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Performance of a flexible electrode based on natural leather

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Abstract

A novel electrode is developed to detect electrocardiogram (ECG) signals using the top grain leather and split leather of pig as the substrate due to their mechanical strength, flexibility, permeability, long-term durability and visual acceptance. The natural leather is pre-treated with Ar plasma and a thin silver paste coating is brush-painted on the surface to gain electrical conductivity. The sheet resistance of the electrodes is approximately 120 mΩ sq−1. The electrodes based on leather can reliably transmit low-frequency and low-voltage signals, which benefit the acquisition of cardiac signals. Although the electrode-skin contact impedance of the dry leather-based electrodes is higher than the silver/silver chloride (Ag/AgCl) electrodes, the contact impedance decreases at least 57.74% after wetting the skin. All cardiac waves obtained by the leather-based electrodes are clear and visible, and the signal-to-noise ratio (SNR) of electrodes are higher than the Ag/AgCl electrodes. The electrodes based on leather have great potential for smart wearable devices.

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References

  1. J. Wannenburg, R. Malekian, G.P. Hancke, Wireless capacitive-based ECG sensing for feature extraction and mobile health monitoring. IEEE Sens. J. 18, 6023–6032 (2018)

    Article  Google Scholar 

  2. E. Lee, I. Kim, H. Liu, G. Cho, Exploration of AgNW/PU nanoweb as ECG textile electrodes and comparison with Ag/AgCl electrodes. Fiber. Polym. 18, 1749–1753 (2017)

    Article  CAS  Google Scholar 

  3. F. Sun, C. Yi, W. Li, Y. Li, A wearable H-shirt for exercise ECG monitoring and individual lactate threshold computing. Comput. Ind. 92–93, 1–11 (2017)

    Article  Google Scholar 

  4. Y. Khan, F.J. Pavinatto, M.C. Lin, A. Liao, S.L. Swisher, K. Mann, V. Subramanian, M.M. Maharbiz, A.C. Arias, Inkjet-printed flexible gold electrode arrays for bioelectronic interfaces. Adv. Funct. Mater. 26, 1004–1013 (2016)

    Article  CAS  Google Scholar 

  5. P. Fiedler, S. Griebel, P. Pedrosa, C. Fonseca, F. Vaz, L. Zentner, F. Zanow, J. Haueisen, Multichannel EEG with novel Ti/TiN dry electrodes. Sensor. Actuat. A-Phys. 221, 139–147 (2015)

    Article  CAS  Google Scholar 

  6. L. Majumder, O. Chen, C.H. Marinov, T. Chen, M.J. Mondal, Deen, noncontact wearable wireless ECG systems for long-term monitoring. IEEE Rev. Biomed. Eng. 11, 306–321 (2018)

    Article  Google Scholar 

  7. A. Ankhili, X. Tao, C. Cochrane, V. Koncar, D. Coulon, J.M. Tarlet, Ambulatory evaluation of ECG signals obtained using washable textile-based electrodes made with chemically modified PEDOT:PSS. Sensors 19, 416 (2019)

    Article  Google Scholar 

  8. M. Weder, D. Hegemann, M. Amberg, M. Hess, L.F. Boesel, R. Abacherli, V.R. Meyer, R.M. Rossi, Embroidered electrode with silver/titanium coating for long-term ECG monitoring. Sensors 15, 1750–1759 (2015)

    Article  CAS  Google Scholar 

  9. H. Cho, H. Lim, S. Cho, J.-W. Lee, Development of textile electrode for electrocardiogram measurement based on conductive electrode configuration. Fiber. Polym. 16, 2148–2157 (2015)

    Article  CAS  Google Scholar 

  10. A.C. Myers, H. Huang, Y. Zhu, Wearable silver nanowire dry electrodes for electrophysiological sensing. Rsc Adv. 5, 11627–11632 (2015)

    Article  CAS  Google Scholar 

  11. Y.-J. Choi, J.-Y. Lee, S.-H. Kong, Driver ECG measuring system with a conductive fabric-based dry electrode. IEEE Access 6, 415–427 (2018)

    Article  Google Scholar 

  12. A. Achilli, D. Bonfiglio, Pani, design and characterization of screen-printed textile electrodes for ECG monitoring. IEEE Sens. J. 18, 4097–4107 (2018)

    Article  CAS  Google Scholar 

  13. Haghdoost, V. Mottaghitalab, A.K. Haghi, Comfortable textile-based electrode for wearable electrocardiogram. Sensor Rev. 35, 20–29 (2015)

    Article  Google Scholar 

  14. C. L. Lam, N. N. Z. M. Rajdi, D. H. B. Wicaksono, MWCNT/cotton-based flexible electrode for electrocardiography. IEEE Sensors 222–225 (2013)

  15. C. Lou, R. Li, Z. Li, T. Liang, Z. Wei, M. Run, X. Yan, X. Liu, Flexible graphene electrodes for prolonged dynamic ECG monitoring. Sensors 16, 1833 (2016)

    Article  Google Scholar 

  16. M.K. Yapici, A.A. Tamador, Y.A. Samad, K. Liao, Graphene-clad textile electrodes for electrocardiogram monitoring. Sensor Actuat. B-Chem. 221, 1469–1474 (2015)

    Article  CAS  Google Scholar 

  17. S.M. Saleh, S.M. Jusob, F.K.C. Harun, L. Yuliati, D.H.B. Wicaksono, Optimization of reduced GO-based cotton electrodes for wearable electrocardiography. IEEE Sens. J. 20, 7774–7782 (2020)

    Article  CAS  Google Scholar 

  18. D. Pani, A. Dessi, J.F. Saenz-Cogollo, G. Barabino, B. Fraboni, A. Bonfiglio, Fully textile, PEDOT:PSS based electrodes for wearable ECG monitoring systems. IEEE Trans. Biomed. Eng. 63, 540–549 (2016)

    Article  Google Scholar 

  19. A. Ankhili, X. Tao, C. Cochrane, D. Coulon, V. Koncar, Washable and reliable textile electrodes embedded into underwear fabric for electrocardiography (ECG) monitoring. Materials 11, 256 (2018)

    Article  Google Scholar 

  20. L. Ke, Y. Wang, X. Ye, W. Luo, X. Huang, B. Shi, Collagen-based breathable, humidity-ultrastable and degradable on-skin device. J. Mater. Chem. C 7, 2548–2556 (2019)

    Article  CAS  Google Scholar 

  21. R. Castrillon, J.J. Perez, H. Andrade-Caicedo, Electrical performance of PEDOT:PSS-based textile electrodes for wearable ECG monitoring: a comparative study. Biomed. Eng. Online 17, 38 (2018)

    Article  Google Scholar 

  22. X. You, L. Gou, X. Tong, Improvement in surface hydrophilicity and resistance to deformation of natural leather through O 2 /H 2 O low-temperature plasma treatment. Appl. Surf. Sci. 360, 398–402 (2016)

    Article  CAS  Google Scholar 

  23. P.S. Das, H.S. Yoon, J. Kim, D.H. Kim, J.Y. Park, Simple fabrication method of an ultrasensitive gold micro-structured dry skin sensor for biopotential recording. Microelectron. Eng. 197, 96–103 (2018)

    Article  CAS  Google Scholar 

  24. T. Takeshita, M. Yoshida, Y. Takei, A. Ouchi, A. Hinoki, H. Uchida, T. Kobayashi, Relationship between contact pressure and motion artifacts in ECG measurement with electrostatic flocked electrodes fabricated on textile. Sci. Rep. 9, 5897 (2019)

    Article  Google Scholar 

  25. Y. Meng, Z. Li, J. Chen, A flexible dry electrode based on APTES-anchored PDMS substrate for portable ECG acquisition system. Microsyst. Technol. 22, 2027–2034 (2015)

    Article  Google Scholar 

  26. P.J. Xu, H. Zhang, X.M. Tao, Textile-structured electrodes for electrocardiogram. Text. Prog. 40, 183–213 (2008)

    Article  Google Scholar 

  27. A. Comert, J. Hyttinen, Investigating the possible effect of electrode support structure on motion artifact in wearable bioelectric signal monitoring. Biomed Eng Online 14, 44 (2015)

    Article  Google Scholar 

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Acknowledgements

This work was supported by ‘Fundamental Research Funds for the Central University’, PR China. The authors would like to acknowledge the testing support from the Analysis & Testing Center of Sichuan University and the test equipment support provided by West China Hospital of Sichuan University.

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Correspondence to Li Gou.

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Song, Y., Huang, Y., Zou, Y. et al. Performance of a flexible electrode based on natural leather. J Mater Sci: Mater Electron 32, 4891–4902 (2021). https://doi.org/10.1007/s10854-020-05229-y

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  • DOI: https://doi.org/10.1007/s10854-020-05229-y

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