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Theoretical and Experimental Studies of Third-Order Nonlinear Optical Susceptibilities of New p-N,N′-Diamethylaniline Tetrathiafulvalene Derivatives

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Abstract

A study was made of third-order nonlinear optical susceptibilities of new tetrathiafulvalene (TTF) derivatives, using the degenerate four wave mixing (DFWM) method, as well as complex quantum chemical calculations. To understand the physical nature of the optical nonlinearities, we separated their electronic and nuclear contributions. We found that the electronic contribution to these nonlinearities predominated. Our investigations suggest that TTF may be a highly promising material for nonlinear optics (NLO).

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Authors and Affiliations

  1. Laboratoire POMA, UMR CNRS 6136, Universite d’Angers, France

    B. Sahraoui

  2. Institute of Physics WSP, Al, Amii Krajowej 13/15, 42217, Czcestochowa, Poland

    M. Makowaska-Janusik & I. V. Kityk

  3. Laboratoire IMMO, UMR CNRS 6501, Universite d’Angers, France

    M. Salle & A. Gorgues

  4. Military University of Technology, 2 Kaliski Str., 00-908, Warsaw, Poland

    K. J. Pluciński

Authors
  1. B. Sahraoui
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  2. K. J. Pluciński
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  3. M. Makowaska-Janusik
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  4. I. V. Kityk
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  5. M. Salle
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  6. A. Gorgues
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Sahraoui, B., Pluciński, K.J., Makowaska-Janusik, M. et al. Theoretical and Experimental Studies of Third-Order Nonlinear Optical Susceptibilities of New p-N,N′-Diamethylaniline Tetrathiafulvalene Derivatives. MRS Online Proceedings Library 660, 825 (2000). https://doi.org/10.1557/PROC-660-JJ8.25

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  • DOI: https://doi.org/10.1557/PROC-660-JJ8.25

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