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Lowest frequency mode in Raman susceptibility: 2-propanol from ambient to supercritical condition

  • Yuko AmoEmail author
  • Takuya Hasegawa Sato
  • Yasuo Kameda
  • Takeshi Usuki
Regular Article
  • 12 Downloads

Abstract

We report the first observation of the low-frequency Raman spectra of 2-propanol from ambient to supercritical condition. Phenomenological analysis is applied to the reduced Raman spectra. The low-frequency component is decomposed into two components: the lowest mode represented by a MRT(multiple random telegraph) model and the 2nd mode represented by a modified Gaussian. Only the characteristic time of the lowest mode sensitively depends on density and decreases with increasing density. The integrated intensity of each mode is proportional to the density.

Graphical abstract

Keywords

Solid State and Materials 

Notes

Author contribution statement

All the authors were involved in the preparation of the manuscript. All the authors have read and approved the final manuscript.

References

  1. 1.
    S. Kinoshita, Y. Kai, M. Yamaguchi, T. Yagi, Phys. Rev. Lett. 75, 148 (1995) ADSCrossRefGoogle Scholar
  2. 2.
    S. Kinoshita, Y. Kai, M. Yamaguchi, T. Yagi, Chem. Phys. Lett. 236, 259 (1995) ADSCrossRefGoogle Scholar
  3. 3.
    G. Brinbaum,Phenomena Induced by Intermolecular Interactions (Plenum Press, New York, 1985) Google Scholar
  4. 4.
    G.C. Tabisz, M.N. Neuman,Collision- and Interacion-Induced Spectroscopy (Kluwer Academic Pulishers, Dordrecht, 1995) Google Scholar
  5. 5.
    R. Biswas, A. Das, H. Shirota, J. Chem. Phys. 141, 134506 (2014) ADSCrossRefGoogle Scholar
  6. 6.
    S. Kakinuma, H. Shirota, J. Phys. Chem. B 122, 6033 (2018) CrossRefGoogle Scholar
  7. 7.
    N. Nishi, K. Koga, C. Ohshima, K. Yamamoto, U. Nagashima, K. Nagami, J. Am. Chem. Soc. 110, 5426 (1988) CrossRefGoogle Scholar
  8. 8.
    K. Mizoguchi, Y. Hori, Y. Tominaga, J. Chem. Phys. 97, 1961 (1992) ADSCrossRefGoogle Scholar
  9. 9.
    Y. Amo, Y. Tominaga, J. Chem. Phys. 109, 3994 (1998) ADSCrossRefGoogle Scholar
  10. 10.
    Y. Amo, Y. Tominaga, Physica A 276, 401 (2000) ADSCrossRefGoogle Scholar
  11. 11.
    R. Böhmer, C. Gainaru, R. Richert, Phys. Rep. 125, 545 (2014) Google Scholar
  12. 12.
    J. Watanabe, Y. Watanabe, S. Kinoshita, Chem. Phys. Lett. 333, 113 (2001) ADSCrossRefGoogle Scholar
  13. 13.
    G.E. Walrafen, Y.C. Chu, G.J. Piermarini, J. Phys. Chem. 100, 10363 (1996) CrossRefGoogle Scholar
  14. 14.
    B.K.P. Scaife,Principles of Dielectrics (Oxford University Press, Oxford, 1989) Google Scholar
  15. 15.
    F. Shibata, C. Uchiyama, K. Maruyama, Physica A 161, 42 (1989) ADSCrossRefGoogle Scholar
  16. 16.
    Y. Amo, Y. Kameda, T. Usuki, AIP Adv. 6, 055319 (2016) ADSCrossRefGoogle Scholar
  17. 17.
    M. Ban, S. Kitajima, K. Maruyama, F. Shibata, Phys. Lett. A 372, 351 (2008) ADSMathSciNetCrossRefGoogle Scholar
  18. 18.
    M. Ricci, P. Bartolini, R. Chelli, G. Cardini, S. Califano, R. Righini, Phys. Chem. Chem. Phys. 3, 2795 (2001) CrossRefGoogle Scholar
  19. 19.
    F. Palombo, P. Sassi, M. Paolantoni, C. Barontini, A. Morresi, M.G. Giorgini, J. Phys. Chem. B 118, 215 (2014) CrossRefGoogle Scholar
  20. 20.
    S. Kakinuma, S. Ramati, J.F. Wishart, H. Shirota, J. Chem. Phys. 148, 193805 (2018) ADSCrossRefGoogle Scholar
  21. 21.
    B. Schmidtke, N. Petzold, B. Pötzschner, H. Weingärtner, E.A. Rössler, J. Phys. Chem. B 118, 7108 (2014) CrossRefGoogle Scholar
  22. 22.
    Q. Zhong, J.T. Fourkas, J. Phys. Chem. B 112, 15342 (2008) CrossRefGoogle Scholar
  23. 23.
    T. Hasegawa, Y. Tanimura, J. Phys. Chem. B 115, 5545 (2011) CrossRefGoogle Scholar
  24. 24.
    J. Martí, J.A. Padró, E. Guàrdia, J. Mol. Liq. 64, 1 (1995) CrossRefGoogle Scholar
  25. 25.
    M.C.C. Ribeiro, J. Chem. Phys. 134, 244507 (2011) ADSCrossRefGoogle Scholar
  26. 26.
    D. Sidler, M. Meuwly, P. Hamm, J. Chem. Phys. 148, 244504 (2018) ADSCrossRefGoogle Scholar
  27. 27.
    H. Yada, M. Nagai, K. Tanaka, Chem. Phys. Lett. 473, 279 (2009) ADSCrossRefGoogle Scholar
  28. 28.
    M. Hou, A. Yu, R. Lu, J. Raman Spectr. 48, 108 (2016) ADSCrossRefGoogle Scholar
  29. 29.
    Y.J. Chang, E.W. Castner jr., J. Phys. Chem. 100, 3330 (1996) CrossRefGoogle Scholar
  30. 30.
    T. Bancewicz, A. Kamiński, J. Mol. Liq. 146, 35 (2009) CrossRefGoogle Scholar
  31. 31.
    G. Knopp, P. Radi, M. tulej, T. Gerber, P. Beaud, J. Chem. Phys. 118, 8223 (2003) ADSCrossRefGoogle Scholar
  32. 32.
    G.C. Schatz, M.A. Ratner,Quantum Mechanics in Chemistry, (Prentice Hall, USA 1993) Google Scholar
  33. 33.
    G.-Z. Jia, Q. Jie, W. Feng, J. Mol. Struct. 1100, 354 (2015) ADSCrossRefGoogle Scholar
  34. 34.
    Y. Amo, Y. Tominaga, Physica A 265, 410 (1999) ADSCrossRefGoogle Scholar
  35. 35.
    J. Watanabe, M. Watanabe, S. Kinoshita, Phys. Rev. B 74, 132105 (2006) ADSCrossRefGoogle Scholar

Copyright information

© EDP Sciences / Società Italiana di Fisica / Springer-Verlag GmbH Germany, part of Springer Nature 2020

Authors and Affiliations

  • Yuko Amo
    • 1
    Email author
  • Takuya Hasegawa Sato
    • 1
  • Yasuo Kameda
    • 1
  • Takeshi Usuki
    • 1
  1. 1.Yamagata University 1-4-12 Kojirakawa-machiYamagataJapan

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