Keywords

1 Extended English/Spanish abstract

Most volcanic systems on Earth are characterized by chemically different magmas that can be found in the erupted products throughout their history, either in synchronous eruptive episodes, or in different epochs of volcanic activity. This chemical heterogeneity can have multiple reasons, and it originates from deep in the mantle, due to variations in the source and/or crustal assimilation during ascent, to shallower crustal regions, where processes such as fractional crystallization or mixing and mingling take place. Magma chamber rejuvenation comprises some of the aforementioned processes at shallow level. Whenever a magma intrudes from the mantle to shallower depths and encounters an already established storage zone (a magma chamber or reservoir), the magma already emplaced gets rejuvenated by the incoming more primitive magma. Magmas rising from the deep regions of a volcano feeding system are typically characterized by higher temperatures, larger volatile contents and more primitive, mantle-like compositions. On the other hand, magmas that have resided at shallower depths for a while (years to thousands of years) have evolved by fractional crystallization, thus they have changed their composition towards a more felsic one, and have lost most of their gaseous phase, that can escape towards the surface. The interaction between primitive and evolved magmas varies the physical and chemical properties of both the end-members involved. Typically, volatile-rich magmas coming from depth are lighter than degassed shallow magma, albeit having a higher liquid density: they are characterized by a much larger gas content. The light magma tends to rise inside the denser reservoir; a gravitational instability sets in as the two magmatic mixtures come into contact, and generates convection inside the reservoir. As a consequence, intense mingling and mixing are generated among the two end-members. These dynamic interactions cause variations in the physical and chemical properties of the magmas themselves, that loose their identity as initial end-members and become a more homogeneous mixture. The volcanic system as a whole enters an unrest scenario, that can evolve to eruption or not depending on the specific conditions. Numerical simulations of a magmatic system representing magma injection into a shallow reservoir show that mixing is very intense at the time of contact, and can be efficient on time scales of hours to day in homogeneizing the system. Depending on the geometry of the volcano feeding system, and even more on the volatile content of the incoming and resident magmas, the process can be suppressed or enhanced. Sills favour mixing, while more vertically elongated, dike-like reservoirs slow the dynamical interactions. As the presence of a gaseous phase is the engine of the gravitational instability that triggers the dynamics, a higher volatile content, which translates into a higher gas content, in the deep regions of the feeding system strongly accelerates the rejuvenation process. As mixing patterns are found almost ubiquitously in products from volcanoes around the world, comparison of the observed features to the model predictions can provide insights on the features of magma chamber rejuvenation, including the time scales over which mixing processes are efficient and possibly the timings for the evolution towards an eruption or not. Coupling to models that describe the visco-elastic response of the host rock to stress variations within the magmatic system provides hints as to how to identify recharge processes at depth from the analysis of geophysical signals observed at the surface. Characteristic features of ground deformation associated to convection and mixing is the appearance of oscillation of exremely long period, on the order of hours (Ultra-Long-Period, ULP), that can be detected by instruments such as continuous tiltmeters and dilatometers. Their records can identify the onset of the interaction among different magmas, thus provide time scales for unrest duration and evolution.

2 Introduction

Magmas evolve in many ways during their residence time within the crust, determining whether they are going to be erupted or not. Magma chamber rejuvenation takes place whenever a magma intruding from the mantle to shallower depths encounters an already established storage zone (i.e. a magma chamber or reservoir). It can involve many different processes such as reheating and melting of the residing magmas, fractional crystallization due to changes in the pressure and temperature conditions, mingling and mixing among the different components; typically, it takes place at shallow crustal depths. Magmas rising from depth are often characterized by higher temperatures, larger volatile contents and more primitive, mantle-like compositions with respect to those that have been residing at shallower levels for a while (months, years to thousands of years). This general scenario can have a variety of declinations, depending on the specific setting and physico-chemical characteristics of the magmatic mixtures involved. The shallow magma can be highly crystalline, a mush, that can be rejuvenated by the heat from the incoming component (Bachmann and Bergantz 2003, 2008; Girard and Stix 2009; Bain et al. 2013; Till et al. 2015); or, at the other end, it can still be hot and more fluidal, especially if injection episodes are frequent (Voight et al. 2010), giving rise to mixing and mingling phenomena (Montagna et al. 2015). The interaction among the deep and shallow components changes the physical and chemical properties of both the involved magmatic end-members, triggering an unrest phase that can evolve to eruption or not depending on the specific conditions. Evidence of chamber rejuvenation both in igneous and in intrusive rocks, manifested mostly by mingling and mixing patterns, is almost ubiquitous at volcanic systems worldwide, and it is often invoked as eruption trigger.

Magma movement at depth implies mass re-distribution, pressure changes, and pressure transients which translate into variations in the gravity field, shape and slope of the volcano flanks, and seismic signals registered at the surface. Understanding the complex relationships between quantities measured by volcano monitoring networks and shallow magma processes is a crucial step for the comprehension of volcanic processes and in evaluating more realistic hazard forecast. The ability to detect the onset of magma recharge at depth is fundamental as it can provide hints to unrest duration and evolution, and possibly eruption timings.

In this work we describe a forward-modeling approach to describe magma chamber dynamics, specifically for what concerns rejuvenation episodes, and link it to the geophysical observables that are expected as a consequence. This provides a framework for the consistent interpretation of geological and geophysical records of unrest periods at active volcanoes. This methodology allows for identification of rejuvenation episodes in ground deformation records, and possibly discrimination between those episodes that lead to eruption or not.

3 Numerical Simulations of Magma Chamber Rejuvenation

3.1 Magmatic System

We refer as an archetypal case to the Phlegraean Fields magmatic system, where seismic imaging and attenuation tomographies have identified a huge (probably around 10 km wide) magma reservoir at a depth of around 8 km (Zollo et al. 2008; De Siena et al. 2010), while a variety of geophysical and geochemical evidence suggests that smaller (probably less than 1 km3), shallower batches of magma have been forming throughout the caldera history at virtually any depth smaller than 9 km (Arienzo et al. 2010; Di Renzo et al. 2011). These shallow magma bodies have been identified as actively involved in past eruptions, which at least in some cases shortly followed the arrival of volatile-rich, less differentiated magmas from the deep feeding system (Arienzo et al. 2009; Fourmentraux et al. 2012). Chemical compositions of erupted magmas range from shoshonitic to trachytic to phonolitic; geochemical analyses on melt inclusions suggest a variety of processes contributing to this variability, such as recharge from depth, intra-chamber mixing, syn-eruptive mingling (Arienzo et al. 2010; Fourmentraux et al. 2012). The same analyses show that deep magmas are typically rich in gas, especially CO2 (Mangiacapra et al. 2008), while shallow magmas are unusually crystal-poor, down to less than 3 wt% (Arienzo et al. 2009). To study the magmatic dynamics occurring as a consequence of a recharge event, we simplify the magmatic system retaining its most peculiar features. We model the injection of CO2-rich shoshonitic magma coming from a deep reservoir into a shallower, much smaller chamber, containing more evolved and partially degassed phonolitic magma (see Table 1 for compositions). The two chambers are connected by a dyke. This idealized layout captures several first-order characteristics of prototype magmatic systems, including a composite structure, vertical extension, and heterogeneous composition, and it approximates systems composed by long-lived, interconnected multiple reservoirs believed to exist at many active volcanoes (Elders et al. 2011).

Table 1 Composition of the phonolite and shoshonite magma types employed in the simulations

Figure 1 shows the system domain for the numerical simulations. We assume one of the horizontal dimensions of the magmatic system to be much larger than the other, so that our domain is two-dimensional. The deep chamber is elliptical, 1 km thick and 8 km wide; its top is at 8 km depth. The geometry of the shallow chamber has been varied as shown in Fig. 1, keeping its surface area fixed. In the elliptical cases, the semi-axes measure 400 and 800 m, respectively, while the circular chamber has a radius of 283 m.

Fig. 1
figure 1

Initial conditions for the numerical simulations of the magmatic system. On the left, the whole domain is shown, indicating the two magmatic end-members. On the right, the upper portion of the domain shows the three different geometries explored

The initial conditions of the system are also shown in Fig. 1. The shallow chamber hosts a differentiated, volatile-poor phonolitic magma. Its volatile content has been varied from 0.3 wt% CO2 and 2.5 wt% H2O to 0.1 wt% CO2 and 1 wt% H2O. In the feeding dyke and deep reservoir is a less evolved, basaltic shoshonite, containing 1 wt% CO2 and 2 wt% H2O. Such a low water content in the phonolitic end-member derives from melt inclusion data from Phlegrean Fields (Arienzo et al. 2010). Typically, more evolved magmas are expected to have a relatively larger water content (Signorelli et al. 2001; Cannatelli et al. 2007; Pappalardo et al. 2007; Mollo et al. 2015), resulting possibly in smaller density contrasts at the interface among the two magmas thus less efficient mixing dynamics.

Volatiles partitioning between gaseous and liquid phases is computed following Papale et al. (2006) as a function of composition and pressure. Pressure at time 0 consists of a depth-dependent magmastatic contribution superimposed to the host rock confining pressure. The interface between the two magmas, at the inlet of the shallow chamber, is gravitationally unstable, the lower magma being less dense due to its higher gas content. The dynamics is solely driven by buoyancy, without any external forcing.

The density contrast at the interface varies for each simulated scenario, as it depends on both volatiles content and their partitioning between liquid and gaseous phases; volatiles exsolution in turn depends on pressure, thus on the depth at which the interface is placed, which is different for each geometry of the shallow chamber (Fig. 1). Temperature differences between interacting magmas are often negligible (Sparks et al. 1977), particularly at Phlegraean Fields (Mangiacapra et al. 2008; Arienzo et al. 2010), thus the system is assumed isothermal. As a result, there is no need to speculate on the thermal status of the surrounding rock, thus reducing model uncertainties. Moreover, heat transfer effects are expected to play a minor role on the short simulated time scales (hours; Di Renzo et al. 2011).

3.2 Magma Dynamics

Interaction among the two magmas develops as a consequence of the initial gravitational instability at the interface. We solve numerically the two-dimensional space-time evolution of the system, consisting of a mixture of two different magmatic components, each of them including a liquid (silicate melt and dissolved volatiles) and a gaseous (exsolved volatiles) fractions. The equations of motion for the mixture express conservation of mass for each component k = 1, 2, and momentum for the whole mixture (Longo et al. 2012a):

figure a
figure b

In the above, t is time; \( \rho \) is mixture density,

figure c

is mass fraction of component k, u is fluid velocity, Dk is the k-th coefficient of mass diffusion, p is pressure, μ is viscosity and g is gravity acceleration.

The magmatic mixture is considered ideal. Its density is evaluated as weighted sum of the components’ densities; for each component, density is calculated using a non-ideal equation of state for the liquid phase, real gas properties and ideal mixture laws for multiphase fluids. Mixture viscosity is computed through standard rules of mixing for one phase mixtures and with a semi-empirical relation in order to account for the effect of non-deformable gas bubbles. Liquid viscosity is modeled as in Giordano et al. (2008), and it depends on liquid composition and dissolved water content. The assumption of Newtonian rheology is justified by the very low strain rates and the crystal-free nature of the magmas. The generalized Fick’s law is used to describe mass diffusion. Volatile partitioning between gaseous and liquid phases is evaluated at every point in the space-time domain as function of mixture composition and pressure as in Papale et al. (2006). All the physical properties of the two magmas are evaluated at every point in the space-time domain depending on the local conditions of pressure, velocity and mass fractions, which are the unknowns in Eqs. (1) and (2). The equations are solved numerically using GALES, a finite element C++ code specifically designed for volcanic fluid dynamics (Longo et al. 2012a).

The evolution in space and time of the system is complex and presents a number of interesting features. Figure 2 summarizes the results regarding magma dynamics, showing the evolution of composition in time in the shallow chamber for the five different simulation scenarios.

Fig. 2
figure 2

Snapshots of variation of composition with time in the shallower parts of the system for the different simulations. Columns correspond to different simulations; rows correspond to different times

The initial inverse density contrast at the contact interface between the two magmas gives rise to convective mass transfer from the deeper parts of the system to shallower depths and vice versa. The unstable density contrast is solely due to the different volatile content of the two mixtures: the shoshonitic melt has an higher density than the phonolitic. The role played by volatiles is crucial, and it is exsolved gases that ultimately determine the buoyant dynamics. A Rayleigh-Taylor instability develops, which acts to bring the system to gravitational equilibrium by overturning it. The instability develops starting from the perturbed interface, with a first plume of light material that rises into the chamber. Depending on the initial density contrast as well as on the geometry of the shallow chamber, the initial plume starts developing at different times. The dynamics is strongly enhanced by higher density contrasts; geometry also plays an important role when density contrasts are similar, with horizontally elongated, sill-like chambers favouring convection with respect to more dyke-like setups (see also Fig. 2).

Plumes of light magma coming from depth keep entering the shallow reservoir as discrete filaments, following irregular trajectories and showing typical convective patterns. The lighter material tends to rise into the chamber, thereby decreasing more and more its density as volatiles exsolve in lower-pressure environments; on the other hand, the denser magmatic mixture initially residing in the chamber sinks into the feeder dyke, increasing its density by the reverse process of volatile dissolution at higher pressures. The plumes thus progressively increase their buoyancy, enhancing their expansion and acceleration. During the rise, vortexes form at the head of the plumes and subsequent plumes interact among themselves, further favouring mixing. The dynamics creates complicated patterns that maximize the interaction among the two different magmatic mixtures (Petrelli et al. 2011). Mingling is evident for all simulated conditions both within the chamber itself and even more in the feeding dyke (Fig. 2), and it is strongly intensified by the chaotic patterns that form as a consequence of deep magma injection.

Independently from system geometry or density contrast at the interface, mingling is very efficient in the feeding dyke, more than inside the upper chamber. Figure 2 shows that since the very beginning of the simulations, the magma entering the chamber is already a mixture of the two initial end-members, and not the pure shoshonitic composition.

As the dynamics proceeds, faster for higher density contrasts and sill-like setups, the gas-rich mixture tends to accumulate at the top of the chamber, thereby originating a stable density stratification that has indeed been testified at various magmatic systems (Arienzo et al. 2009). The stratification is more prominent in vertically elongated, dyke-like reservoirs (Fig. 2). The density profile along the vertical direction, evaluated averaging along horizontal planes (Fig. 3), illustrates that a quasi-stable profile is reached after some hours of simulated time.

Fig. 3
figure 3

Total mixture density averaged over horizontal planes as function of depth for simulation 1, at different times. The inset shows the upper 5 km of the domain; the black line represents the quasi-equilibrium density profile at the end of the simulation

As time proceeds, convection slows down due to smaller buoyancy of the incoming already mixed component, and the instability proceeds in time asymptotically: the more the two end-members have mingled, the less intense is convection.

The evolution of pressure in the system is highly heterogeneous in space and time. Alternating phases dominated by buoyancy and sinking at chamber inlet result in pressure fluctuations with periods of hundreds of seconds and amplitudes decreasing with time (Fig. 4). Typically pressure variations are smaller than 1 MPa; under these conditions, it is unlikely that rejuvenation can trigger eruption, as the stresses needed to create a pathway to the surface in the host rock are typically larger than that (Gudmundsson 2006).

Fig. 4
figure 4

Pressure variations as a function of time at a point on the boundary of the upper chamber, for simulation #1. The upper diagram shows the difference between the local pressure at current time and at time zero, while the bottom diagram shows the same quantity after subtraction of a detrending function (red curve in the upper diagram)

3.3 Ground Deformation

Determining the time–space-dependent ground displacement requires modeling the magma–rocks boundary conditions and the mechanical response of rocks, the latter depending on heterogeneous rock properties, presence and distribution of faults, interfaces, fluids, and volcano topography (e.g., O’Brien and Bean 2004). A first-order analysis performed here assumes magma–rock one-way coupling and adopts the Green’s functions formulation for a homogeneous, infinite medium (Aki and Richards 2002).

We consider as point sources the fluid dynamics computational grid nodes located at the reservoir walls. As source time functions, we use the respective temporal evolutions of magmatic forces computed from pressures and stresses provided at those nodes by the numerical simulations of magma convection and mixing dynamics. Ground displacement at a series of virtual receivers is finally obtained by integrating, over all sources, the Green’s functions associated with individual sources.

Continuity of pressure and stress is taken as the boundary condition along the non moving magma–rock interface. Physical properties of rocks are homogeneous averages that describe the volcanic edifices within the range of considered depths (<10 km, vP = 3000 m/s; vP/vS = 1/√3, ρ = 2500 kg/m3).

Propagation of pressure disturbances in the host rock medium reveals that the computed pressure oscillations, originated by the ingression of buoyant magma in the magma chamber, translate into Ultra Long Period ground displacement dynamics with amplitudes of millimeter to micrometer order (Fig. 5; Longo et al. 2012b). ULP ground movements like those predicted by the present modeling could not be detected by classical broadband seismometers (although more recent seismometers extend their working range up to 100–200 s periods), while they are visible in the records from other instruments, especially borehole dilatometers characterized by high signal-to-noise ratio (Sacks et al. 1971).

Fig. 5
figure 5

Synthetic seismic signal (blue detrended as to represent an instrumental record, black filtered [0.001,0.01] Hz) and corresponding frequency spectrum for the vertical component at all synthetic stations. Example from simulation #1

4 Discussion and Conclusions

The arrival of fresh magma into an already emplaced reservoir and the consequent internal dynamics have often been invoked as possible eruption triggers, especially at Phlegraean Fields (Arienzo et al. 2010); on the other hand, footprints of magma chamber rejuvenation are often found in intrusive granites as well, testifying that it does not necessarily lead to eruption. Magma chamber rejuvenation can thus be regarded as a prototypical volcanic unrest process, that can lead to eruption or not depending on the specific system conditions (e.g. host rock compliance, volume and volatile content of injected magma).

The time scales for rejuvenation processes to be effective in magmatic reservoirs are relatively short, on the order of hours. This is consistent with what has been observed from the analyses of erupted products (Fourmentraux et al. 2012) as well as from experiments on diffusive fractionation (Perugini et al. 2010), and opens a completely new perspective in terms of unrest duration: indications of mixing in erupted products suggest that recharge events can happen within a very short time frame from eruption, otherwise the evidence would be wiped out by the efficient mixing process (Montagna et al. 2015).

In terms of geophysical observables, convective mingling dynamics in magmatic reservoirs is associated with ultra-long-period seismic signals, characterized by frequencies in the range 10−2 − 10−4 Hz (Longo et al. 2012b).

The results obtained by our modeling specifically refer to the Phlegraean system. They can be extended to many other volcanoes where evidence of rejuvenation has been observed in similar magmatic settings, characterized by relatively primitive magmas that are not very different in composition and temperature, such as e.g. Mount Etna (Viccaro et al. 2006) or Stromboli (La Felice et al. 2011). For more evolved magmas, reservoirs can be dominated by crystal-rich regions (Marsh 1981; Koyaguchi and Kaneko 1999; Bachmann and Bergantz 2004; Hildreth 2004; Huber et al. 2009; Cooper and Kent 2014), and they are often at a lower temperature. The approach described above must be applied with caution in such cases, as the dynamics of the incoming primitive magma is more likely to be described as flow through a porous medium (mush) than as fluid mingling and mixing. Nonetheless, there is some evidence for crystal-poor silicic magma reservoirs to be reactivated as well (Bachmann et al. 2002; Deering et al. 2011; Huber et al. 2012; Sliwinski et al. 2015; Wolff et al. 2015).

Given the short time scales over which the dynamical processes described here can be effective and lead to eruption, it would be beneficial to be able to routinely detect the signals described above for eruption forecasting and mitigation actions. This is especially true for long-dormant volcanoes such as Phlegraean Fields, one of the highest-risk volcanic areas in the world given the large population living within the caldera borders (Arienzo et al. 2010), for which there is still no widely accepted means of discriminating the precursors of an impending eruption (Druitt et al. 2012).