Abstract
210Pb is an effective tracer of constraining particle transport and sedimentation in shelf regions. To reveal the spatial pattern of 210Pb over the East China Sea (i.e. ECS) Shelf, 210Pb in the surface sediments were examined at 11 stations, as well as 234Th and 210Pb in the water column at four stations. Overall, the plume zone of the Yangtze River along the coastline is a source area of 210Pb for the outer shelf, exporting 0.46 dpm cm−2 year−1 at least, which accounts for about 25 % of 210Pb input into this region. In the southern ECS Shelf to the north of the Taiwan Strait, the focusing factor (f) values are higher than unity, indicating a sink area of 210Pb. Boundary scavenging of 210Pb contributes 0.36 dpm cm−2 year−1 to this sink area on the basis of a mass balance model evaluation. Lateral transport of 210Pb to this region, quantified by 234Th and 210Pb in the water column, varied from 3.34 to 6.39 dpm cm−2 year−1 with an average of 4.83 dpm cm−2 year−1, also supporting its sink characteristic. To the southwest of the Cheju Island, the f values were less than unity, revealing a source region of 210Pb. The average export flux of 210Pb from this region was 1.64 dpm cm−2 year−1. Therefore, 210Pb sedimentation/settling showed significantly heterogeneous sedimentation of particulate matter over the ECS Shelf.
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References
Gao S, Jia JJ (2003) Modeling suspended sediment distribution in continental shelf upwelling/down welling settings. Geo Mar Lett 22:218–226
Milliman JD, Meade RH (1983) World-wide delivery of sediment to the oceans. J Geology 91(3):1–21
Xu KH, Milliman JD (2009) Seasonal variations of sediment discharge from the Yangtze River before and after impoundment of the Three Gorges Dam. Geomorph 104:276–283
Xu KH, Milliman JD, Li AC, Liu JP, Kao SJ, Wan SM (2009) Yangtze- and Taiwan-derived sediments on the inner shelf of East China Sea. Cont Shelf Res 29:2240–2256
Huh CA, Su CC (1999) Sedimentation dynamics in the East China Sea elucidated from 210Pb, 137Cs and 239,240Pu. Mar Geol 160:183–196
Guo ZG, Yang ZS, Lei K, Qu YH, Fan DJ (1999) Seasonal variation of the sedimentary dynamic processes for the mud area in the northern East China Sea. J Ocean Univ Qingdao 29(3):507–513 (in Chinese)
Lei K, Yang ZS, Guo ZG (2001) Sedimentation with aggregation of suspended sediment in a mud area of the northern East China Sea. Oceanol Limnol Sin 32(3):288–295 (in Chinese)
Liu JP, Li AC, Xu KH, Velozzi DM, Yang ZS, Milliman JD, DeMaster DJ (2006) Sedimentary features of the Yangtze River-derived along-shelf clinoform deposit in the East China Sea. Cont Shelf Res 26:2141–2156
Liu JP, Xu KH, Li AC, Milliman JD, Velozzi DM, Xiao SB, Yang ZS (2007) Flux and fate of Yangtze River sediment delivered to the East China Sea. Geomorph 85:208–224
Su CC, Huh CA (2002) 210Pb, 137Cs and 239,240Pu in East China Sea sediments: sources, pathways and budgets of sediments and radionuclides. Mar Geol 183:163–178
Jiao N, Zhang Y, Zeng Y, Gardner WD, Mishonov AV, Richardson MJ, Hong N, Pan D, Yan X-H, Jo Y-H, Chen C-TA, Wang P, Chen Y, Hong H, Bai Y, Chen X, Huang B, Deng H, Shi Y, Yang D (2007) Ecological anomalies in the East China Sea: impacts of the Three Gorges Dam? Water Res 41:1287–1293
Du JZ, Wu YF, Huang YF, Zhang J (2010) Use of 7Be, 210Pb and 137Cs tracers to the transport of surface sediments of the Changjing Estuary, China. J Mar Sys 82:286–294
Yang W, Chen M, Li G, Cao J, Guo Z, Ma Q, Liu J, Yang J (2009) Relocation of the Yellow River as revealed by sedimentary isotopic and elemental signals in the East China Sea. Mar Pollut Bull 58:923–927
Yang W (2005) Marine biogeochemistry of 210Po and 210Pb and their implications regarding the cycling and export of particles. Ph.D. dissertation, Xiamen University, 176–211 (in Chinese)
Yang W, Huang Y, Chen M, Zhang L, Li H, Liu G, Qiu Y (2006) Disequilibria between 210Po and 210Pb in surface waters of the southern South China Sea and their implications. Sci China Ser D 49:103–114
Wei CL, Chou LH, Tsai JR, Wen LS, Pai SC (2009) Comparative Geochemistry of 234Th, 210Pb and 210Po: a case study in the Hung-Tsai Trough off Southwestern Taiwan. Terr Atmos Ocean Sci 20(2):411–423
Yao SC, Li SJ, Zhang HC (2008) 210Pb and 137Cs dating of sediments from Zigetang lake, Tibetan Plateau. J Radioanal Nucl Chem 278:55–58
Gelen A, Soto J, Gómez J, Díaz O (2004) Sediment dating of Santander Bay, Spain. J Radioanal Nucl Chem 261:437–441
Liu GS, Huang YP (1998) Simultaneous measurement of 238U, 235U, 210Pb, 228Th, 228Ra, 226Ra, 60Co and 137Cs in sediment samples using HP Ge γ spectrometer. J Oceanogr Taiwan Strait 17(4):359–363 (in Chinese)
Ma Q, Chen M, Qiu YS, Huang YP (2005) MnO2 precipitation and direct beta counting technique for determining 234Th in small volume seawater. Acta Oceanol Sin 27(4):68–75 (in Chinese)
Benitez-Nelson CR, Buesseler KO, Rutgers van der Loeff M, Andrews J, Ball L, Crossin G, Charette MA (2001) Testing a new small-volume technique for determining 234Th in seawater. J Radioanal Nucl Chem 248:795–799
Yang W, Guo L, Chuang C-Y, Schumann D, Ayranov M, Santschi PH (2013) Adsorption characteristics of 210Pb, 210Po and 7Be onto micro-particle surfaces and the effects of macromolecular organic compounds. Geochim Cosmchim Acta 107:47–64
Pan SM, Xu YH, Wang A, Povinec PP (2012) The 137Cs distribution in sediment profiles from the Yangtze River estuary: a comparison of modeling and experimental results. J Radioanal Nucl Chem 292:1207–1214
Mahmood ZUW, Mohamed CAR, Ishak AK, Bakar NSA, Ishak K (2011) Vertical distribution of 210Pb and 226Ra and their activity ratio in marine sediment core of the East Malaysia coastal waters. J Radioanal Nucl Chem 289:953–959
Li DM, Xu MQ, Liu GS, Li C (2007) Distribution of radioisotopes in sediment cores from nearshore off Xinghua Bay mouth, Fujian, China. J Radioanal Nucl Chem 273:151–155
Yi Y, Zhou P, Liu GS (2007) Atmospheric deposition fluxes of 7Be, 210Pb and 210Po at Xiamen, China. J Radioanal Nucl Chem 273:157–162
Singh AK, Marcantonio F, Lyle M (2011) Sediment focusing in the Panama Basin, Eastern Equatorial Pacific Ocean. Earth Planet Sci Lett 309:33–44
Suman DO, Bacon MP (1989) Variations in Holocene sedimentation in the North-American basin determined from Th-230 measurements. Deep-Sea Res I 36(6):869–878
Chen M, Ma Q, Guo LD, Qiu YS, Huang YP, Yang WF (2012) Importance of lateral transport processes to 210Pb budget in the eastern Chukchi Sea during summer 2003. Deep-Sea Res II 81–84:53–62
Cochran JK, McKibbin-Vaughan T, Dornblaser MM, Hirschberg D, Livingston H, Buesseler KO (1990) 210Pb scavenging in the North Atlantic and North Pacific Oceans. Earth Planet Sci Lett 97:332–352
Yi Y, Bai J, Liu G, Yang W, Yi Q, Huang Y, Chen H (2005) Measurements of atmospheric deposition fluxes of 7Be, 210Pb and 210Po. Mar Sci 29:20–24 (in Chinese)
Su C-A, Huh C-A, Lin F-J (2003) Factors controlling atmospheric fluxes of 7Be and 210Pb in northern Taiwan. Geophys Res Lett 30(19):2018. doi:10.1029/2003GL018221
Men W (2008) The study on the oceanography of the Yellow Sea and the East China Sea traced by radium isotopes. Ph.D. dissertation, Xiamen University, 71–123 (in Chinese)
Jacobs GA, Hur HB, Riedlinger SK (2000) Yellow and East China Seas response to winds and currents. J Geophys Res 105:21947–21968
Zhao BR (1993) Upwelling off the Changjiang river mouth. Acta Oceanol Sin 15(2):108–114 (in Chinese)
Guo ZG, Yang ZS, Zhang DQ, Fan DJ, Lei K (2002) Seasonal distribution of suspended matter in the northern East China Sea and barrier effect of current circulation on its transport. Acta Oceanol Sin 24(5):71–80 (in Chinese)
Chung Y, Chang HC, Hung GW (2004) Particulate flux and 210Pb determined on the sediment trap and core samples from the northern South China Sea. Cont Shelf Res 24:672–691
Ye YG, He J, Diao SB, Cai SQ, Song SQ (1992) Standardization of 210Pb profile in the modern Huanghe river delta-the correlation method of grain size. Sci Geograph Sin 12(4):279–286 (in Chinese)
Men W, Wang FF, Liu GS (2011) 224Ra and its implications in the East China Sea. J Radioanal Nucl Chem 288:189–197
Qu TD, Hu DX (1993) Upwelling and sedimentary dynamics II. A simple model. Chinese J Oceanol Limol 11(2): 289–295
Men W, Liu GS, Huang YP (2010) Measurement of 228Ra in the Yellow Sea and East China Sea using the radon emanation method. J Radioanal Nucl Chem 284:65–72
Mckee BA, Nittrouer CA, DeMaster DJ (1983) Concepts of sediment deposition and accumulation applied to the continental shelf near the mouth of the Yangtze River. Geology 11:631–633
Fan DJ, Yang ZS, Sun XG, Zhang DQ, Guo ZG (2002) Quantitative evaluation of sediment provenance on the north area of the East China Sea shelf. J Ocean Univ Qingdao 32(5):748–756 (in Chinese)
Qin YS (1979) A study on sediment and mineral compositions of the floor of the East China Sea. Ocean Sel 2(2):130–142
Lei K, Yang ZS, Guo ZG, Bai H (2001) Suspended sediment flux in spring on the East China Sea shelf with different surface sediment types. Oceanol Limnol Sin 32(1):50–57 (in Chinese)
Lim DI, Choi JY, Jung HS, Rho KC, Ahn KS (2007) Recent sediment accumulation and origin of shelf mud deposits in the Yellow and East China Seas. Prog Oceanogr 73:145–159
Chen JH, Edwards RL, Wasserburg GJ (1986) 238U, 234U and 232Th in sea water. Earth Planet Sci Lett 80:241–251
Wang YH, Jan S, Wang DP (2003) Transports and tidal current estimates in the Taiwan Strait from shipboard ADCP observations (1999–2001). Est Coast Shelf Sci 57:193–199
Wu CR, Chao SY, Hsu C (2007) Transient, seasonal and interannual variability of the Taiwan Strait Current. J Oceanogr 63:821–833
Zhao BR, Fang GH (1991) Estimation of water fluxes of major waterways in East China Sea. Acta Oceanol Sin 13(2):169–178 (in Chinese)
Kawakami H, Yang YL, Kusakabe M (2009) Distribution of 210Po and 210Pb radioactivity in the intermediate layer of the northwestern North Pacific. J Radioanal Nucl Chem 279:561–566
Huh CA, Chen WF, Hsu FH, Su CC, Chiu JK, Lin S, Liu CS, Huang BJ (2010) Modern (<100 years) sedimentation in the Taiwan Strait: rates and source-to-sink pathways elucidated from radionuclides and particle size distribution. Cont Shelf Res 31:47–63
Acknowledgments
We appreciate Professor Tibor Braun and tow anonymous reviewers for their constructive suggestions, which greatly improved the presentation of this manuscript. This work is supported jointly by a Chinese COMRA program (No. DY125-13-E-01) and the Chinese National Science Foundation (41076043 and 41125020).
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Fang, Z., Yang, W., Zhang, X. et al. Sedimentation and lateral transport of 210Pb over the East China Sea Shelf. J Radioanal Nucl Chem 298, 739–748 (2013). https://doi.org/10.1007/s10967-013-2561-4
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DOI: https://doi.org/10.1007/s10967-013-2561-4