Skip to main content
Log in

Improving the efficiency in the detection of gamma activities in environmental soil samples: influence of the granulometry and soil density

  • Published:
Journal of Radioanalytical and Nuclear Chemistry Aims and scope Submit manuscript

Abstract

In this work the efficiency calibration curves for a HPGe gamma detector were obtained from soil standards prepared in our laboratory using typical Argentine regional soils. They were made in pot and Petri dish geometries, for different soil granulometries, by using two mixed nuclide reference solutions manufactured by Eckert & Ziegler and provided by the IAEA. The efficiency curves obtained were tested with the reference materials IAEA-375, IAEA-447, CNEA-81-11 as well as the soil sample used in the IAEA-2013 proficiency test. The results allow to improve the quality in the analytical measurements on the content of radionuclides in local soils.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Institutional subscriptions

Fig. 1
Fig. 2
Fig. 3
Fig. 4
Fig. 5
Fig. 6

Figure taken from Genie 2000 software [16]

Fig. 7

Similar content being viewed by others

References

  1. Murray AS, Marten R, Johnston A, Martin P (1987) Analysis for naturally occuring radionuclides at environmental concentrations by gamma spectrometry. J Radioanal Nucl Chem 115:263–288

    Article  CAS  Google Scholar 

  2. Gilmore G, Hemingway JD (1995) Practical gamma-ray spectrometry. Wiley, New York

    Google Scholar 

  3. Boson J, Ågren G, Johansson L (2008) A detailed investigation of HPGe detector response for improved Monte Carlo efficiency calculations. Nucl Instrum Methods Phys Res Sect A 587:304–314

    Article  CAS  Google Scholar 

  4. Vargas MJ, Timón AF, Dı́az NC, Sánchez DP (2002) Monte Carlo simulation of the self-absorption corrections for natural samples in gamma-ray spectrometry. Appl Radiat Isot 57:893–898

    Article  PubMed  Google Scholar 

  5. Mabit L, Benmansour M, Walling DE (2008) Comparative advantages and limitations of the fallout radionuclides 137Cs, 210Pbex and 7Be for assessing soil erosion and sedimentation. J Environ Radioact 99:1799–1807

    Article  CAS  PubMed  Google Scholar 

  6. Boshkova T, Minev L (2001) Corrections for self-attenuation in gamma-ray spectrometry of bulk samples. Appl Radiat Isot 54:777–783

    Article  CAS  PubMed  Google Scholar 

  7. He Q, Walling DE (1996) Interpreting particle size effects in the adsorption of 137Cs and unsupported 210Pb by mineral soils and sediments. J Environ Radioact 30:117–137

    Article  CAS  Google Scholar 

  8. Haddadchi A, Ryder DS, Evrard O, Olley J (2013) Sediment fingerprinting in fluvial systems: review of tracers, sediment sources and mixing models. Int J Sedim Res 28:560–578

    Article  Google Scholar 

  9. Li G, Liang Y, Xu J, Bai L (2015) Efficiency corrections in determining the 137Cs inventory of environmental soil samples by using relative measurement method and GEANT4 simulations. J Environ Radioact 146:94–101

    Article  CAS  PubMed  Google Scholar 

  10. Moens L, De Donder J, Xi-lei L, De Corte F, De Wispelaere A, Simonits A, Hoste J (1981) Calculation of the absolute peak efficiency of gamma-ray detectors for different counting geometries. Nucl Instrum Methods Phys Res 187:451–472

    Article  CAS  Google Scholar 

  11. Nikolic JK, Rajačić MM, Todorovic D, Vidmar T (2016) The first experimental test of the MEFFTRAN software on HPGe detector calibration for environmental samples. J Environ Radioact 165:191–196

    Article  CAS  PubMed  Google Scholar 

  12. Vidmar T, Kanisch G, Vidmar G (2011) Calculation of true coincidence summing corrections for extended sources with EFFTRAN. Appl Radiat Isot 69:908–911

    Article  CAS  PubMed  Google Scholar 

  13. Vukanac I, Djurašević M, Kandić A, Novković D, Nadjerdj L, Milošević Z (2008) Experimental determination of the HPGe spectrometer efficiency curve. Appl Radiat Isot 66:792–795

    Article  CAS  PubMed  Google Scholar 

  14. Ebaid YY (2009) On the use of reference materials in gamma-ray spectrometric efficiency calibration for environmental samples. J Radioanal Nucl Chem 280:21–25

    Article  CAS  Google Scholar 

  15. Harb S, Salahel Din K, Abbady A (2009) Study of efficiency calibrations of HPGe detectors for radioactivity measurements of environmental samples. In: Proceedings of the 3rd Environmental Physics Conference, 19–23 Feb. 2008, Aswan, Egypt

  16. Canberra (2009) Genie 2000 version 3.2.1 basic spectroscopy software & documentation. Canberra (2010) Genie 2000 version 3.2.2 gamma analysis software

  17. Xhixha G, Alberi M, Baldoncini M, Bode K, Bylyku E, Cfarku F, Callegari I, Hasani F, Landsberger S, Mantovani F, Rodriguez E, Shala F, Strati V, Xhixha Kaceli M (2016) Calibration of HPGe detectors using certified reference materials of natural origin. J Radioanal Nucl Chem 307:1507–1517

    Article  CAS  Google Scholar 

Download references

Acknowledgements

This research was supported by Universidad Nacional de San Luis (UNSL), Consejo Nacional de Investigaciones Científicas y Técnicas (CONICET) and International Atomic Energy Agency (IAEA).

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to M. G. Rizzotto.

Ethics declarations

Conflict of interest

The authors declare that they have no conflict of interest.

Additional information

Publisher's Note

Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Torres Astorga, R., Rizzotto, M.G. & Velasco, H. Improving the efficiency in the detection of gamma activities in environmental soil samples: influence of the granulometry and soil density. J Radioanal Nucl Chem 321, 805–814 (2019). https://doi.org/10.1007/s10967-019-06643-1

Download citation

  • Received:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s10967-019-06643-1

Keywords

Navigation