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Ultrafast Optical Spectroscopy and Optical Control

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Ultrafast Dynamics of Quantum Systems

Part of the book series: NATO Science Series: B: ((NSSB,volume 372))

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Abstract

A pedagogical review of optical spectroscopy and control at the “impulsive” limit, defined as a time scale faster than the fundamental vibrational or molecular motion under examination, is presented. Optical absorption and stimulated Raman scattering in this limit are seen to result in coherent vibrational motion in molecules and materials. A theoretical description of impulsive absorption and stimulated Raman scattering is followed by a survey of illustrative examples in which time-resolved observations of molecular and collective vibrational excitations are recorded. The topic then turns to optical control, beginning with a discussion of femtosecond pulse shaping through which complex ultrafast optical waveforms needed for many control objectives are produced. Theoretical formulations for optical control are reviewed, and a series of examples illustrating optical control over molecules and materials is presented.

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  1. Department of Chemistry, Massachusetts Institute of Technology, Cambridge, MA, 02139, USA

    Timothy F. Crimmins, Richard M. Koehl & Keith A. Nelson

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  1. Boston College, Chestnut Hill, Massachusetts, USA

    Baldassare Di Bartolo  & Giulio Gambarota  & 

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Crimmins, T.F., Koehl, R.M., Nelson, K.A. (2002). Ultrafast Optical Spectroscopy and Optical Control. In: Di Bartolo, B., Gambarota, G. (eds) Ultrafast Dynamics of Quantum Systems. NATO Science Series: B:, vol 372. Springer, Boston, MA. https://doi.org/10.1007/0-306-47080-2_13

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