Abstract
A cross section database on excitation functions of reactions produced by charged particles is essential for many areas of nuclear research. Particularly, accurate knowledge on nuclear cross sections for the cyclotron production of radioisotopes is very important for nuclear medicine. In the present paper, the cross section calculations for the production of 43,44Sc, 45Ti, 51Cr, 54Mn, and 55Fe radioisotopes were carried out by the use of ALICE/ASH code using the Fermi gas model, Kataria Ramamurthy Fermi gas model, and superfluid nuclear model for nuclear level density. Thereby, these model calculations were compared with the available measured data.
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References
F. Szelecsenyi, Measurement of cross sections of proton induced nuclear reactions on Ti, Ni, Zn, Cd, and Au up to 30 MeV and their application in radioisotope production, PhD Thesis (Lajos Kossuth University, Hungary) (1997)
S.M. Qaim, Radiochemical determination of nuclear data for theory and applications. J. Radioanal. Nucl. Chem. 284, 489 (2010). https://doi.org/10.1007/s10967-010-0460-5
M. Yiǧit, New empirical formulae for (n,t) cross sections at 14.6 MeV. Appl. Radiat. Isot. 128, 307 (2017). https://doi.org/10.1016/j.apradiso.2017.07.047
M. Yiğit, Theoretical predictions of excitation functions of neutron-induced reactions on 6Li, 9Be, 12C and 23Na nuclei at low energies. J. Fusion Energy 34, 140 (2015). https://doi.org/10.1007/s10894-014-9773-7
J. Luo, C. Wu, L. Jiang, L. He, Cross sections for d-3H neutron interactions with samarium isotopes. Radiochim. Acta 104, 523 (2016). https://doi.org/10.1515/ract-2016-0001
C. Yalçın, The cross section calculation of 112Sn(α, γ)116Te reaction with different nuclear models at the astrophysical energy range. Nucl. Sci. Tech. 28, 113 (2017). https://doi.org/10.1007/s41365-017-0267-y
M. Yiğit, E. Tel, Theoretical determination of (d, n) and (d,2n) excitation functions of some structural fusion materials irradiated by deuterons. Nucl. Sci. Tech. 28, 165 (2017). https://doi.org/10.1007/s41365-017-0316-6
C.W. Ma, J.L. Xu, An empirical formula for isotopic yield in Fe + p spallation reactions. J. Phys. G Nucl. Part Phys. 44, 125101 (2017). https://doi.org/10.1088/1361-6471/aa90e6
C.W. Ma, C.J. Lv, G.Q. Zhang et al., Neutron-induced reactions on AlF3 studied using the optical model. Nucl. Instrum. Methods Phys. Res. B 356–357, 42 (2015). https://doi.org/10.1016/j.nimb.2015.04.060
C.J. Lv, C.W. Ma, Y.P. Liu, An investigation on γ induced activation reactions on human essential elements. Nucl. Sci. Tech. 26, 030503 (2015). https://doi.org/10.13538/j.1001-8042/nst.26.030503
IAEA. Proceedings of the IAEA Consultants, Meeting on nuclear data for medical radioisotope production, Tokyo (Japan) (1987). http://www-nds.iaea.org/. Accessed 19 June 2017
M. Yiğit, E. Tel, Nuclear model calculation for production of 18F, 22Na, 44,46Sc, 54Mn, 64Cu, 68Ga, 76Br and 90Y radionuclides used in medical applications. Ann. Nucl. Energy 69, 44 (2014). https://doi.org/10.1016/j.anucene.2014.01.036
M.U. Khandaker, K. Kim, M.W. Lee et al., Investigations of the natTi(p, x) 43,44 m,44 g,46,47,48Sc, 48 V nuclear processes up to 40 MeV. Appl. Rad. Isot. 67, 1348 (2009). https://doi.org/10.1016/j.apradiso.2009.02.030
E. Koumarianou, D. Pawlak, A. Korsak et al., Comparison of receptor affinity of natSc-DOTA-TATE versus natGa-DOTA-TATE. Nucl. Med. Rev. 14, 85 (2011). https://doi.org/10.5603/NMR.2011.00021
F. Roesch, Scandium-44: benefits of a long-lived PET radionuclide available from the (44)Ti/(44)Sc generator system. Curr. Radiopharm. 5, 187 (2012). https://doi.org/10.2174/1874471011205030187
M. Al-Abyad, I. Spahn, S.M. Qaim, Experimental studies and nuclear model calculations on proton induced reactions on manganese up to 45 MeV with reference to production of 55Fe, 54Mn and 51Cr. Appl. Rad. Isot. 68, 2393 (2010). https://doi.org/10.1016/j.apradiso.2010.06.013
M. Sadeghi, M. Enferadib, H. Nadib, 45Ti, a candidate for positron emission tomography: study of the cyclotron production. Radiochemistry 53, 411 (2011). https://doi.org/10.1134/S106636221104014X
C.H.M. Broeders, A. Yu. Konobeyev, Yu. A. Korovin et al., FZK 7183, ALICE/ASH manual (2006). http://bibliothek.fzk.de/zb/berichte/FZKA7183.pdf. Accessed 19 June 2017
Experimental Nuclear Reaction Data (EXFOR), (2017). https://www-nds.iaea.org/exfor/exfor.htm. Accessed 19 June 2017
A.J. Koning, D. Rochman, J. Kopecky et al., TENDL-2015: TALYS-based evaluated nuclear data library. http://www.talys.eu/home/. Accessed 19 June 2017
M. Sadeghi, N. Soheibi, T. Kakavand et al., Targetry and nuclear data for the cyclotron production of 55Fe via various reactions. J. Radioanal. Nucl. Chem. 293, 1 (2012). https://doi.org/10.1007/s10967-012-1719-9
M. Sadeghi, M. Enferadi, Nuclear model calculations on the production of 119Sb via various nuclear reactions. Ann. Nucl. Energy 38, 825 (2011). https://doi.org/10.1016/j.anucene.2010.11.014
M. Sadeghi, N. Zandi, M. Bakhtiari, Nuclear model calculation for cyclotron production of 61Cu as a PET imaging. J. Radioanal. Nucl. Chem. 292, 777 (2012). https://doi.org/10.1007/s10967-011-1557-1
M. Sadeghi, M. Bakhtiari, M.K. Bakht et al., Overview of mercury radionuclides and nuclear model calculations of 195Hgm, g and 197Hgm, g to evaluate experimental cross section data. Phys. Rev. C 85, 034605 (2012). https://doi.org/10.1103/PhysRevC.85.034605
M. Sadeghi, M. Enferadi, M. Aref et al., Nuclear data for the cyclotron production of 66Ga, 86Y, 76Br, 64Cu and 43Sc in PET imaging. Nukleonika 55, 293 (2010)
M. Yiğit, Investigating the (p, n) excitation functions on 104–106,108,110Pd isotopes. Appl. Rad. Isot. 130, 109 (2017). https://doi.org/10.1016/j.apradiso.2017.09.027
M. Yiğit, A. Kara, Model-based predictions for nuclear excitation functions of neutron-induced reactions on 64,66−68Zn targets. Nucl. Eng. Technol. 49, 996 (2017). https://doi.org/10.1016/j.net.2017.03.006
M.E. Korkmaz, M. Yiğit, O. Ağar, Excitation functions of neutron induced nuclear reactions for 59Co nucleus using different level density models. Acta Phys. Pol. A 132, 670 (2017). https://doi.org/10.12693/APhysPolA.132.670
M. Yiğit, E. Tel, Study on (n,2n) and (n, p) reactions of strontium nucleus. Nucl. Eng. Des. 293, 97 (2015). https://doi.org/10.1016/j.nucengdes.2015.07.043
H. Korkut, T. Korkut, A. Kara et al., Monte carlo simulations of 17.9–22.3 MeV energetic proton irradiation effects on bcc-zirconium fusionic materials. J. Fusion Energ. 35, 591–596 (2016). https://doi.org/10.1007/s10894-016-0068-z
M. Yiğit, E. Tel, Theoretical study of deuteron induced reactions on 6,7Li, 9Be and 19F targets. Kerntechnik 79, 63 (2014). https://doi.org/10.3139/124.110394
E. Tel, M. Yiğit, G. Tanır, Cross sections calculations of (d, t) nuclear reactions up to 50 MeV. J. Fusion Energy 32, 273 (2013). https://doi.org/10.1007/s10894-012-9564-y
V.F. Weisskopf, D.H. Ewing, On the yield of nuclear reactions with heavy elements. Phys. Rev. 57, 472 (1940). https://doi.org/10.1103/PhysRev.57.472
M. Blann, Hybrid model for pre-equilibrium decay in nuclear reactions. Phys. Rev. Lett. 27, 337 (1971). https://doi.org/10.1103/PhysRevLett.27.337
M. Blann, H.K. Vonach, Global test of modified pre-compound decay models. Phys. Rev. C 28, 1475 (1983). https://doi.org/10.1103/PhysRevC.28.1475
A.V. Ignatyuk, G.M. Smirenkin, A. Tishin, Phenomenological description of energy dependence of the level density parameter. Sov. J. Nucl. Phys. 21, 255 (1975)
A.V. Ignatyuk, K.K. Istekov, G.N. Smirenkin, Role of collective effects in the systematics of nuclear level densities. Yadernaja Fizika 29, 875 (1979)
S.K. Kataria, V.S. Ramamurthy, M. Blann et al., Shell-dependent level densities in nuclear reaction codes. Nucl. Instrum. Methods Phys. Res. A 288, 585 (1990). https://doi.org/10.1016/0168-9002(90)90155-Y
V.N. Levkovskij, Book:Levkovskij, Act Cs. by Protons and Alphas (USSR, Moscow, 1991)
R. Ejnisman, I.D. Goldman, P.R. Pascholati et al., Cross sections for 45Sc(p,2n)44Ti and related reactions. Phys. Rev. C 54, 2047 (1996). https://doi.org/10.1103/PhysRevC.54.2047
J.W. Meadows, R.M. Diamond, R.A. Sharp, Excitation functions and yield ratios for the isomeric pairs Br 80,80 m, Co58,58 m, and Sc44,44 m formed in (p, pn) reactions. Phys. Rev. 102, 190 (1956). https://doi.org/10.1103/PhysRev.102.190
T. Mcgee, C.L. Rao, G.B. Saha et al., Nuclear interactions of 45Sc and 68Zn with protons of medium energy. Nucl. Phys. A 150, 11 (1970). https://doi.org/10.1016/0375-9474(70)90451-3
A.J. Howard, H.B. Jensen, M. Rios et al., Measurement and theoretical analysis of some reaction rates of interest in silicon burning. Astrophys. J. 188, 131 (1974). https://doi.org/10.1086/152694
R.G. Thomas, W. Bartolini, Excitation functions for (p, n) and (p,2n) interactions in Sc, Cr, Mo, Cd and W between 8 and 14 MeV. Nucl. Phys. A 106, 323 (1968). https://doi.org/10.1016/0375-9474(67)90877-9
F. Ditroi, F. Tarkanyi, S. Takacs et al., Activation cross sections of longer lived products of proton induced nuclear reactions on manganese up to 70 MeV. Nucl. Instrum. Methods Phys. Res. B 308, 34 (2013). https://doi.org/10.1016/j.nimb.2013.04.058
R. Michel, G. Brinkmann, On the depth-dependent production of radionuclides (44 ≤ A≤59) by solar protons in extraterrestrial matter. J. Radioanal. Nucl. Chem. 59, 467 (1980). https://doi.org/10.1007/BF02517298
M. Gusakow, G. Albouy, N. Poffe et al., Reactions (p, pn) a moyenne energie. Journal de Physique 22, 636 (1961). https://doi.org/10.1051/jphysrad:019610022010063600
R.C. Albert, (p, n) Cross section and proton optical-model parameters in the 4 to 5.5 MeV energy region. Phys. Rev. 115, 925 (1959). https://doi.org/10.1103/PhysRev.115.925
C.H. Johnson, C.C. Trail, A. Galonsky, Thresholds for (p, n) reactions on 26 intermediate weight nuclei. Phys. Rev. 136, B1719 (1964). https://doi.org/10.1103/PhysRev.136.B1719
G.F. Dell, W.D. Ploughe, H.J. Hausman, Total reaction cross sections in the mass range 45 to 65. Nucl. Phys. 64, 513 (1965). https://doi.org/10.1016/0029-5582(65)90576-6
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Yiğit, M. Model-based cross section calculations on production of 43,34Sc, 45Ti, 51Cr, 54Mn, and 55Fe radioisotopes. NUCL SCI TECH 29, 55 (2018). https://doi.org/10.1007/s41365-018-0394-0
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DOI: https://doi.org/10.1007/s41365-018-0394-0