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Stabilizing and scaling up carbon-based perovskite solar cells

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Abstract

Organometal trihalide perovskite solar cells (PSCs) have sparked a frantic excitement in the scientific community because they can achieve high power conversion efficiencies (PCEs) even when fabricated by low-cost solution-processing technologies. However, the poor stability of PSCs has seriously hindered their commercialization. Among various kinds of PSCs, carbon-based PSCs without hole transport materials (C-PSCs) seem to be the most promising for addressing the stability issue because carbon materials are stable, inert to ion migration, and inherently water-resistant. Concurrent with the steady rise in PCE of C-PSCs, great progresses have also been attained on the device stability and scaling-up fabrication of C-PSCs, which have well signified the possible commercialization of PSCs in the near future. In this review, we will summarize these progresses with a view of exposing the promising prospect. We start by collating recent stability testing results of C-PSCs with reference to those of HTM-PSCs. Then, we update the research status on large-scale C-PSCs and their associated scalable fabrication technologies. Finally, we identify main issues to be addressed alongside future research directions.

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ACKNOWLEDGMENTS

This work is financially supported by the Young Talent of “Zhuoyue” Program of Beihang University, the National Natural Science Foundation of China (Nos. 51371020 and 21603010), the HK-RGC General Research Funds (GRF Nos. 16312216 and 16300915), and the HK Innovation and Technology Fund (ITS/219/16).

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  1. School of Materials Science and Engineering, Beihang University, Beijing, 100191, People’s Republic of China

    Haining Chen

  2. Department of Chemistry, The Hong Kong University of Science and Technology, Kowloon, Hong Kong, China

    Shihe Yang

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Chen, H., Yang, S. Stabilizing and scaling up carbon-based perovskite solar cells. Journal of Materials Research 32, 3011–3020 (2017). https://doi.org/10.1557/jmr.2017.294

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