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Development of High-Field and High-Pressure ESR System and Application to Triangular Antiferromagnet \(\hbox {CsCuCl}_{3}\)

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Abstract

We have developed a new hybrid-type pressure cell for the high-pressure and high-field electron spin resonance (ESR) measurement using a widely used Oxford 15 T superconducting magnet with the variable temperature insert (VTI). The size of the pressure cell was optimized and a probe was also specially designed so as to be fitted to the VTI. We confirmed that the new pressure cell can generate the pressure up to at least 2.0 GPa repeatedly. Using this new ESR system, high-pressure and high-field ESR measurement was performed on the triangular antiferromagnet \(\hbox {CsCuCl}_{3}\) for \(H \parallel c\) at 4.2 K in the frequency region 60 GHz–420 GHz. We succeeded in observing the significant pressure effect of this compound. Moreover, a new ESR mode which is expected to correspond to the 1/3 magnetization plateau was observed at 0.80 GPa.

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Acknowledgements

This research was partially supported by Grants-in-Aid for Scientific Research (C) (No. 16K05416) from Japan Society for the Promotion of Science.

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Authors and Affiliations

  1. Graduate School of Science, Kobe University, Kobe, 657-8501, Japan

    Ryosuke Okuto, Eito Ohki & Eiji Ohmichi

  2. Research Facility Center for Science and Technology, Kobe University, Kobe, 657-8501, Japan

    Takahiro Sakurai

  3. Molecular Photoscience Research Center, Kobe University, Kobe, 657-8051, Japan

    Keigo Hijii, Susumu Okubo & Hitoshi Ohta

  4. Organization for Advanced and Integrated Research, Kobe Univ., Nada, Kobe, 657-8501, Japan

    Hideyuki Takahashi

  5. Institute for Solid State Physics, University of Tokyo, Chiba, 277-8581, Japan

    Yoshiya Uwatoko

  6. Department of Physics, Tokyo Institute of Technology, Tokyo, 152-8551, Japan

    Hidekazu Tanaka

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  1. Ryosuke Okuto
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  2. Eito Ohki
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  3. Takahiro Sakurai
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  5. Hideyuki Takahashi
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  6. Eiji Ohmichi
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  7. Susumu Okubo
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  8. Hitoshi Ohta
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  9. Yoshiya Uwatoko
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  10. Hidekazu Tanaka
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Correspondence to Takahiro Sakurai.

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Okuto, R., Ohki, E., Sakurai, T. et al. Development of High-Field and High-Pressure ESR System and Application to Triangular Antiferromagnet \(\hbox {CsCuCl}_{3}\). Appl Magn Reson 50, 1059–1065 (2019). https://doi.org/10.1007/s00723-019-01134-8

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  • DOI: https://doi.org/10.1007/s00723-019-01134-8

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