Tsukuba, March 1991) pp. 717

    Google Scholar 

Download references

Author information

Authors and Affiliations

Authors

Editor information

Editors and Affiliations

Rights and permissions

Reprints and permissions

Copyright information

© 2002 Springer-Verlag Berlin Heidelberg

About this chapter

Cite this chapter

Ehlers, G., Casalta, H., Lechner, R.E., Maletta, H. (2002). Dynamics of Frustrated Magnetic Moments in Antiferromagnetically Ordered TbNiAl Probed by Spin Echo and Time-of-Flight Spectroscopy. In: Mezei, F., Pappas, C., Gutberlet, T. (eds) Neutron Spin Echo Spectroscopy. Lecture Notes in Physics, vol 601. Springer, Berlin, Heidelberg. https://doi.org/10.1007/3-540-45823-9_18

Download citation

  • DOI: https://doi.org/10.1007/3-540-45823-9_18

  • Published:

  • Publisher Name: Springer, Berlin, Heidelberg

  • Print ISBN: 978-3-540-44293-6

  • Online ISBN: 978-3-540-45823-4

  • eBook Packages: Springer Book Archive

Publish with us

Policies and ethics