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Non-Linear Optical Properties of Matter pp 645–669Cite as

Second Harmonic Generation from Gold and Silver Nanoparticles in Liquid Suspensions

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Part of the book series: Challenges and Advances in Computational Chemistry and Physics ((COCH,volume 1))

Abstract

A general review of the second harmonic (SH) light scattered from aqueous suspensions of small gold and silver metallic particles is presented. The first part is devoted to the general theory of the SH generation from particles in order to discuss the incidence of the shape of the particles and the retardation effects of the electromagnetic fields on the total SH scattered field. The next part focuses on the problem of the polarization fields, a problem rather specific to metallic particles. Because of their strong polarizability and the possibility of resonance enhancements through surface plasmon (SP) excitations, the exciting field cannot be taken as the incident field only but rather as the superposition of the incident and the polarization fields. An illustration of this problem is presented with the determination of the exact origin of the SH response from metallic particles. This experimental section presents two different sets of data: the size dependence of the SH intensity and the polarization patterns recorded in the geometrical configuration of Hyper Rayleigh Scattering. SP resonance enhancements of the absolute values of the hyperpolarizabilities are then discussed before a presentation of the SH response of aggregating suspensions of particles and their possible applications is given

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Authors and Affiliations

  1. Laboratoire de Spectrométrie Ionique et Moléculaire, UMR CNRS 5579, Université Claude Bernard Lyon 1, 43 Boulevard du 11 Novembre 1918, 69622 Villeurbanne cedex, France

    Jérôme Nappa, Guillaume Revillod, Gaelle Martin, Isabelle Russier-Antoine, Emmanuel Benichou, Christian Jonin & Pierre-François Brevet

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  1. Jérôme Nappa
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  2. Guillaume Revillod
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  3. Gaelle Martin
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  4. Isabelle Russier-Antoine
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  5. Emmanuel Benichou
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  6. Christian Jonin
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  7. Pierre-François Brevet
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Editor information

Editors and Affiliations

  1. National Hellenic Research Foundation, Greece

    Manthos G. Papadopoulos

  2. Nicolaus Copernicus University, Poland

    Andrzej J. Sadlej

  3. Jackson State University, USA

    Jerzy Leszczynski

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Nappa, J. et al. (2006). Second Harmonic Generation from Gold and Silver Nanoparticles in Liquid Suspensions. In: Papadopoulos, M.G., Sadlej, A.J., Leszczynski, J. (eds) Non-Linear Optical Properties of Matter. Challenges and Advances in Computational Chemistry and Physics, vol 1. Springer, Dordrecht. https://doi.org/10.1007/1-4020-4850-5_20

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