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Orthogonal Supramolecular Interaction Motifs for Functional Monolayer Architectures

  • Book
  • © 2012

Overview

Authors:
  1. Mahmut Deniz Yilmaz

    1. , Department of Chemistry, Northwestern University, Evanston, USA

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  • Nominated by the University of Twente, Netherlands, for a SpringerTheses Prize
  • Describes the development and design of new monolayer-based sensing platforms as chemical and biosensors
  • Provides a wide range of application examples of the new sensor systems - from biological problems to nanoelectronic and spintronic devices
  • Includes supplementary material: sn.pub/extras
  • Includes supplementary material: sn.pub/extras

Part of the book series: Springer Theses (Springer Theses)

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Table of contents (7 chapters)

  1. Front Matter

    Pages i-xix
    Download chapter PDF

  2. General Introduction

    • Mahmut Deniz Yilmaz
    Pages 1-2

  3. Orthogonal Supramolecular Interaction Motifs for Functional Monolayer Architectures

    • Mahmut Deniz Yilmaz
    Pages 3-26

  4. Expression of Sensitized Eu3+ Luminescence at a Multivalent Interface

    • Mahmut Deniz Yilmaz
    Pages 27-43

  5. Ratiometric Fluorescent Detection of an Anthrax Biomarker at Molecular Printboards

    • Mahmut Deniz Yilmaz
    Pages 45-56

  6. A Supramolecular Sensing Platform in a Microfluidic Chip

    • Mahmut Deniz Yilmaz
    Pages 57-70

  7. Local Doping of Silicon Using Nanoimprint Lithography and Molecular Monolayers

    • Mahmut Deniz Yilmaz
    Pages 71-89

  8. Fabrication of Two-Dimensional Organic Spin Systems on Gold

    • Mahmut Deniz Yilmaz
    Pages 91-100

  9. Back Matter

    Pages 101-101
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Keywords

About this book

Deniz Yilmaz' thesis describes a combination of orthogonal supramolecular interactions for the design of functional monolayer architectures on surfaces, that can be used as chemical and biosensors in a wide range of applications. The term “orthogonal supramolecular interactions” refers to non-covalent interactions that do not influence each other's assembly properties. Orthogonal self-assembly thus allows extended control over the self-assembly process and promotes new materials properties. The first part of the thesis employs orthogonal host-guest and lanthanide-ligand coordination interaction motifs to create supramolecular luminescent monolayers. The second part of the thesis describes the fabrication of functional monolayers on silicon and gold substrates for applications in electronics.
The results illustrate the power of weak supramolecular interactions to direct the immobilization of functional systems on surfaces. The combination of host-guest and lanthanide-ligand coordination interaction motifs on surfaces demonstrates that hybrid, multifunctional supramolecular monolayers can be fabricated by integrating different non-covalent interactions in the same system. This combination opens up new avenues for the fabrication of complex hybrid organic-inorganic materials and stimuli-responsive surfaces. Their utility is demonstrated through applications of the functional interfaces to biosensing and nanotechnology.

Authors and Affiliations

  • , Department of Chemistry, Northwestern University, Evanston, USA

    Mahmut Deniz Yilmaz

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