Abstract
The previous chapters have been devoted to summarizing the vast knowledge acquired about the single phonon vibrations of atoms in or near the surface and about atoms and molecules on the surface and their dispersion curves. This new knowledge was made possible largely thanks to the development of He atom scattering spectroscopy and the progress made in theoretical analysis. Single phonon inelastic scattering processes were implicit since only in this case is it possible to extract accurate phonon dispersion curves from the data. The high resolution of HAS spectroscopy, especially in its 3He-spin echo version also allows for the observation of dynamical phenomena far beyond the harmonic motion, like multiphonon processes involving low energy phonons or the diffusion of adsorbates on the surface. Moreover, the unique property of closed shell He atoms to exchange energy and momentum with the ion cores of the surface atoms via the virtual excitation of interposed electrons makes HAS also a valuable tool for investigating collective surface electron excitations in the THz domain. It therefore seems appropriate to discuss also some of these and other emerging areas of HAS research where new important insight can be expected in the future.
You see things; and you say “Why?” But I dream things that never were; and I say “Why not?”.
(George Bernard Shaw, Back to Methuselah, 1921)
Access this chapter
Tax calculation will be finalised at checkout
Purchases are for personal use only
References
See articles in Kinetics of Interface Reactions, ed. by M. Grunze, H.J. Kreutzer (Springer, Heidelberg, 1987)
J.R. Manson, Energy Transfer to Phonons in Atom and Molecule Collisions with Surfaces, in Handbook of Surface Science, ed., Vol. 3: Surface Dynamics, ed. by W.N. Unertl (North Holland, Amsterdam, 2008), pp. 53–93
V. Celli, D. Himes, P. Tran, J.P. Toennies, Ch. Wöll, G. Zhang, Phys. Rev. Lett. 66, 3160 (1991)
F. Hofmann, J.P. Toennies, J.R. Manson, J. Chem. Phys. 101, 10155 (1994)
F. Hofmann, J.P. Toennies, J.R. Manson, Surf. Sci. Lett. 349, L184 (1996)
F. Hofmann, J.P. Toennies, J.R. Manson, J. Chem. Phys. 106, 1234 (1997)
J.R. Manson, Comput. Phys. Commun. 80, 145 (1994)
J.R. Manson, Phys. Rev. B 43, 6924 (1991)
B. Gumhalter, A. Bilić, Surf. Sci. 370, 47 (1997)
B. Gumhalter, J. Phys.: Condens. Matter 24, 104015 (2012)
S. Daon, E. Pollak, J. Chem. Phys. 142, 174102 (2015)
B. Gumhalter, Phys. Rep. 351, 1–159 (2001)
J. Braun, D. Fuhrmann, M. Bertino, A.P. Graham, J.P. Toennies, Ch. Wöll, A. Bilić, B. Gumhalter, J. Chem. Phys. 106, 9911 and 9922 (1997)
A. Šiber, B. Gumhalter, J. Braun, A.P. Graham, M.F. Bertino, J.P. Toennies, D. Fuhrmann, Ch. Wöll, Phys. Rev. B 59, 5898 (1999)
J. Braun, D. Fuhrmann, J.P. Toennies, Ch. Wöll, A. Bilic, B. Gumhalter, Surf. Sci. 368, 232 (1996)
A. Šiber, B. Gumhalter, Ch. Wöll, J. Phys.: Cond. Matter 14, 5913 (2002)
A. Šiber, B. Gumhalter, Surf. Sci. 502–503, 422–428 (2002)
R.J. Glauber, Phys. Rev. 98, 1692 (1955); Phys. Rev. 131, 2766 (1963)
N. Terzi, in Collective Excitations in Solids, ed. by. B. Di Bartolo (Plenum, New York, 1983), pp. 149–181; G.M. Mazzucchelli, N. Terzi, Solid State Comm. 48, 679 (1983)
M. Li, J.R. Manson, A.P. Graham, Phys. Rev. B 65, 195404 (2002)
B. Gumhalter, D.C. Langreth, Phys. Rev. B 60, 2789 (1999)
F. Hofmann, J.P. Toennies, G. Benedek, unpublished
A. Graham, F. Hofmann, J.P. Toennies, J. Chem. Phys. 104, 5311 (1996)
C.F. McConville, D.P. Woodruff, K.C. Prince, G. Paducci, V. Chab, M. Surman, A.M. Bradshaw, Surf. Sci. 166, 221 (1986)
M. Li, J.R. Manson, A.P. Graham, Phys. Rev. B 63, 155410 (2001)
J.R. Manson, A.P. Graham, M. Li, J. Phys.: Cond. Matter 14, 6233 (2002)
A.P. Graham, F. Hofmann, J.P. Toennies, G.P. Williams, C.J. Hirschmugl, J. Ellis, J. Chem. Phys. 108, 7825 (1998)
G. Antczak, G. Ehrlich, Surface Diffusion (Cambridge University Press, Cambridge, 2010)
J.W.M. Frenken, J.P. Toennies, Ch. Wöll, Phys. Rev. Lett. 60, 1727 (1988)
J.W.M. Frenken, B.J. Hinch, J.P. Toennies, Ch. Wöll, Phys. Rev. B 41, 938 (1990)
T. Springer, in Springer Tracts in Modern Physics, vol. 64 (Springer, Berlin, 1972), p. 2
T. Springer, in Dynamics of Solids and Liquids by Neutron Scattering, ed. by S.W. Lovesey, T. Springer (Springer, Berlin, 1977), p. 255
M. Bèe, Quasielastic Neutron Scattering (Adam Hilgar, Bristol, 1988)
C.T. Chudley, R.J. Elliott, Proc. Phys. Soc. 77, 353 (1961)
A.C. Levi, R. Spadacini, G.E. Tommei, Surf. Sci. 121, 504 (1982)
J.W.M. Frenken, B.J. Hinch, in Helium Atom Scattering from Surfaces, ed. by E. Hulpke, Springer Series in Surface Sciences, vol. 27 (1992), p. 287
L. Van Hove, Phys. Rev. 95, 249 (1954)
G.H. Vineyard, Phys. Rev. 110, 999 (1958)
K.S. Singwi, A. Sjölander, Phys. Rev. 119, 863 (1960)
J.F. Van der Veen, J.W.M. Frenken, Surf. Sci. 251–252, 1 (1991)
A.P. Graham, F. Hofmann, J.P. Toennies, L.Y. Chen, S.C. Ying, Phys. Rev. B 56, 10567 (1997)
A.P. Graham, J.P. Toennies, Surf. Sci. 427(428), 1 (1999)
A.P. Graham, W. Silvestri, J.P. Toennies, in Surface Diffusion: Atomistic and Collective Processes, ed. by M. Tringides (Plenum Press, New York, 1997), p. 565
B.H. Choi, A.P. Graham, K.T. Tang, J.P. Toennies, J. Chem. Phys. 112, 10538 (2000)
J. Ellis, J.P. Toennies, Phys. Rev. Lett. 70, 2118 (1993)
J.V. Barth, Surf. Sci. Rep. 40, 75 (2000)
L.Y. Chen, S.C. Ying, Phys. Rev. Lett. 71, 4361 (1993)
J. Ellis, J.P. Toennies, Surf. Sci. 317, 99 (1994)
M. Diamant, S. Rahav, R. Ferrando, G. Alexandrowicz, J. Phys.: Condens. Matter 27, 125008 (2015)
A.P. Graham, F. Hofmann, J.P. Toennies, L.Y. Chen, S.C. Ying, Phys. Rev. Lett. 78, 3900 (1997)
T. Ala-Nissila, R. Ferrandos, S.C. Ying, Adv. Phys. 51, 949 (2002)
J. Ellis, A.P. Graham, F. Hofmann, J.P. Toennies, Phys. Rev. B 63, 195408 (2001)
R. Martinez-Casado, A.S. Sanz, G. Rojas-Lorenzo, S. Miret-Artés, J. Chem. Phys. 132, 054704 (2010). See also the preceding papers: R. Guantes, J.L. Vega, S. Miret-Artés, E. Pollak, J. Chem. Phys. (2003), 119, 2780 (2003) and R. Martínez-Casado, J.L. Vega, A.S. Sanz, S. Miret-Artés, Phys. Rev. Lett. 98, 216102 (2007)
G.J. Alexandrowicz, A.P. Jardine, H. Hedgeland, W. Allison, J. Ellis, Phys. Rev. Lett. 97, 156103 (2006)
A.L. Glebov, J.P. Toennies, S. Vollmer, Phys. Rev. Lett. 82, 3300 (1999)
F. Hofmann, W. Schöllkopf, J.P. Toennies, in Proceedings R. A. Welch Foundation, 38th Conference on Chemical Research, Chemical Dynamics of Transient Species (Houston TX, 1994), pp. 197–218
F. Hofmann, Ph.D. Dissertation (Göttingen University, Germany, 1995)
A.P. Graham, J.P. Toennies, Europhys. Lett. 42, 449 (1998)
F. Mezei, Z. Phys. 255, 146 (1972)
A.P. Jardine, J. Ellis, W. Allison, J. Phys.: Condens. Matter 14, 6173 (2002)
P. Fouquet, A.P. Jardine, S. Dworski, G. Alexandrowicz, W. Allison, J. Ellis, Rev. Sci. Inst. 76, 053109 (2005)
A.P. Jardine, H. Hedgeland, G. Alexandrowicz, W. Allison, J. Ellis, Prog. Surf. Sci. 84, 323 (2009)
A.P. Jardine, G. Alexandrowicz, H. Hedgeland, W. Allison, J. Ellis, Phys. Chem. Chem. Phys. 11, 3355 (2009)
R. Gähler, R. Golub, K. Habicht, T. Keller, J. Felber, Phys. B 229, 1 (1996)
B.A.J. Lechner, Studying Complex Surface Dynamical Systems Using Helium-3 Spin-Echo Spectroscopy, (Springer Theses, Springer Cham, Heidelberg 2014)
A.P. Graham, J.P. Toennies, J. Chem. Phys. 114, 1051 (2001)
G. Alexandrowicz, A.P. Jardine, P. Fouquet, S. Dworski, W. Allison, J. Ellis, Phys. Rev. Lett. 93, 156103 (2004)
P.R. Kole, H. Hedgeland, A.P. Jardine, W. Allison, J. Ellis, G. Alexandrowicz, J. Phys.: Condens. Matter 24, 104016 (2012)
P. Fouquet, R.A. Olsen, E.J. Baerends, J. Chem. Phys. 119, 509 (2003)
J.C. Tully, M. Gomez, J. Vac. Sci. Technol. A 11, 1914 (1993)
Q. Ge, D.A. King, J. Chem. Phys. 111, 9461 (1999)
Q. Ge, D.A. King, J. Chem. Phys. 114, 1053 (2001)
A.P. Graham, Surf. Sci. Rep. 49, 115 (2003)
A.P. Jardine, J. Ellis, W. Allison, J. Chem. Phys. 120, 8724 (2004)
R. Marquardt, F. Cuvelier, R.A. Olsen, E.J. Baerends, J.C. Tremblay, P. Saalfrank, J. Chem. Phys. 132, 074108 (2010)
P. Fouquet, H. Hedgland, A. Jardine, G. Alexandrowicz, W. Allison, J. Ellis, Phys. B 385–386, 269–271 (2006)
H. Hedgeland, P. Fouquet, A.P. Jardine, G. Alexandrowicz, W. Allison, J. Ellis, Nat. Phys. 5(8), 561–564 (2009)
P. Fouquet, M.R. Johnson, H. Hedgeland, A.P. Jardine, J. Ellis, W. Allison, Carbon 47, 2627 (2009)
G. Alexandrowicz, P.R. Kole, E.Y.M. Lee, H. Hedgeland, R. Ferrando, A.P. Jardine, W. Allison, J. Ellis, J. Am. Chem. Soc. 130, 6789–6794 (2008)
B.A.J. Lechner, M. Sacchi, A.P. Jardine, H. Hedgeland, W. Allison, J. Ellis, S.J. Jenkins, P.C. Dastoor, B.J. Hinch, J. Phys. Chem. Lett. 1953 (2013)
P. Rotter, B.A.J. Lechner, A. Morherr, D.M. Chisnall, D.J. Ward, A.P. Jardine, J. Ellis, W. Allison, B. Eckhardt, G. Witte, Nat. Mater. 397 (2016)
O.P. Godsi, G. Corem, Y. Alkoby, J.T. Cantin, R. Krems, M. Somers, J. Meyer, G.-J. Kroes, T. Maniv, G. Alexandrowicz, Nature Comm. 8, 15357 (2017)
R. Gomer, Rep. Prog. Phys. 53, 917 (1990)
M.F. Bertino, F. Hofmann, W. Steinhögl, J.P. Toennies, J. Chem. Phys. 105, 11297 (1996)
G.X. Cao, E. Nabighian, X.D. Zhu, Phys. Rev. Lett. 79, 3696 (1997)
M. Ondrejcek, W. Stenzel, H. Conrad, V. Chab, Z. Chvoj, W. Engel, A.M. Bradshaw, Chem. Phys. Lett. 215, 528 (1993)
S.K.S. Ma, F.W. de Wette, G.P. Alldredge, Surf. Sci. 78, 598 (1978)
L. Yang, T.S. Rahman, M.S. Daw, Phys. Rev. B 44, 13725 (1991)
A.N. Al-Rawi, A. Kara, T.S. Rahman, Phys. Rev. B 66, 165439 (2002)
J. Blomquist, P. Uvdal, Phys. Chem. Chem. Phys. 12, 14121 (2010)
T. Tanaka, A. Tajima, R. Moriizumi, C. Ostuma, Y. Tsunoda, M. Seto, S. Kitao, T. Mitsui, J.Phys. Soc. Japan 74, 1762 (2009)
S.P. Lewis, A.M. Rappe, Phys. Rev. Lett. 77, 5241 (1996)
J.L. Vega, R. Guantes, S. Miret-Artés, D.A. Micha, J. Chem. Phys. 121, 8580 (2004)
T.S. Rahman, J.D. Spangler, A. Al-Rawi, Surf. Sci. 502–503, 429–436 (2002)
I.S. Ulusoy, Y. Scribano, D.M. Benoit, A. Tschetschetkin, N. Maurer, B. Koslowski, P. Ziemann, Phys. Chem. Chem. Phys. 13, 612 (2011)
B.N.J. Persson, Phys. Rev. B 44, 3277 (1991)
B.N.J. Persson, Sliding Friction: Physical Principles and Applications (Springer, Heidelberg, 1998)
B.N.J. Persson, H. Ueba, Surf. Sci. 502–503, 18 (2002)
T. Komeda, Y. Kim, M. Kawai, B.N.J. Persson, H. Ueba. Science 295, 2055 (2002)
V.A. Ermoshin, A.K. Kazanski, K.S. Smirnov, D. Bougeard, J. Chem. Phys. 105, 9371 (1996)
S.P. Lewis, A.M. Rappe, Phys. Rev. Lett. 77, 5241 (1996)
K. Liu, S. Gao, Phys. Rev. Lett. 95, 226102 (2005)
A.P. Baddorf, E.W. Plummer, Phys. Rev. Lett. 66, 2770 (1991)
G. Benedek, J.P. Toennies, Phys. Rev. (Rapid Comm.) B46, 13643 (1992)
R.M. Nicklow, G. Gilat, H.G. Smith, L.J. Raubenheimer, M.K. Wilkinson, Phys. Rev. 164, 922 (1967)
E.C. Svensson, B.N. Brockhouse, J.M. Rowe, Phys. Rev. 155, 619 (1967)
G. Nilsson, R. Rolandson, Phys. Rev. B 7, 2393 (1973)
A. Larose, B.N. Brockhouse, Can. J. Phys. 49, 1990 (1976)
A.P. Miller, B.N. Brockhouse, Can. J. Phys. 49, 704 (1971)
H. Ibach, D.L. Mills, Electron Energy Loss Spectroscopy and Surface Vibrations (Academic Press, New York, 1982)
A. Reichmuth, Diplom Thesis (University of Göttingen, 1991)
M. Gester, D. Kleinhesselink, P. Ruggerone, J.P. Toennies, Phys. Rev. B 49, 5777 (1994)
L. Yang, T.S. Rahman, Phys. Rev. Lett. 67, 2327 (1991)
R. Zivieri, G. Santoro, V. Bortolani, Phys. Rev. B 59, 15959 (1999)
A.N. Al-Rawi, A. Kara, T.S. Rahman, Phys. Rev. B 66, 165436 (2002)
G. Alexandrowicz, A.P. Jardine, J. Phys.: Condens. Matter 19, 305001 (2007)
H.-J. Ernst, E. Hulpke, J.P. Toennies, Phys. Rev. B 46, 16081 (1992)
C.S. Jayanthi, E. Tosatti, L. Pietronero, Phys. Rev. B 31, 3456 (1985)
E. Tosatti, in The Structure of Surfaces II, ed. by J.F. van der Veen, et al. (Springer, Berlin, 1988), p. 535
G. Bracco, L. Bruschi, L. Pedemonte, R. Tatarek, Surf. Sci. 352, 964 (1996)
G. Bracco, L. Bruschi, R. Tatarek, A. Franchini, V. Bortolani, G. Santoro, Europhys. Lett. 34, 687 (1996)
G. Bracco, L. Bruschi, L. Pedemonte, R. Tatarek, Surf. Sci. 377, 325 (1997)
L. Pedemonte, G. Bracco, Phys. Rev. B 68, 205420 (2003)
L. Pedemonte, R. Tatarek, G. Bracco, Phys. Rev. B 66, 045414 (2002)
A. Fasolino, E. Tosatti, Phys. Rev. B 35, 4264 (1987)
C.Z. Wang, A. Fasolino, E. Tosatti, Europhys. Lett. 7, 263 (1988)
C.Z. Wang, A. Fasolino, E. Tosatti, Phys. Rev. B 37, 2116 (1988)
G. Piccini, J. Sauer, J. Chem. Theory Comput. 10, 2479 (2014)
H. Frank, H. Hoinkes, H. Wilsch, U. Wonka, Surf. Sci. 64, 362 (1974)
H.U. Finzel, H. Frank, H. Hoinkes, M. Luschka, H. Nahr, H. Wilsch, U. Wonka, Surf. Sci. 49, 577 (1975)
Y. Watanabe, A. Sakai, T. Sakurai, J. Phys. Soc. Jpn. 66(3), 649 (1974)
Y. Ekinci, J.P. Toennies. Surf. Sci. 563, 127–134 (2004)
E.G. McRae, R.A. Malic, Phys. Rev. Lett. 58, 1437 (1987); Phys. Rev. B 38, 13163 (1988)
M. Abraham, G. Lelay, J. Hila, Phys. Rev. B 41, 9828 (1990)
A. Mak, K.W. Evans-Lutterodt, K. Blum, D.Y. Noh, J.D. Brock, G.A. Held, R.J. Birgenau, Phys. Rev. Lett. 66, 2002 (1991)
N. Takeuchi, A. Selloni, E. Tosatti, Phys. Rev. Lett. 72, 2227 (1994)
N. Takeuchi, A. Selloni, E. Tosatti, Phys. Rev. B 49, 10757 (1994)
N. Takeuchi, A. Selloni, E. Tosatti, Phys. Rev. B 55, 15405 (1997)
S. Modesti, V.R. Dhanak, M. Sancrotti, A. Cantoni, B.N.J. Persson, E. Tosatti, Phys. Rev. Lett. 73, 1951 (1994)
A. Di Cicco, B. Giovenali, R. Gunnella, E. Principi, S. Simonucci, Solid State Commun. 134, 577–582 (2005)
A. Santoni, V.R. Dhanak, A. Goldoni, M. Sancrotti, S. Modesti, Europhys. Lett. 34, 275 (1996)
A.W. Denier van der Gon, J.M. Gay, J.W.M. Frenken, J.F. van der Veen, Surf. Sci. 241, 335 (1991)
T.T. Tran, S. Thevuthasan, Y.J. Kim, D.J. Friedman, A.P. Kaduwela, G.S. Herman, C.S. Fadley, Surf. Sci. 281, 270 (1993)
C.A. Meli, E.F. Greene, G. Lange, J.P. Toennies, Phys. Rev. Lett. 74, 2054 (1995)
A.L. Glebov, J.P. Toennies, S. Vollmer, G. Benedek, Europhys. Lett. 46, 369 (1999)
A.L. Glebov, J.P. Toennies, S. Vollmer, Phys. Rev. Lett. 82, 3300 (1999)
G. Lange, C.A. Meli, J.P. Toennies, Phys. Rev. B 56, 4642 (1997)
D. Cvetko, L. Floreano, A. Crottini, A. Morgante, F. Tommasini, Surf. Sci. 447, L147–L151 (2000)
C.A. Meli, E.F. Greene, J. Chem. Phys. 101, 7139 (1994)
X. Zeng, H.E. Elsayed-Ali, Surf. Sci. 497, 373–384 (2002)
H.C. Siegmann, J. Phys.: Condens. Matter 4, 8395–8434 (1992)
F.J. Himpsel, J.E. Ortega, G.J. Mankey. Adv. Phys. 47, 511–597 (1998)
O. Fruchart, A. Thiaville. C.R. Phys. 6, 921–933 (2005)
C.A.F. Vaz, J.A.C. Bland, G. Lauhoff. Rep. Prog. Phys. 71, 056501 (2008)
J.J. Hernández, S.A. Safron, J.G. Skofronick, J. Vac. Sci. Technol. A 13, 1416 (1995)
W. Allison, B. Feuerbacher, Phys. Rev. Lett. 45, 2040 (1980)
G. Brusdeylins, J.P. Toennies, Surf. Sci. 126, 647 (1983)
R.S. Timit, J.M. Daniels, A.D. May, Can. J. Phys. 49, 560 (1971)
G. Witte, Dissertation, University of Göttingen 1995 (Max Planck Institut für Strömungsforschung, Report no. 8/1995)
H.D. Hagstrum, Phys. Rev. 96, 325 (1954)
H. Conrad, G. Ertl, J. Küppers, S.W. Wang, Phys. Rev. Lett. 42, 1082 (1979)
Y. Harada, S. Masuda, H. Ozaki, Chem. Rev. 97, 1897–1952 (1997)
M. Marynowski, A. Swan, W. Franzen, M. El-Batanouny, K.M. Martini, Surf. Interface Anal. 23, 105 (1995)
A. Swan, M. Marynowski, W. Franzen, M. El-Batanouny, K.M. Martini, Phys. Rev. Lett. 71, 1250 (1993)
A. Swan, M. Marynowski, W. Franzen, M. El-Batanouny, K.M. Martini, J. Vac. Sci. Technol. A 12, 2219 (1994)
M. Marynowski, W. Franzen, M. El-Batanouny, V. Staemmler, Phys. Rev. B 60, 6053 (1999)
P. Fouquet, P.K. Day, G. Witte, Surf. Sci. 400, 140 (1998)
M. El-Batanouny, G. Murthy, C.R. Willis, S. Kais, V. Staemmler, Phys. Rev. B 58, 7391 (1998)
M. El-Batanouny, J. Phys.: Condens. Matter 14, 6281 (2002)
P. Banerjee, X. Liu, M. Farzaneh, C.R. Willis, W. Franzen, M. El-Batanouny, V. Staemmler, arXiv:cond-mat/0401130v1 (8 Jan 2004)
G. Witte, P. Senet, J.P. Toennies, Phys. Rev. B 58, 13264 (1998)
J.P. Toennies, G. Witte, A.M. Shikin, K.H. Rieder, J. Electr. Spectr. Rel. Phenom. 64/65, 677 (1993)
M. Kurahashi, T. Suzui, X. Ju, Y. Yamauchi, Phys. Rev. Lett. 91, 267203-1 (2003)
M. Kurahashi, Y. Yamauchi, Surf. Sci. 590, 21–30 (2005)
T. Suzuki, M. Kurahashi, X. Ju, Y. Yamauchi, Surf. Sci. 549, 97–102 (2004)
M. Kurahashi, X. Sun, Y. Yamauchi, Surf. Sci. 601, 1371–1376 (2007)
R. Moroni, M. Canapea, L. Mattera, Phys. Res. B 256, 438–441 (2007)
M. Kurahashi, Y. Yamauchi, Rev. Sci. Instrum. 77, 023904 (2006)
M. Kurahashi, S. Entani, Y. Yamauchi, Rev. Sci. Instrum. 79, 073902 (2008)
M. Kurahashi, X. Sun, Y. Yamauchi, Phys. Rev. B 86, 245421 (2012)
A. Pratt, M. Kurahashi, Y. Yamachi, J. Appl. Phys. 109, 07C111 (2011)
M. Kurahashi, A. Pratt, Y. Yamauchi, Surf. Sci. 605, 612–615 (2011)
S. Achilli, G.P. Brivio, G. Fratesi, M.I. Trioni, J. Phys. Chem. A 115, 8498–8503 (2011)
B. Rohwedder, Am. J. Phys. 75, 394 (2007)
S.K. Satija, R.P. Comes, G. Shirane, Phys. Rev. B 32, 3309 (1985)
T. Slezak, J. Lazewski, S. Stankov, K. Parlinski et al., Phys. Rev. Lett. 99, 066103 (2007)
G. Benedek, J.P. Toennies, G. Zhang, Phys. Rev. Lett. 68, 2644 (1992)
G. Zhang, Dissertation (University of Göttingen 1991 and Max-Planck-Institut für Strömungsforschung, Bericht 102/1991)
R.F. Sabiryanov, S.S. Jaswal, Phys. Rev. Lett. 83, 2062 (1999)
G. Benedek, E. Hulpke, W. Steinhögl, Phys. Rev. Lett. 87, 027201 (2001)
J. Thomassen, F. May, B. Feldmann, M. Wuttig, H. Ibach, Phys. Rev. Lett. 69, 3831 (1992)
M. Zharnikov, A. Dittschar, W. Kuch, C.M. Schneider, J. Kirschner, Phys. Rev. Lett. 76, 4620 (1996)
L. Hammer, S. Müller, K. Heinz, Surf. Sci. 569, 1–3 (2004)
T. Kraft, P.M. Marcus, M. Scheffler, Phys. Rev. B 49, 11511 (1994)
R. Lorenz, J. Hafner, Thin Solid Films 281–282, 482 (1996)
T. Asada, S. Blügel, Phys. Rev. Lett. 79, 507 (1997)
R. Kläsges, D. Schmitz, C. Carbone, W. Eberhardt, T. Kachel, Solid State Commun. 107, 13 (1998)
G. Benedek, M. Bernasconi, V. Chis, E. Chulkov, P.M. Echenique, B. Hellsing, J.P. Toennies, J. Phys.: Cond. Matter 22, 084020 (2010)
D. Li, M. Freitag, J. Pearson, Z.Q. Qiu, S.D. Baker, Phys. Rev. Lett. 72, 3112 (1994)
N. Memmel, Th. Detzel, Surf. Sci. 307–309, 490 (1994)
D. Spišàk, J. Hafner, Phys. Rev. B 61, 16129 (2000)
V.M. Silkin, A. García-Lekue, J.M. Pitarke, E.V. Chulkov, E. Zaremba, P.M. Echenique, Europhys. Lett. 66, 260 (2004)
S. Stankov, R. Röhlsberger, T. Slezak, M. Sladecek, B. Sepiol, G. Vogl, A.I. Chumakov, R. Rüffer, N. Spriridis, J. Lazewski, K. Parlinski, J. Korecki, Phys. Rev. Lett. 99, 185501 (2007)
W. Sturhahn, T.S. Toellner, E.E. Alp, X. Zhang, M. Ando, Y. Yoda, S. Kikuta, M. Seto, C.W. Kimball, B. Dabrowski, Phys. Rev. Lett. 74, 3832 (1995)
E.G. d’Agliano, P. Kumar, W. Schaich, H. Suhl, Phys. Rev. B 11, 2122 (1975)
A. Nourtier, J. Phys. (Paris) 38, 479 (1977)
R. Brako, D.M. Newns, Solid State Commun. 33, 713 (1980)
J.W. Gadzuk, H. Metiu, Phys. Rev. B 22, 2603 (1980)
J.K. Nørskov, B.I. Lundqvist, Surf. Sci. 89, 251 (1979)
G.P. Brivio, T.B. Grimley, J. Phys. C 10, 2351 (1977)
G.P. Brivio, T.B. Grimley, Surf. Sci. 89, 226 (1980)
K. Schönhammer, O. Gunnarsson, Z. Phys. B 38, 127 (1980)
K. Schönhammer, O. Gunnarsson, Phys. Rev. B 22, 1629 (1980)
O. Gunnarsson, K. Schönhammer, Phys. Rev. B 25, 2503 (1982)
O. Gunnarsson, K. Schönhammer, Phys. Rev. B 25, 2514 (1982)
B. Feuerbacher, R.F. Willis, Phys. Rev. Lett. 47, 526 (1981)
B. Feuerbacher, in Dynamics of Gas-Surface Interactions, ed. by G. Benedek, U. Valbusa (Springer, Heidelberg, 1982), p. 263
B. Diaconescu, K. Pohl, L. Vattuone, L. Savio, P. Hofmann, V.M. Silkin, J.M. Pitarke, E.V. Chulkov, P.M. Echenique, D. Farías, M. Rocca, Nature 448, 57 (2007)
S.J. Park, R.E. Palmer, Phys. Rev. Lett. 105, 016801 (2010)
K. Pohl, B. Diaconescu, G. Vercelli, L. Vattuone, V.M. Silkin, E.V. Chulkov, P.M. Echenique, M. Rocca, EPL 90, 57006 (2010)
L. Vattuone, G. Vercelli, M. Smerieri, L. Savio, M. Rocca, Plasmonics 7, 323 (2012)
L. Vattuone, M. Smerieri, T. Langer, C. Tegenkamp, H. Pfnür, V.M. Silkin, E.V. Chulkov, P.M. Echenique, M. Rocca, Phys. Rev. Lett. 110, 127405 (2013)
W.L. Schnaich, J. Harris, J. Phys. F 11, 65 (1981)
E. Hulpke, J. Lüdecke, Phys. Rev. Lett. 68, 2846 (1992)
E. Hulpke, J. Lüdecke, Surf. Sci. 287(288), 83 (1993)
J.M. Pitarke, V.M. Silkin, E.V. Chulkov, P.M. Echenique, Rep. Prog. Phys. 70, 1 (2007)
H. Yu, J.C. Hermanson, Phys. Rev. B 40, 11851 (1989)
H. Yu, J.C. Hermanson, Phys. Rev. B 41, 5991 (1990)
Y. Chen, J.C. Hermanson, G.J. Lapeyre, Phys. Rev. B 39, 12682 (1989)
J.I. Gersten, I. Wagner, A. Rosenthal, Y. Goldstein, A. Many, R.E. Kirby, Phys. Rev. B 29, 2458 (1984)
V.M. Silkin, J.M. Pitarke, E.V. Chulkov, P.M. Echenique, Phys. Rev. B 72, 115435 (2005)
J. Fritsch, U. Schröder, Phys. Rep. 309, 209 (1999)
R.H. Ritchie, J.C. Ashley, T.L. Ferrell, in Electromagnetic Surface Modes, ed. by A.B. Boardman (Wiley, Chichester, 1982), p. 119
G. Benedek, M. Pardo, J.P. Toennies, Theory of inelastic atom scattering from surface electron-hole and plasmon excitations, in Highlights on Spectroscopies of Semiconductors and Nanostructures, ed. by G. Guizzetti, A.C. Andreani, F. Marabelli, M. Patrini, Conference Proceedings, vol. 94 (SIF, Bologna, 2007), pp. 151–167
H. Nienhaus, Phys. Rev. B 56, 13194 (1997)
J. Braun, J.P. Toennies, C. Wöll, Phys. Rev. B 60, 11707 (1999)
G. Benedek, M. Bernasconi, D. Campi, P.M. Echenique, V.M. Silkin, E.V. Chulkov, D. Farías, D. Maccariello, J.P. Toennies (to be published)
P.R. Kole, Dynamics and Morphology of Metal and Metal Oxide Surfaces (Ph.D. Dissertation, University of Cambridge, 2011), and P.R. Kole, G. Benedek, ICSFS 16 Genova July 1–6, 2012—abstr. PLA 1.2
U. Fano, Phys. Rev. 124, 1866 (1961)
V. Chis, B. Hellsing, G. Benedek, M. Bernasconi, E.V. Chulkov, J.P. Toennies, Phys. Rev. Letters 101, 206102 (2008)
G. Lange, J.P. Toennies, Phys. Rev. B 53, 9614 (1996)
W. Menezes, P. Knipp, G. Tisdale, S.J. Sibener, Phys. Rev. B 41, 5648 (1990)
J. Lobo-Checa, T. Okuda, M. Hengsberger, L. Patthey, T. Greber, P. Blaha, J. Osterwalder, Phys. Rev. B 77, 075415 (2008)
N. Bundaleski, H. Khemliche, P. Soulisse, P. Roncin, Phys. Rev. Lett. 101, 177601 (2008)
A. Schüller, H. Winter, Phys. Rev. Lett. 100, 097602 (2008)
H. Khemliche, P. Rousseau, P. Roncin, V.H. Etgens, F. Finocchi, Appl. Phys. Lett. 95, 151901 (2009)
H. Winter, A. Schüller, Progr. Surf. Sci. 86, 169 (2011)
M. Busch, J. Lienemann, J. Seifert, A. Schüller, H. Winter, Vacuum 86, 1618 (2012)
J. Lienemann, D. Hülsewede, J. Seifert, K. Maass, M. Busch, H. Winter, Nucl. Instr. Meth. Phys. Res. B 315, 30 (2013)
M. Debiossac, A. Zugarramurdi, P. Lunca-Popa, A. Momeni, H. Khemliche, A.G. Borisov, P. Roncin, Phys. Rev. Lett. 112, 023203 (2014)
J. Seifert, J. Lienemann, A. Schuller, H. Winter, Nucl. Instrum. Meth. B 350, 99 (2015)
N.-P. Wang, M. Rohlfing, P. Krüger, J. Pollmann, Phys. Rev. B 67, 115111 (2003)
R.J. Glauber, Phys. Rev. 84, 395 (1951)
K. Huang, A. Rhys, Proc. R. Soc. (Lond.) A 204, 406 (1950); when referred to the multi-phonon sidebands of optical transitions S is known as Huang-Rhys exponent
H. Khemliche, J. Villette, P. Roncin, M. Barat, Nucl. Instrum. Methods Phys. Res. B 164, 608 (2000)
A.A. Lucas, M. Sunjic M, in Progress in Surface Science, vol. 2, ed. by S.G. Davison (Pergamon, New York, 1971)
G. Benedek, E. Mulazzi, Phys. Rev. 179, 906 (1969)
J. Villette, A. G. Borisov, H. Khemliche, A. Momeni, P. Roncin, Phys. Rev. Lett. 85, (2000)
A.A. Lucas, M. Sunjic, G. Benedek, P.M. Echenique, New. J. Phys. 16, 063015 (2014)
S. Suto, K.-D. Tsuei, E. W. Plummer, E. Burstein, Phys. Rev. Lett. 63, 2590 (1989)
H. Haberland, in Fundamental Processes of Atomic Dynamics, ed. by J.S. Brigss, H. Kleinpoppen, H.O. Lutz (Plenum Press, New York, 1988)
G. Benedek, T.P. Martin, G. Pacchioni (eds.), Elemental and Molecular Clusters (Springer, Heidelberg, 1988)
G. Scoles (ed.), The Chemical Physics of Atomic and Molecular Clusters (North-Holland, 1991)
U. Buck, R. Krohne, J. Siebers, Z. Phys. D 26, 169 (1993)
U. Buck, in Physics of Electronic And Atomic Collisions: XVIII International Conference, ed. by T. Andersen, B. Fastrup, F. Folkmann, H. Knudsen, N. Andersen, AIP Conference Proceedings, vol. 295, (1993), p. 719
U. Buck, R. Krohne, J. Chem. Phys. 105, 5408 (1996)
U. Buck, Surf. Rev. Lett. 3, 467 (1996)
U. Buck, R. Krohne, Phys. Rev. Lett. 73, 947 (1994)
U. Buck, R. Krohne, P. Lohbrandt, J. Chem. Phys. 106, 3205 (1997)
T. Schroder, R. Schinke, R. Krohne, U. Buck, J. Chem. Phys. 106, 9067 (1997)
T.A. Beu, C. Steinbach, U. Buck, J. Chem. Phys. 117, 3149 (2002)
J. Brudermann, P. Lohbrandt, U. Buck, Phys. Rev. Lett. 80, 2821 (1998)
J. Brudermann, U. Buck, E. Fredj, R.B. Gerber, M.A. Ratner, J. Chem. Phys. 111, 10069 (1999)
J. Brudermann, P. Lohbrandt, U. Buck, J. Chem. Phys. 112, 11038 (2000)
A. Glebov, A.P. Graham, A. Menzel, J.P. Toennies, P. Senet, J. Chem. Phys. 112, 11011 (2000)
R.B. Doak, in E. Hulpke (ed.) Helium Atom Scattering from Surfaces, (Springer, Berlin, 1992), pp. 5–24
B. Holst, W. Allison, Nature 390, 244 (1997)
K. Fladischer, H. Reingruber, T. Reisinger et al., New J. Phys. 12, 033018 (2010)
D. Barredo, F. Calleja, A.E. Weeks, P. Nieto, J.J. Hinarejos, G. Laurent, A.L. Vazquez de Parga, D. McLaren, D. Farias, W. Allison, R. Miranda, et al., Surf. Sci. 601, 24–29 (2007)
R.B. Doak, R.E. Grisenti, S. Rehbein, G. Schmal, J.P. Toennies, C. Wöll, Phys. Rev. Lett. 83, 4229 (1999)
D. Barredo, F. Calleja, P. Nieto, J.J. Hinarejos, G. Laurent, A.L. Vazquez de Parga, D. Farias, R. Miranda, Adv. Mater. 20, 3492–3497 (2008)
D. Barredo, G. Laurent, F. Calleja, P. Nieto, J.J. Hinarejos, G. Laurent, A.L. Vazquez de Parga, D. Farias, R. Miranda, Appl. Phys. Lett. 96, 081901 (2010)
G. Anemone, C. Weingarten, A. AlTaleb, C. Prieto, D. Farias, Appl. Phys. Lett. 111, 181602 (2017)
H.C. Schewe, B.S. Zhao, G. Meijer, W. Schöllkopf, New J. Phys. 11, 113030 (2009)
O. Carnal, M. Sigle, T. Sleator, H. Takuma, J. Mlynek, Phys. Rev. Lett. 67, 3231 (1991)
M. Koch, S. Rehbein, G. Schmahl et al., J. Microsc. 229, 1–5(2008)
S.D. Eder, T. Reisinger, M.M. Greve, G. Bracco, B. Holst, New J. Phys. 14, 073014 (2012)
P. Witham, E. Sanchez, Rev. Sci. Instr. 82, 103705 (2011)
P.J. Witham, E.J. Sanchez, J. of Microscopy 248, 223–227 (2012)
P. J. Witham, Master Thesis (2013), Portland State Univ
P. Witham, E. Sanchez, Cryst. Res. Technol. 49, 690–698 (2014)
A.S. Palau, G. Bracco, B. Holst, Phys. Rev. A 94, 063624 (2016)
M. Barr, A. Fahy, A. Jardine, J. Ellis, D. Ward, D.A. MacLaren, W. Allison, P.C. Dastoor, Nuc. Instr. Meth. Phys. Res. B 340, 76–80 (2014)
A. Fahy, M. Barr, J. Martens, P.C. Dastoor, Rev. Sci. Instrum. 86, 023704 (2015)
M. Barr, A. Fahy, J. Martens, J. Martens, A.P. Jardine, D.J. Ward, J. Ellis, W. Allison, P.C. Dastoor, Nat. Commun. 7, 10189 (2016)
P. Witham, private communication
H. Morgner, Adv. At. Mol. Opt. Phys. 42, 387–488 (2000)
E. Bauer, Rep. Prog. Phys. 57, 895 (1994)
N. Ueno, H. Yasufuku, S. Kera, K.K. Okudaira, Y. Harada, Lect. Notes Phys. 588, 131–144 (2002) (Springer, Berlin)
Y. Harada, S. Yamamoto, M. Aoki, S. Masuda, T. Ichinokawa, M. Kato, Y. Sakai, Nature 372, 657 (1994)
R. Castillo-Garza, J. Gardner, S. Zisman, M.G. Raizen, ACS Nano, 4378 (2013)
B.W. Ward, J.A. Notte, N.P. Economou, J. Vac. Sci. Technol. B 24, 2871 (2006)
N. Klingner, R. Heller, G. Glawacek, J. Von Borany, J. Notte, J. Huang, S. Facsko, Ultramicroscopy 162, 91–97 (2016)
Author information
Authors and Affiliations
Corresponding author
Rights and permissions
Copyright information
© 2018 Springer-Verlag GmbH Germany, part of Springer Nature
About this chapter
Cite this chapter
Benedek, G., Toennies, J.P. (2018). Experimental Results: Beyond Single Phonons. In: Atomic Scale Dynamics at Surfaces. Springer Series in Surface Sciences, vol 63. Springer, Berlin, Heidelberg. https://doi.org/10.1007/978-3-662-56443-1_13
Download citation
DOI: https://doi.org/10.1007/978-3-662-56443-1_13
Published:
Publisher Name: Springer, Berlin, Heidelberg
Print ISBN: 978-3-662-56441-7
Online ISBN: 978-3-662-56443-1
eBook Packages: Physics and AstronomyPhysics and Astronomy (R0)