Abstract
In this paper, we first describe and then demonstrate the soundness of a new experimental method that is designed to deliver a wide range of accurately measured nucleation rates of solids in supercooled liquid Si. The method utilizes thin-film processes, as well as laser-quenching and detection techniques, in order to first induce isothermal transformation and then extract the corresponding solid nucleation rates over a frequency range potentially greater than ten orders of magnitude. The technological and scientific gains that can result from acquiring such information are discussed.
Similar content being viewed by others
References
G. Devaud and D. Turnbull, Appl. Phys. Lett. 46, 844 (1985).
Yan Shao and Frans Spaepen, see this volume.
Y. -W. Kim, H. -M. Lin, and T. F. Kelly, Acta Metall. 37, 247 (1989).
D. Dutarte, J. Appl. Phys. 59, 1977 (1986).
S. R. Stiffler, M. O. Thompson, P. S. Peercy, Phys. Rev. Lett. 60, 2519 (1988).
T. Eiumchotchawalit and James S. Im, Mat. Res. Soc. Symp. Proc. 321, 725 (1994).
James S. Im, H. J. Kim, and M. O. Thompson, Appl. Phys. Lett. 63, 1969 (1993).
James S. Im and H. J. Kim, Appl. Phys. Lett. 64, 2303 (1994).
James S. Im and Robert S. Sposili, Materials Research Society Bulletin, vol. xxi, no. 3, 39 (1996).
H. Jin Song and James S. Im, accepted for publication in Appl. Phys. Lett.
J. H. Hollomon and D. Turnbull, “Nucleation”, in Progress in Metal Physics, 4: 333 (1953).
D. M. Herlach, Mat. Sci. Eng., R12, 177 (1994).
W. A. Tiller, The Science of Crystallization: Microscopic Interfacial Phenomena (Cambridge University Press, Cambridge, UK, 1991).
D. Turnbull, J. Chem. Phys. 18, 768 (1950).
G. M. Pound and V. K. La Mer, J. Am. Chem. Soc. 74, 2323 (1952).
The program was obtained from M. O. Thompson, Department of Materials Science and Engineering, Cornell University, Ithaca, NY.
S. A. Cohen, T. O. Sedgwick, and J. L. Speidel, Mat. Res. Soc. Symp. Proc. 23, 321 (1984).
B. Chalmers, Principles of Solidification (John Wiley & Sons, New York, 1964).
M. O. Thompson, J. W. Mayer, A. G. Cullis, H. C. Webber, N. G. Chew, J. M. Poate, and D. C. Jacobson, Phys. Rev. Lett. 50, 896 (1983).
Vikas V. Gupta, H. Jin Song, and James S. Im, accepted for publication in Mat. Res. Soc. Symp. Proc. 397, (1996).
James S. Im, H. Tomita, and C. V. Thompson, Appl. Phys. Lett. 51, 685 (1987).
Author information
Authors and Affiliations
Rights and permissions
About this article
Cite this article
Jin Song, H., Im, J.S. A New Experimental Method for Investigating the Nucleation Kinetics of Solids in Supercooled Liquid Si. MRS Online Proceedings Library 398, 93–98 (1995). https://doi.org/10.1557/PROC-398-93
Published:
Issue Date:
DOI: https://doi.org/10.1557/PROC-398-93