Abstract
Turbulent mixing in stratified environments represents a challenging task in experimental turbulence research, especially when large density gradients are desired. When optical measurement techniques like particle image velocimetry (PIV) are applied to stratified liquids, it is common practice to combine two aqueous solutions with different density but equal refractive index, to suppress particle image deflections. While refractive image matching (RIM) has been developed in the late 1970s, the achieved limit of 4% density ratio was not rivalled up to day. In the present work, we report a methodology, based on the behavior of excess properties and their change in a multicomponent system while mixing, that allows RIM for solutions with higher density differences. The methodology is then successfully demonstrated using a ternary combination of water, isopropanol and glycerol, for which RIM in presence of a density ratio of 8.6% has been achieved. Qualitative PIV results of a turbulent buoyant jet with 8.6% density ratio are shown.
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References
Adrian RJ, Westerweel J (2011) Particle image velocimetry. Cambridge University Press, Cambridge
Alahyari A, Longmire EK (1994) Particle image velocimetry in a variable density flow: application to a dynamically evolving microburst. Exp Fluids 17:434–440
Anwar A, Tariq M (2007) Deviations in refractive index parameters and applicability of mixing rules in binary mixtures of benzene + 1,2-dichloroethane at different temperatures. J Chem Eng Com 195(1):43–56
Augier P, Billant P, Negretti M, Chomaz J-M (2014) Experimental study of stratified turbulence forced with columnar dipoles. Phys Fluids 26:046603
Bos WJT (2014) On the anisotropy of the turbulent passive scalar in the presence of a mean scalar gradient. J Fluid Mech 744:38–64
Brocos P, Pinerio A, Bravo R, Amigo A (2003) Refractive indices, molar volumes and molar refractions of binary liquid mixtures: concepts and correlations. Chem Phys 5:550–557
Daviero GJ, Roberts PJW, Maile K (2001) Refractive index matching in large-scale stratified experiments. Exp Fluids 31:119–126
Garcia B, Alcalde R, Aparicio S, Leal JM (2002) The N-methylpyrrolidone–(C1–C10) alkan-1-ols solvent systems. Phys Chem 4:1170–1177
Hannoun IA (1985) Matching the refractive index in density stratified flows. Tech Memo 85-1, WK Keck Laboratory of Hydraulics and Water Resources, California Institute of Technology
McDougall TJ (1979) On the elimination of refractive-index variations in turbulent density-stratified liquid flows. J Fluid Mech 93:83–96
Paladino D, Andreani M, Zboray R, Dreier J (2012) Toward CFD-grade database addressing LWR containment phenomena. Nucl Eng Dsgn 253:331–342
Petrov V, Manera A (2011). Validation of STAR-CCM+ for buoyancy driven mixing in a PWR reactor pressure vessel. In: Proc. of 14th int. topical meeting on nuclear reactor thermal-hydraulics (NURETH-14), Toronto, Canada, September 25–30
Riley JJ, De Bruyn Kops SM (2003) Dynamics of turbulence strongly influenced by buoyancy. Phys Fluids 15:2047–2059
Touriño A, Hervello M, Moreno V, Marino G, Iglesias M (2004) Changes of refractive indices in ternary mixtures containing chlorobenzene + n-hexane + (n-heptane or n-octane) at 298.15 K. J Serbian Chem Soc 69(6):461–475
Xiang X, Madison TJ, Sellappan P, Spedding GR (2015) The turbulent wake of a towed grid in a stratified fluid. J Fluid Mech 775:149–177
Yahya M, Saghir MZ (2015) Prediction and experimental measurement of refractive index in ternary hydrocarbon mixtures. J Chem Eng Data 60(8):2329–2342
Acknowledgements
We are indebted to colleagues at the Experimental and Computational Multiphase Flow Group of University of Michigan for many helpful discussions as well as assistance with various aspects of the experiments. The work was made possible by the generous support of DOE NEUP under Grant no 14-6552.
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Krohn, B., Manera, A. & Petrov, V. A novel method to create high density stratification with matching refractive index for optical flow investigations. Exp Fluids 59, 66 (2018). https://doi.org/10.1007/s00348-018-2522-3
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DOI: https://doi.org/10.1007/s00348-018-2522-3