Abstract
Self-phase modulation (SPM) is the principal mechanism responsible for the generation of picosecond and femtosecond white-light supercontinua. When an intense ultrashort pulse propagates through a medium, it distorts the atomic configuration of the material, which changes the refractive index. The pulse phase is time modulated, which causes the generation of new frequencies. This phase modulation originates from the pulse itself (self-phase modulation). It can also be generated by a copropagating pulse (cross-phase modulation).
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Baldeck, P.L., Ho, P.P., Alfano, R.R. (1989). Cross-Phase Modulation: A New Technique for Controlling the Spectral, Temporal, and Spatial Properties of Ultrashort Pulses. In: Alfano, R.R. (eds) The Supercontinuum Laser Source. Springer, New York, NY. https://doi.org/10.1007/978-1-4757-2070-9_4
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