Abstract
We present femtosecond differential reflectivity studies of few-layer graphene from weak to strong excitation regime. Temporal profiles of the differential reflectivity exhibit strong non-exponential decay. A nonlinear, cubic root dependence of their peak amplitudes on the pump fluence is clearly observed under relatively high intensity excitation, which indicates three-particle decay of transient carrier population via Auger scattering. Our results identify the critical role of such three-particle scattering in the initial electronic relaxation in photo-excited graphene with increasing phase-space filling of the correlated Dirac Fermions.
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References
- 1.
A. K. Geim, A. K., Novoselov, K. S., Nature Materials, 6, 183 (2007).
- 2.
Hupalo, M., Conrad, E., and Tringides, M. C. Phys. Rev. B 80, 041401 (2009).
- 3.
Dawlaty J. M.; Shivaraman S.; Strait J.; George P.; Chandrashekhar M.; Rana F.; Spencer M. G.; Veksler D.; Chen Y. Appl. Phys. Lett. 93, 131905 (2008)
- 4.
Dawlaty J. M.; Shivaraman S.; Chandrashekhar M.; Rana F.; Spencer M. G. Appl. Phys. Lett. 92, 042116 (2008)
- 5.
George P.; Strait J.; Dawlaty J.; Shivaraman S.; Chandrashekhar M.; Rana F.; Spencer M. G. Nano. Lett. 8, 12, 4248–4251 (2008)
- 6.
Choi H.; Borondics F.; Siegel D. A.; Zhou S. Y.; Martin M. C.; Lanzara A.; Kaindl R. A. Appl. Phys. Lett. 94, 172102 (2009)
- 7.
D. Sun, et al., Phys. Rev. Lett 101, 157402 (2008).
- 8.
M. Ghanassi, M., et al., Appl. Phys. Lett, 62, 78 (2008).
- 9.
Huang, L., et al., Phys. Rev. Lett. 96, 057407 (2006).
- 10.
Htoon. H., et al., Phys. Rev. Lett. 91, 227401 (2003).
- 11.
Bostwick, A., Ohta, T., Seyller, T., Horn, K., and Rotenberg, E., Nature Physics, 3, 36 (2007).
- 12.
Rana F. Phys Rev. B 76 155431 (2007).
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Li, T., Luo, L., Hupalo, M. et al. Ultrafast Dynamics of Highly Excited Dirac Fermions in Few-Layer Graphene: Evidence for Three-Particle Auger Scattering. MRS Online Proceedings Library 1230, 206 (2009). https://doi.org/10.1557/PROC-1230-MM02-06
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