Skip to main content
SpringerLink
Log in

Influence of composition ratio on ferroelectric, magnetic and magnetoelectric properties of PMN–PT/CFO composite thin films

  • Published:
Journal of Materials Science: Materials in Electronics Aims and scope Submit manuscript

Abstract

Multiferroic 0.68Pb(Mg1/3Nb2/3)O3–0.32PbTiO3/CoFe2O4 (PMN–PT/CFO) composite films have been grown on Pt/Ti/SiO2/Si substrate via sol–gel spin-coating technique. PMN–PT and CFO precursor solutions were mixed before the spin-coating process to optimize the interface interaction. We investigated the influence of the composition ratio and annealing process on the property of the multiferroic PMN–PT/CFO composite films. The films which entirely consist of PMN–PT and CFO phases have a good performance in the ferroelectric, ferromagnetic property and direct magnetoelectric coupling effect when they were annealed at 730 °C and air atmosphere. It was obviously noticed that the composition ratio between PMN–PT and CFO has an effect on the properties of PMN–PT/CFO multiferroic composites.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Log in via an institution

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Institutional subscriptions

Fig. 1
Fig. 2
Fig. 3
Fig. 4
Fig. 5

Similar content being viewed by others

References

  1. R. Ramesh, N.A. Spaldin, Nat. Mater. 6, 21–29 (2007)

    Article  CAS  Google Scholar 

  2. J. Ma, J. Hu, Z. Li, C.W. Nan, Adv. Mater. 23, 1062–1087 (2011)

    Article  CAS  Google Scholar 

  3. M. Feng, J.J. Wang, J.M. Hu, J. Wang, J. Ma, H.B. Li, Y. Shen, Y.H. Lin, L.Q. Chen, C.W. Nan, Appl. Phys. Lett. 106, 072901 (2015)

    Article  Google Scholar 

  4. S. Dash, R.N.P. Choudhary, P.R. Das, A. Kumar, Can. J. Phys. 93, 738–744 (2015)

    Article  CAS  Google Scholar 

  5. L.G. Wang, C.M. Zhu, H. Luo, S.L. Yuan, J. Electroceram. 35, 59–67 (2015)

    Article  Google Scholar 

  6. M.J. Miah, M.N.I. Khan, A.K.M.A. Hossain, J. Magn. Magn. Mater. 397, 39–50 (2016)

    Article  CAS  Google Scholar 

  7. W.T. Xie, H.Q. Zhou, Q.X. Jiang, H.X. Xu, L.C. Ren, X.F. Luo, L. Qian, J. Mater. Sci.: Mater. Electron. 27, 3839–3844 (2016)

    CAS  Google Scholar 

  8. J.G. Wu, Z. Fan, D.Q. Xiao, J.G. Zhu, J. Wang, Prog. Mater. Sci. 84, 335–402 (2016)

    Article  CAS  Google Scholar 

  9. K. Veerannan, A. Arockiarajan, Sens. Actuators A 236, 380–393 (2015)

    Article  CAS  Google Scholar 

  10. C.P. Fernández, F.L. Zabotto, D. Garcia, R.H.G.A. Kiminami, Ceram. Int. 42, 3239–3249 (2016)

    Article  Google Scholar 

  11. C.A.F. Vaz, J. Hoffman, C.H. Ahn, R. Ramesh, Adv. Mater. 22, 2900–2918 (2010)

    Article  CAS  Google Scholar 

  12. M. Fiebig, T. Lottermoser, D. Meier, M. Trassin, Nat. Rev. Mater. 1, 16046 (2016)

    Article  CAS  Google Scholar 

  13. A. Sundararaj, G. Chandrasekaran, H.A. Therese, K. Annamalai, Nanotechnology 26, 315704 (2015)

    Article  Google Scholar 

  14. M. Feng, J.M. Hu, J.J. Wang, Z. Li, L. Shu, C.W. Nan, Appl. Phys. Lett. 19, 192903 (2013)

    Article  Google Scholar 

  15. A. Kumar, D. Barrionuevo, N. Ortega, A.K. Shukla, S. Shannigrahi, J.F. Scott, R.S. Katiyar, J. Appl. Phys. 106, 132901 (2015)

    Google Scholar 

  16. S.W. Yang, L. Feng, D.L. Zhang, W.C. Huang, S.N. Dong, J.J. Wang, L.J. Zou, X.G. Li, C.W. Nan, J. Alloys Compd. 646, 472–476 (2015)

    Article  CAS  Google Scholar 

  17. R. Gupta, J. Shah, S. Chaudhary, R.K. Kotnala, J. Alloys Compd. 638, 115–120 (2015)

    Article  CAS  Google Scholar 

  18. T. Katayama, S. Yasui, Y. Hamasaki, T. Shiraishi, A. Akama, T. Kiguchi, M. Itoh, Adv. Funct. Mater. 28, 1704789 (2017)

    Article  Google Scholar 

  19. N.S. Negi, K. Bala, A. Yadav, R.K. Kotnala, J. Appl. Phys. 117, 164101 (2015)

    Article  Google Scholar 

  20. H.C. Yu, H.Y. Guo, W.M. Zhua, J. Zhuang, W. Ren, Z.G. Ye, Thin Solid Films 585, 82–85 (2015)

    Article  CAS  Google Scholar 

  21. F.W. Zhang, F. Yang, C.F. Dong, X.T. Liu, H.L. Nan, Y.Y. Wang, Z.H. Zong, M.H. Tang, J. Electron. Mater. 44, 2348–2352 (2015)

    Article  CAS  Google Scholar 

  22. J.W. Kim., C.M. Raghavan, S.S. Kim, J. Sol–Gel. Sci. Technol. 76, 693–698 (2015)

    Article  CAS  Google Scholar 

  23. G. Tan, W. Yang, W. Ye, Z.W. Yue, H.J. Ren, A. Xia, J. Mater. Sci. 52, 2694–2704 (2017)

    Article  CAS  Google Scholar 

  24. G.H. Dong, G.Q. Tan, Y.Y. Luo, T. Wang, H.J. Ren, A. Xia, J. Alloys Compd. 654, 419–423 (2016)

    Article  CAS  Google Scholar 

  25. P.C. Sati, M. Arora, M. Kumar, M. Tomar, V. Gupta, J. Mater. Sci: Mater. Electron. 18, 1011–1014 (2014)

    Google Scholar 

  26. J. Li, Y.W. Li, D.P. Zhu, Q.W. Wang, Y. Zhang, Y.D. Zhu, M.Y. Li, J. Alloys Compd. 661, 38–42 (2016)

    Article  CAS  Google Scholar 

  27. P. Zhang, C. Gao, F. Lv, Y. Wei, Appl. Phys. Lett. 105, 152904 (2014)

    Article  Google Scholar 

  28. S. Roy, S.B. Majumder, J. Alloys Compd. 538, 153–159 (2012)

    Article  CAS  Google Scholar 

  29. S.E. Park, T.R. Shrout, IEEE. Trans. Ultrason. Ferroelectr. 44, 1140–1147 (1997)

    Article  Google Scholar 

  30. B. Zhu, C.T. Yang, Q.T. Xie, Y.L. Zhang, P. Li, Ferroelectrics 445, 18–25 (2013)

    Article  CAS  Google Scholar 

  31. D. Zhou, R. Takahashi, Y. Zhou, D. Kim, V.K. Suresh, Y.H. Chu, Q. He, P. Munroe, M. Lippmaa, J. Seidel, N. Valanoor, Adv. Electron. Mater. 3, 1600295 (2016)

    Article  Google Scholar 

  32. M. Shi, R.Z. Zuo, Y.D. Xu, Y.Z. Jiang, G.Y. Yu, H.L. Su, J.G. Zhong, J. Alloys Compd. 512, 165–170 (2012)

    Article  CAS  Google Scholar 

  33. M. Feng, W. Wang, H. Ke, J.C. Rao, Y. Zhou, J. Alloys Compd. 495, 154–157 (2010)

    Article  CAS  Google Scholar 

  34. W. Rao, Y.B. Wang, Y.A. Wang, J.X. Gao, W.L. Zhou, J. Yu, J. Mater. Sci.: Mater. Electron. 24, 4192–4196 (2013)

    CAS  Google Scholar 

Download references

Acknowledgements

The authors would like to thank the financial support for this work from National Natural Science Foundation of China (Grant Nos. 51372055, 51621091, 51772126, and 21201078), Key Laboratory of Functional Materials Physics and Chemistry of the Ministry of Education (Item Nos. 2015003, 2015003 and 2016010), State Key Laboratory of New Ceramic and Fine Processing of Tsinghua University (Item No. KF201505), Program for the Development of Science and Technology of Jilin Province (Item No. 20170101062JC), and the 13th Five-Year Program for Science and Technology of Education Department of Jilin Province (Item No. JJKH20170370KJ).

Author information

Authors and Affiliations

  1. Institute for Advanced Ceramics, Materials Science and Engineering, Harbin Institute of Technology, Harbin, 150001, People’s Republic of China

    Ao-pei Wang, Wen Wang, Hua Ke & Yu Zhou

  2. Key Laboratory of Functional Materials Physics and Chemistry of the Ministry of Education, Jilin Normal University, Changchun, 130103, People’s Republic of China

    Ao-pei Wang, Ming Feng, Hai-bo Li, Xue Zhao & Hang Xu

Authors
  1. Ao-pei Wang
    View author publications

    You can also search for this author in PubMed Google Scholar

  2. Ming Feng
    View author publications

    You can also search for this author in PubMed Google Scholar

  3. Wen Wang
    View author publications

    You can also search for this author in PubMed Google Scholar

  4. Hai-bo Li
    View author publications

    You can also search for this author in PubMed Google Scholar

  5. Xue Zhao
    View author publications

    You can also search for this author in PubMed Google Scholar

  6. Hang Xu
    View author publications

    You can also search for this author in PubMed Google Scholar

  7. Hua Ke
    View author publications

    You can also search for this author in PubMed Google Scholar

  8. Yu Zhou
    View author publications

    You can also search for this author in PubMed Google Scholar

Corresponding authors

Correspondence to Ming Feng or Wen Wang.

Rights and permissions

Reprints and permissions

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Wang, Ap., Feng, M., Wang, W. et al. Influence of composition ratio on ferroelectric, magnetic and magnetoelectric properties of PMN–PT/CFO composite thin films. J Mater Sci: Mater Electron 29, 10164–10169 (2018). https://doi.org/10.1007/s10854-018-9065-5

Download citation

  • Received:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.1007/s10854-018-9065-5

Search

Navigation