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Journal of Cluster Science

, Volume 21, Issue 3, pp 235–278 | Cite as

Electronic Interactions Between and Through Covalently-Bonded Polymetallic Complexes

  • Paul J. Low
  • Neil J. Brown
Review Paper

Abstract

The diverse structures and rich electrochemical response of polynuclear complexes have made them attractive objects with which to study bridge-mediated electronic interactions. In this review, the role of polymetallic systems as both electro-active sites (electrophores) in {cluster}–bridge–{cluster} systems, and bridging elements in {M}–{cluster}–{M} structures (M = organometallic fragment) has been reviewed. Methods for the characterisation of bridge-mediated charge transfer processes are highlighted, and where possible mechanisms of interaction are identified in specific systems.

Keywords

Cluster Mixed-valence Electronic interaction Electrochemistry Spectroscopy 

Notes

Acknowledgements

Dr Mark A. Fox is sincerely thanked for providing Figs. 11 and 26. PJL holds an EPSRC Fellowship.

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© Springer Science+Business Media, LLC 2010

Authors and Affiliations

  1. 1.Department of ChemistryDurham UniversityDurhamUK

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