Skip to main content

Advertisement

Log in

Groundwater hydrogeochemical characteristics and quality suitability assessment for irrigation and drinking purposes in an agricultural region of the North China plain

  • Original Article
  • Published:
Environmental Earth Sciences Aims and scope Submit manuscript

Abstract

Eighty-one samples from both shallow and deep aquifers were collected and analyzed to reveal groundwater hydrogeochemical characteristics and estimate groundwater quality suitability for irrigation and drinking purposes based on groundwater quality indexes models including the sodium adsorption ratio (SAR), residual sodium carbonate (RSC), solute sodium percentage (%Na), magnesium hazard (MH), permeability index (PI) and health risk model. The results from groundwater quality suitability assessment indicated that shallow groundwater in the most part of the study region was suitable for irrigation regardless of EC, RSC and MH, while groundwater from the deep aquifer was suitable for irrigation purpose in nearly all parts of the study region. 24.49% and 14.29% of the deep groundwater sampling locations presented high fluoride (F) concentrations exceeded the Grade III value (1 mg/L) from Quality Standard for Groundwater of China and the maximum permissible value of 1.5 mg/L recommended by the WHO for drinking use, respectively. Non-carcinogens hazard quotient (HQ) values of NO3–N, NH4+–N, NO2–N, Fe, and Mn with the exception of F were all within the acceptable safety limit (HQ < 1). Efficient strategies and scientific decisions were suggested for groundwater resource protection and water quality improvements should be adopted for sustainable groundwater exploitation.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig. 1
Fig. 2
Fig. 3
Fig. 4
Fig. 5

Similar content being viewed by others

References

  • Abboud IA (2018) Geochemistry and quality of groundwater of the Yarmouk basin aquifer, north Jordan[J]. Environ Geochem Health 40(4):1405–1435

    Article  Google Scholar 

  • AbdEl-Aziz SH (2017) Evaluation of groundwater quality for drinking and irrigation purposes in the north-western area of Libya (Aligeelat)[J]. Environ Earth Sci 76(4):1–7

    Google Scholar 

  • Adimalla N, Li P (2019) Occurrence, health risks, and geochemical mechanisms of fluoride and nitrate in groundwater of the rock-dominant semi-arid region, Telangana State, India[J]. Hum Ecol Risk Assess Int J Spec Issue Sustain Living Risks 25(1–2):81–103

    Article  Google Scholar 

  • Adimalla N, Qian H (2019) Groundwater quality evaluation using water quality index (WQI) for drinking purposes and human health risk (HHR) assessment in an agricultural region of Nanganur, south India[J]. Ecotoxicol Environ Saf 176:153–161

    Article  Google Scholar 

  • Adimalla N, Venkatayogi S (2017) Mechanism of fluoride enrichment in groundwater of hard rock aquifers in Medak, Telangana State, South India[J]. Environ Earth Sci 76(1):45

    Article  Google Scholar 

  • Adimalla N, Li P, Venkatayogi S (2018a) Hydrogeochemical evaluation of groundwater quality for drinking and irrigation purposes and integrated interpretation with water quality index studies[J]. Environ Process 5(2):363–383

    Article  Google Scholar 

  • Adimalla N, Vasa SK, Li P (2018b) Evaluation of groundwater quality, Peddavagu in Central Telangana (PCT), South India: an insight of controlling factors of fluoride enrichment[J]. Model Earth Syst Environ 4(2):841–852

    Article  Google Scholar 

  • Aghapour S, Bina B, Tarrahi MJ, Amiri F, Ebrahimi A (2018) Distribution and health risk assessment of natural fluoride of drinking groundwater resources of Isfahan, Iran, using GIS[J]. Environ Monit Assess 190(3):1–3

    Article  Google Scholar 

  • Aghazadeh N, Mogaddam AA (2010) Assessment of Groundwater Quality and its Suitability for Drinking and Agricultural Uses in the Oshnavieh Area, Northwest of Iran[J]. J Environ Prot 01(01):30–40

    Article  Google Scholar 

  • Aghazadeh N, Mogaddam AA (2011) Investigation of hydrochemical characteristics of groundwater in the Harzandat aquifer, Northwest of Iran[J]. Environ Monit Assess 176(1–4):183–195

    Article  Google Scholar 

  • Akoto O, Teku JA, Gasinu D (2019) Chemical characteristics and health hazards of heavy metals in shallow groundwater: case study Anloga community, Volta Region, Ghana[J]. Appl Water Sci 9(2):1–9

    Article  Google Scholar 

  • Alaya MB, Saidi S, Zemni T, Zargouni F (2014) Suitability assessment of deep groundwater for drinking and irrigation use in the Djeffara aquifers (Northern Gabes, south-eastern Tunisia)[J]. Environ Earth Sci 71(8):3387–3421

    Article  Google Scholar 

  • Anim-Gyampo M, Anornu GK, Appiah-Adjei EK, Agodzo SK (2019) Quality and health risk assessment of shallow groundwater aquifers within the Atankwidi basin of Ghana[J]. Groundw Sustain Dev 9:100217

    Article  Google Scholar 

  • Bian J, Nie S, Wang R, Wan H, Liu C (2018) Hydrochemical characteristics and quality assessment of groundwater for irrigation use in central and eastern Songnen Plain, Northeast China[J]. Environ Monit Assess 190(7):1–6

    Article  Google Scholar 

  • Bura B, Goni IB (2012) Tracing the factors influencing occurrence of fluoride in groundwater of the Middle zone aquifer in Borno State, North-Eastern Nigeria[J]. J Min Geol 48(2):177–184

    Google Scholar 

  • Chen J, Wu H, Qian H, Gao Y (2017) Assessing nitrate and fluoride contaminants in drinking water and their health risk of rural residents living in a semiarid region of northwest China[J]. Expo Health 9(3):183–195

    Article  Google Scholar 

  • Chen B, Gong H, Lei K, Li J, Zhou C, Gao M, Guan H, Lv W (2019) Land subsidence lagging quantification in the main exploration aquifer layers in Beijing plain, China[J]. Int J Appl Earth Obs Geoinf 75:54–67

    Google Scholar 

  • Dar MA, Sankar K, Dar IA (2011) Fluorine contamination in groundwater: a major challenge[J]. Environ Monit Assess 173(1–4):955–968

    Article  Google Scholar 

  • Dev R, Bali M (2019) Evaluation of groundwater quality and its suitability for drinking and agricultural use in district Kangra of Himachal Pradesh, India[J]. J Saudi Soc Agric Sci 18(4):462–468

    Google Scholar 

  • Doneen LD (1964) Water Quality for Agriculture. Department of Irrigation, University of California[D]. Department of Irrigation, University of California

  • Duan L, Wang W, Sun Y, Zhang C (2016) Iodine in groundwater of the Guanzhong Basin, China: sources and hydrogeochemical controls on its distribution[J]. Environ Earth Sci 75(11):1–11

    Article  Google Scholar 

  • Duan L, Wang W, Sun Y, Zhang C, Sun Y (2020) Hydrogeochemical characteristics and health effects of iodine in groundwater in Wei River Basin[J]. Expo Health 12:369–383

    Article  Google Scholar 

  • Eaton FM (1950) Significance of carbonates in irrigation waters[J]. Soil Sci 69:123–133

    Article  Google Scholar 

  • Egbi CD, Anornu GK, Ganyaglo SY, Appiah-Adjei EK, Li S, Dampare SB (2020) Nitrate contamination of groundwater in the Lower Volta River Basin of Ghana: sources and related human health risks[J]. Ecotoxicol Environ Saf 191:110227

    Article  Google Scholar 

  • Emenike CP, Tenebe IT, Jarvis P (2018) Fluoride contamination in groundwater sources in Southwestern Nigeria: assessment using multivariate statistical approach and human health risk[J]. Ecotoxicol Environ Saf 156:391–402

    Article  Google Scholar 

  • Gu X, Xiao Y, Yin S, Pan X, Niu Y, Shao J, Cui Y, Zhang Q, Hao Q (2017) Natural and anthropogenic factors affecting the shallow groundwater quality in a typical irrigation area with reclaimed water, North China Plain[J]. Environ Monit Assess 189(10):1–12

    Article  Google Scholar 

  • Gu X, Xiao Y, Yin S, Hao Q, Liu H, Hao Z, Meng G, Pei Q, Yan H (2018) Hydrogeochemical characterization and quality assessment of groundwater in a long-term reclaimed water irrigation area, North China Plain[J]. Water 10(9):1209

    Article  Google Scholar 

  • Handa BK (1964) Modified classification procedure fro rating irrigation waters[J]. Soil Sci 98(4):264–269

    Article  Google Scholar 

  • He S, Wu J (2019) Hydrogeochemical characteristics, groundwater quality, and health risks from hexavalent chromium and nitrate in groundwater of Huanhe Formation in Wuqi county, northwest China[J]. Expo Health 11(2):125–137

    Article  Google Scholar 

  • Hossain M, Patra PK (2020) Contamination zoning and health risk assessment of trace elements in groundwater through geostatistical modelling[J]. Ecotoxicol Environ Saf 189:110038

    Article  Google Scholar 

  • Jasmin I, Mallikarjuna P (2015) Evaluation of groundwater suitability for irrigation in the Araniar River Basin, South India—a case study using Gis approach[J]. Irrig Drain 64(5):600–608

    Article  Google Scholar 

  • Jianmin B, Yu W, Juan Z (2015) Arsenic and fluorine in groundwater in western Jilin Province, China: occurrence and health risk assessment[J]. Nat Hazards 77(3):1903–1914

    Article  Google Scholar 

  • Karunanidhi D, Aravinthasamy P, Kumar D, Subramani T, Roy PD (2020) Sobol sensitivity approach for the appraisal of geomedical health risks associated with oral intake and dermal pathways of groundwater fluoride in a semi-arid region of south India. Ecotoxicol Environ Saf 194:1–12

    Article  Google Scholar 

  • Kim K, Jeong GY (2005) Factors influencing natural occurrence of fluoride-rich groundwaters: a case study in the southeastern part of the Korean Peninsula[J]. Chemosphere 58(10):1399–1408

    Article  Google Scholar 

  • Li P, Wu J, Qian H (2013) Assessment of groundwater quality for irrigation purposes and identification of hydrogeochemical evolution mechanisms in Pengyang County, China[J]. Environ Earth Sci 69(7):2211–2225

    Article  Google Scholar 

  • Li P, Qian H, Wu J, Chen J, Zhang Y, Zhang H (2014) Occurrence and hydrogeochemistry of fluoride in alluvial aquifer of Weihe River, China[J]. Environ Earth Sci 71(7):3133–3145

    Article  Google Scholar 

  • Li C, Gao X, Wang Y (2015) Hydrogeochemistry of high-fluoride groundwater at Yuncheng Basin, northern China[J]. Sci Total Environ 508:155–165

    Article  Google Scholar 

  • Li J, Wang Y, Xie X, Depaolo DJ (2016a) Effects of water-sediment interaction and irrigation practices on iodine enrichment in shallow groundwater[J]. J Hydrol 543:293–304

    Article  Google Scholar 

  • Li P, Li X, Meng X, Li M, Zhang Y (2016b) Appraising groundwater quality and health risks from contamination in a semiarid region of northwest China[J]. Expo Health 8(3):361–379

    Article  Google Scholar 

  • Li J, Zhou H, Qian K, Xie X, Xue X, Yang Y, Wang Y (2017) Fluoride and iodine enrichment in groundwater of North China Plain: evidences from speciation analysis and geochemical modeling[J]. Sci Total Environ 598:239–248

    Article  Google Scholar 

  • Li P, He X, Li Y, Xiang G (2019) Occurrence and health implication of fluoride in groundwater of loess aquifer in the Chinese loess plateau: a case study of Tongchuan, Northwest China[J]. Expo Health 11(2):95–107

    Article  Google Scholar 

  • Liu H, Guo H, Yang L, Wu L, Li F, Li S, Ni P, Liang X (2015) Occurrence and formation of high fluoride groundwater in the Hengshui area of the North China Plain[J]. Environ Earth Sci 74(3):2329–2340

    Article  Google Scholar 

  • Lyu R, Gao Z, Li D, Yang Z, Zhang T (2020) Bioaccessibility of arsenic from gastropod along the Xiangjiang River: assessing human health risks using an in vitro digestion model[J]. Ecotoxicol Environ Saf 193:110334

    Article  Google Scholar 

  • Magesh NS, Chandrasekar N, Elango L (2017) Trace element concentrations in the groundwater of the Tamiraparani river basin, South India: insights from human health risk and multivariate statistical techniques[J]. Chemosphere 185:468–479

    Article  Google Scholar 

  • Manjeet SBP, Sharma JK (2014) Distribution of fluoride in groundwater in Bhiwani district and its suitability assessment for drinking purpose[J]. Int J Eng Res Technol 3(4):2731–2734

    Google Scholar 

  • Narsimha A, Rajitha S (2018) Spatial distribution and seasonal variation in fluoride enrichment in groundwater and its associated human health risk assessment in Telangana State, South India[J]. Hum Ecol Risk Assess Int J 24(8):2119–2132

    Article  Google Scholar 

  • Narsimha A, Sudarshan V (2017a) Assessment of fluoride contamination in groundwater from Basara, Adilabad District, Telangana State, India[J]. Appl Water Sci 7(6):2717–2725

    Article  Google Scholar 

  • Narsimha A, Sudarshan V (2017b) Contamination of fluoride in groundwater and its effect on human health: a case study in hard rock aquifers of Siddipet, Telangana State, India[J]. Appl Water Sci 7(5):2501–2512

    Article  Google Scholar 

  • Piper AM (1944) A graphic procedure in the geochemical interpretation of water-analyses[J]. Trans Am Geophys Union 25(6):914–928

    Article  Google Scholar 

  • Qian K, Li J, Xie X, Wang Y (2017) Organic and inorganic colloids impacting total iodine behavior in groundwater from the Datong Basin, China[J]. Sci Total Environ 601–602:380–390

    Article  Google Scholar 

  • Qin L, Pang X, Zeng H, Liang Y, Mo L, Wang D, Dai J (2020) Ecological and human health risk of sulfonamides in surface water and groundwater of Huixian karst wetland in Guilin, China[J]. Sci Total Environ 708:134552

    Article  Google Scholar 

  • Raju NJ (2007) Hydrogeochemical parameters for assessment of groundwater quality in the upper Gunjanaeru River basin, Cuddapah District, Andhra Pradesh, South India[J]. Environ Geol 52(6):1067–1074

    Article  Google Scholar 

  • Ravindra K, Mor S (2019) Distribution and health risk assessment of arsenic and selected heavy metals in Groundwater of Chandigarh, India[J]. Environ Pollut 250:820–830

    Article  Google Scholar 

  • Ravindra K, Thind PS, Mor S, Singh T, Mor S (2019) Evaluation of groundwater contamination in Chandigarh: Source identification and health risk assessment[J]. Environ Pollut 255:113062

    Article  Google Scholar 

  • Richards LA (1954) Diagnosis and improvement of saline alkali soils: Agriculture, vole 160. Handbook 60[D]. US Department of Agriculture, Washington DC

  • Su X, Wang H, Zhang Y (2013) Health risk assessment of nitrate contamination in groundwater: a case study of an agricultural area in northeast China[J]. Water Resour Manag 27(8):3025–3034

    Article  Google Scholar 

  • Subramani T, Elango L, Damodarasamy SR (2005) Groundwater quality and its suitability for drinking and agricultural use in Chithar River Basin, Tamil Nadu, India[J]. Environ Geol 47(8):1099–1110

    Article  Google Scholar 

  • Szaboles I, Darab C (1964) The influence of irrigation water of high sodium carbonate content of soils. In Proceedings of 8th international congress of ISSS[J]. Trans, vol 2, pp 803–812

  • Teng Y, Zuo R, Xiong Y, Wu J, Zhai Y, Su J (2019) Risk assessment framework for nitrate contamination in groundwater for regional management[J]. Sci Total Environ 697:134102

    Article  Google Scholar 

  • USSL Salinity Laboratory (1954) Diagnosis and Improvement of Saline and Alkaline Soils. US Department of Agriculture Handbook, No. 60

  • USEPA (1989) Risk assessment guidance for superfund, vol I., Human health evaluation manual (Part A). Office of Emergency and Remedial Response, Washington, DC

    Google Scholar 

  • USEPA (1991) Risk Assessment Guidance for Superfund Volume I—Human Health Evaluation Manual (Part B, Development of Risk Based Preliminary Remediation Goals). EPA/540/R92/003, Wash-ington DC

  • UNEP (1999) Global environment outlook 2000. Earthscan, UK

  • USEPA (2004) Risk Assessment Guidance for Superfund Volume I: Human Health Evaluation Manual (Part E, Supplemental Guidance for Dermal Risk Assessment). Office of Superfund Remediation and Technology Innovation U.S. Environmental Protection Agency Washington, DC

  • Wang Y, Song X, Li B, Ma Y, Zhang Y, Yang L, Bu H, Holm PE (2018) Temporal variation in groundwater hydrochemistry driven by natural and anthropogenic processes at a reclaimed water irrigation region[J]. Hydrol Res 49(5):1652–1668

    Article  Google Scholar 

  • World Health Organization (WHO) (2011) Guidelines for drinking water quality, vol 4. World Health Organization, Genva

    Google Scholar 

  • World Health Organization (WHO) (2017) Guidelines for drinking water quality: Fourth Edition Incorporating the First Addendum. Geneva

  • Wilcox LV (1955) Classification and use of irrigation water. USDA, Circular. Washington, 969

  • Wu J, Sun Z (2016) Evaluation of shallow groundwater contamination and associated human health risk in an alluvial plain impacted by agricultural and industrial activities, mid-west China[J]. Expo Health 8(3):311–329

    Article  Google Scholar 

  • Wu J, Li P, Qian H (2015) Hydrochemical characterization of drinking groundwater with special reference to fluoride in an arid area of China and the control of aquifer leakage on its concentrations[J]. Environ Earth Sci 73(12):8575–8588

    Article  Google Scholar 

  • Wu J, Li J, Teng Y, Chen H, Wang Y (2019) A partition computing-based positive matrix factorization (PC-PMF) approach for the source apportionment of agricultural soil heavy metal contents and associated health risks[J]. J Hazard Mater 388:121766

    Article  Google Scholar 

  • Xi B, Li J, Wang Y, Tang J, Hong H (2019) Strengthening the innovation capability of groundwater science and technology to support the coordinated development of Beijing-Tianjin-Hebei region: status quo, problems and goals[J]. Res Environ Sci 32(01):1–9

    Google Scholar 

  • Xing L, Guo H, Zhan Y (2013) Groundwater hydrochemical characteristics and processes along flow paths in the North China Plain[J]. J Asian Earth Sci 70–71:250–264

    Article  Google Scholar 

  • Xiong G, Chen G, Xu X, Liu W, Fu T, Khokiattiwong S, Kornkanitnan N, Ali Seddique A, Shi X, Liu S, Su Q, Xu X (2020) A comparative study on hydrochemical evolution and quality of groundwater in coastal areas of Thailand and Bangladesh[J]. J Asian Earth Sci 195:104336

    Article  Google Scholar 

  • Yadav KK, Kumar V, Gupta N, Kumar S, Rezania S, Singh N (2019) Human health risk assessment: Study of a population exposed to fluoride through groundwater of Agra city, India[J]. Regul Toxicol Pharmacol 106:68–80

    Article  Google Scholar 

  • Yang M, Fei Y, Ju Y, Ma Z, Li H (2012) Health risk assessment of groundwater pollution—a case study of typical city in North China plain[J]. J Earth Sci 23(3):335–348

    Article  Google Scholar 

  • Yang Y, Yu Y, Wei W, Li D, Yang J (2013) Health risk assessment of heavy metals in shallow groundwater in urban and suburban areas of Changzhou (In Chinese)[J]. Envrion Chem 32(02):202–211

    Google Scholar 

  • Yu Y, Yang J (2020) Health risk assessment of fluorine in fertilizers from a fluorine contaminated region based on the oral bioaccessibility determined by Biomimetic Whole Digestion-Plasma in-vitro Method (BWDPM)[J]. J Hazard Mater 383:121124

    Article  Google Scholar 

  • Zhai Y, Wang J, Teng Y, Zuo R (2013) Hydrogeochemical and isotopic evidence of groundwater evolution and recharge in aquifers in Beijing Plain, China[J]. Environ Earth Sci 69(7):2167–2177

    Article  Google Scholar 

  • Zhai Y, Lei Y, Wu J, Teng Y, Wang J, Zhao X, Pan X (2016) Does the groundwater nitrate pollution in China pose a risk to human health? A critical review of published data[J]. Environ Sci Pollut Res 24(4):3640–3653

    Article  Google Scholar 

  • Zhai Y, Zhao X, Teng Y, Li X, Zhang J, Wu J, Zuo R (2017) Groundwater nitrate pollution and human health risk assessment by using HHRA model in an agricultural area, NE China[J]. Ecotoxicol Environ Saf 137:130–142

    Article  Google Scholar 

  • Zhang Z, Shi D, Fuhong R, Yin Z, Sun J, Zhang C (1997) Evolution of quaternary groundwater system in North China Plain[J]. Sci China (Ser D) 40(3):276–283

    Article  Google Scholar 

  • Zhang LE, Huang D, Yang J, Wei X, Qin J, Ou S, Zhang Z, Zou Y (2017) Probabilistic risk assessment of Chinese residents’ exposure to fluoride in improved drinking water in endemic fluorosis areas[J]. Environ Pollut 222:118–125

    Article  Google Scholar 

  • Zhang Y, Wu Y, Sun J, Hu S, Zhang Y, Xiang X (2018b) Controls on the spatial distribution of iodine in groundwater in the Hebei Plain, China[J]. Environ Sci Pollut Res 25(17):16702–16709

    Article  Google Scholar 

  • Zhang Y, Wu J, Xu B (2018a) Human health risk assessment of groundwater nitrogen pollution in Jinghui canal irrigation area of the loess region, northwest China[J]. Environ Earth Sci 77(7):1–12

    Article  Google Scholar 

  • Zhao L, Gong D, Zhao W, Lin L, Yang W, Guo W, Tang X, Li Q (2020) Spatial-temporal distribution characteristics and health risk assessment of heavy metals in surface water of the Three Gorges Reservoir, China[J]. Sci Total Environ 704:134883

    Article  Google Scholar 

Download references

Acknowledgements

This work was supported by the National Natural Science Foundation of China (Grant No. 41877294) and the China Geological Survey (Grant No. DD20190679). This research obtained technical guidance and support from Observation and Research Station of Groundwater and Land Subsidence in Beijing-Tianjin-Hebei Plain. The authors would be also appreciated for valuable comments and advice given by the editors and anonymous reviewers.

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to Haipeng Guo.

Additional information

Publisher's Note

Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.

Supplementary Information

Below is the link to the electronic supplementary material.

Supplementary file1 (DOCX 23 KB)

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Zhao, X., Guo, H., Wang, Y. et al. Groundwater hydrogeochemical characteristics and quality suitability assessment for irrigation and drinking purposes in an agricultural region of the North China plain. Environ Earth Sci 80, 162 (2021). https://doi.org/10.1007/s12665-021-09432-w

Download citation

  • Received:

  • Accepted:

  • Published:

  • DOI: https://doi.org/10.1007/s12665-021-09432-w

Keywords

Navigation