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Hydrogen, Methane and Carbon Dioxide Adsorption in Metal-Organic Framework Materials

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Book cover Functional Metal-Organic Frameworks: Gas Storage, Separation and Catalysis

Part of the book series: Topics in Current Chemistry ((TOPCURRCHEM,volume 293))

Abstract

The role of porous coordination polymers (metal-organic frameworks) as storage materials for hydrogen, carbon dioxide and methane and the current state-of-the-art in this rapidly developing field are reviewed. The significant potential of porous materials to store fuel gases effectively and reversibly illustrates the great promise of engineered solid-state materials as the next generations of applied multi-functional materials.

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Abbreviations

BET:

Brunauer-Emmett-Teller

DABCO:

1,4-Diazabicyclo[2.2,2]octane

diPyNI:

N,N′-Di-(4-pyridyl)-1,4,5,8-naphthalenetetracarboxydiimide

diPyTz:

Di-3,6-(4-pyridyl)-1,2,4,5-tetrazine

DoE:

Department of Energy (USA)

H2BDC:

Benzene-1,4-dicarboxylic acid

H2BDP:

Benzene-1,4-di(4′-pyrazole)

H2BPnDC:

Benzophenone-4,4′-dicarboxylic acid

H2BPPC:

Pyridine-3,5-bis(phenyl-4-carboxylic acid)

H2ImDC:

Imidazole-4,5-dicarboxylic acid

H2NDC:

Naphthalene-2,6-dicarboxylic acid

H2PPZ:

Dihydropiperazinium cation

H2T2DC:

Thieno[3,2-b]thiophene-2,5-dicarboxylic acid

H3BTB:

1,3,5-Tris-(4-carboxyphenyl)benzene

H3BTC:

Benzene-1,3,5-tricarboxylic acid

H3BTT:

Benzene-1,3,5-tris-tetrazole

H4ABTC:

Azodibenzene-3,3′,5,5′-tetracarboxylic acid

H4BPTC:

Biphenyl-3,3′,5,5′-tetracarboxylic acid

H4MDIP:

5,5′-Methylene diisophthalic acid

H4QPTC:

Quaterphenyl-3,5,3′,5′-tetracarboxylic acid

INS:

Inelastic neutron scattering

IRMOF:

Isoreticular metal-organic framework

LDA:

Lithium diisopropylamide

MOF:

Metal-organic framework

NH2-H2BDC:

2-Amino-benzene-1,4-dicarboxylic acid

NPD:

Neutron powder diffraction

PDF:

Pair distribution function

Pyen:

5-Methyl-4-oxo-1,4-dihydropyridine-3-carboxaldehyde

ZIF:

Zeolitic imidazolate framework

ΔHads :

Heat of enthalpy of adsorption

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Acknowledgments

We thank the EPSRC (Supergen consortium UKSHEC) for support. MS gratefully acknowledges receipt of a Wolfson Royal Society Merit Award and the ERC for an Advanced Grant to MS.

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Authors and Affiliations

  1. School of Chemistry, University of Nottingham, Nottingham, NG7 2RD, UK

    Xiang Lin, Neil R. Champness & Martin Schröder

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  1. Xiang Lin
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Correspondence to Martin Schröder .

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  1. Faculty of Science, School of Chemistry, University of Nottingham, University Park, Nottingham, NG72RD, United Kingdom

    Martin Schröder

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Lin, X., Champness, N.R., Schröder, M. (2009). Hydrogen, Methane and Carbon Dioxide Adsorption in Metal-Organic Framework Materials. In: Schröder, M. (eds) Functional Metal-Organic Frameworks: Gas Storage, Separation and Catalysis. Topics in Current Chemistry, vol 293. Springer, Berlin, Heidelberg. https://doi.org/10.1007/128_2009_21

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