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Electrical properties and impedance spectroscopy of crystallographically textured 0.675 [Pb(Mg1/3Nb2/3)O3]-0.325 [PbTiO3] ceramics

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Abstract

Crystallographically \(\left\langle {00{\text{1}}} \right\rangle\)-textured lead magnesium niobate (PMN)—lead titanate (PT) solid solution in the ratio of 0.675PMN-0.325PT was fabricated by tape-casting method using barium titanate (BaTiO3-BT) templates. Random PMN-PT with the same composition was also produced by tape-casting method for comparison. According to electromechanical and dielectric investigations, textured PMN-PT ceramics produced at 1150 °C for 2 h in oxygen atmosphere with 1 vol% BT were found to display the optimum properties. Dielectric constant, dielectric loss and piezoelectric coefficient of these samples were found to be as 1950, 0.002 and 700 pC/N, respectively. The impedance spectroscopy of the samples was conducted and the results of measurements taken at 300 and 500 °C were compared. A significant decrease in the electrical conductivity was observed with the development of texture in PMN-PT. The slightly depressed semicircles that were obtained from Nyquist diagrams indicated non-Debye-type relaxation with a distribution of relaxation time.

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Acknowledgements

The authors wish to acknowledge the financial support of Turkish Academy of Sciences (Gebip Programme) and TUBITAK Project #217M086. The authors also would like to thank Prof. Sedat Alkoy and Prof. Huseyin Yilmaz for fruitful discussions.

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Authors and Affiliations

  1. Department of Materials Science and Engineering, Gebze Technical University, 41400, Gebze, Kocaeli, Turkey

    Ayşe Berksoy-Yavuz & Ebru Mensur-Alkoy

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  1. Ayşe Berksoy-Yavuz
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  2. Ebru Mensur-Alkoy
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Correspondence to Ebru Mensur-Alkoy.

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Berksoy-Yavuz, A., Mensur-Alkoy, E. Electrical properties and impedance spectroscopy of crystallographically textured 0.675 [Pb(Mg1/3Nb2/3)O3]-0.325 [PbTiO3] ceramics. J Mater Sci: Mater Electron 29, 13310–13320 (2018). https://doi.org/10.1007/s10854-018-9455-8

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  • DOI: https://doi.org/10.1007/s10854-018-9455-8

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