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Design Strategies of Metal Complexes Based on Chelating Polymer Ligands and Their Application in Nanomaterials Science

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Abstract

The advances and problems associated with the synthesis, properties and structure of metal complexes based on chelating polymer ligands are presented and assessed. The polymeric metal chelates (PMCs) are divided into molecular, intracomplex, macrocyclic and polynuclear types, which in turn are grouped according to the nature of the donor atoms (N,N-, N,О-, N,S-, О,О-, O,S-, S,S-, Р,Р-chelates, etc.). The main attention is focused on the similarities and differences between low and high molecular weight metal chelates, as well as the spatial organization of PMCs. The most important areas of research in the field of such compounds are highlighted. Thermal transformations of metal complexes based on chelating polymer ligands leading to the formation of nanostructured materials are considered. The bibliography includes the articles published after 2010.

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Abbreviations

AAm:

Acrylamide

Acac:

Acetylacetonate anion

ATRP:

Atom transfer radical polymerization

BINAM:

2,2′-Binaphthyldiamine

BINOL:

1,1′-Bi-2-naphtol

BPP:

2,6-Bis(pyrazolyl)pyridine

bpy:

2,2′-Bipyridine

CIE:

International Commission on Illumination

CMC:

Critical concentration of micelle formation

CN:

Coordinative number

COD:

1,5-Cyclooctadiene

CPL:

Chelating polymer ligand

dien:

Diethylene triamine

DIPY:

Dipyromethene

DP:

Polymerization degree

DOTA:

1,4,7,10-Tetraazacyclododecane-1,4,7,10-tetraacetic acid

DTPA:

Diethylenetriamine pentacetic acid

DVB:

Divinylbenzene

EDAX:

Energy dispersive X-ray analysis

EDTA:

Ethylenediaminetetraacetic acid

EL:

Electroluminescence

en:

Ethylenediamine

GMA:

Glycidyl methacrylate

HQ:

8-Hydroxyquinoline

8HQ5S:

8-Hydroxyquinoline-5-sulfonic acid

IDA:

Iminodiacetic acid

Ksv :

Stern–Volmer constant

LCST:

Lower critical solution temperature

LMC:

Low molecular weight metal chelate

MC:

Merocyanine

MLCT:

Metal-to-ligand charge transfer

MMA:

Methyl methacrylate

Mn :

Number-average molecular weight

MRI:

Magnetic resonance imaging

MXn :

Metal compound

Mw :

Weight-average molecular weight

NCF:

Nitrogen-doped carbon microfiber

NIPAM:

N-Isopropylacrylamide

NIR:

Near-infrared

NVK:

N-Vinylcarbazole

PAA:

Polyacrylic acid

PAAm:

Polyacrylamide

PAMAM:

Polyamidoamines

PAN:

Polyacrylonitrile

Pc:

Phthalocyanine

PCD:

Poly(chloromethylstyrene-co-divinylbenzene)

PCN:

Porphyrinic conjugated network

PCS:

Polychloromethylstyrene

PDI:

Polydispersity index

PEG:

Polyethylene glycol

PEI:

Polyethylene imine

PEO:

Poly(ethylene oxide)

PET:

Photoinduced electron transfer

phen:

1,10-Phenanthroline

PIB:

Polyisobutylene

PL:

Photoluminescence

PLL:

Poly-l-lysine

PLQY:

Photoluminescence quantum yield

PMA:

Poly(methacrylate)

PMC:

Polymeric metal chelate

Pp:

Porphyrin

ppy:

2-Phenylpyridine

PS:

Polystyrene

PVC:

Poly(vinyl chloride)

pybox:

Pyridine-bis(oxazoline)

ROMP:

Ring-open metathesis polymerization

ROP:

Ring-opening polymerization

salen:

N,N′-Bis(salicylidene)ethylenediamine

salphen:

N,N′-Phenylenebis(salicylideneimine)

SEM:

Scanning electron microscopy

SP:

Spiropyran

St:

Styrene

TEM:

Transmission electron microscopy

tpy:

2,2′,6′,2′′-Terpyridine

trien:

Triethylenetetramine

TTA:

1-(2-Thenoyl)-3,3,3-trifluoroacetonate

XPS:

X-ray photoelectron spectrometry

XRD:

X-ray diffraction

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Authors and Affiliations

  1. Laboratory of Metallopolymers, The Institute of Problems of Chemical Physics RAS, Academician Semenov avenue 1, Chernogolovka, Moscow Region, 142432, Russian Federation

    Gulzhian I. Dzhardimalieva

  2. Department of Chemistry, Southern Federal University, Zorge Str. 7, Rostov-on-Don, 344090, Russian Federation

    Igor E. Uflyand

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Dzhardimalieva, G.I., Uflyand, I.E. Design Strategies of Metal Complexes Based on Chelating Polymer Ligands and Their Application in Nanomaterials Science. J Inorg Organomet Polym 28, 1305–1393 (2018). https://doi.org/10.1007/s10904-018-0841-8

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