Abstract
Understanding the fundamental mechanisms behind industrial laser-based technologies represents one the cornerstones of the development and tailoring of new materials. With the thin-film deposition using laser ablation being one of the most important techniques for obtaining complex materials with controllable stoichiometry, there is a high request for both experimental and theoretical studies towards understanding the behavior of multi-component alloys under high-power laser irradiation. Here we investigate the laser ablation process on two ternary metallic alloys (Cu–Mn–Al and Fe–Mn–Si) by means of space-and time-resolved optical emission spectroscopy and fast camera imaging with the focus being on the spatial distribution of each composing element. Information regarding the kinetic and thermal energy of the ejected particles is extracted and discussed in the framework of an inner structuring of the laser-produced plasmas based on a mass and energy distribution. The hypothesis is then verified by implementing a fractal analysis to the multi-component plasmas. The theoretical fractal approach offers results in good agreement with the experimental data gives important insight in the inner dynamics of complex laser-produced plasmas.
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A. Blug, F. Abt, L. Nicolosi, A. Heider, R. Weber, D. Carl, H. Höfler, R. Tetzlaff, Appl. Phys. B 108, 97–107 (2012)
K. Deng, X. Wei, X. Wang, Y. Chen, M. Yin, Appl. Phys. B 102, 555–558 (2011)
D. Bäuerle, Appl. Phys. B 46(3), 261–270 (1988)
D.K. PallottiX, R. Ni, X. Fittipaldi, S. Wang, A. Lettieri, S.Amoruso Vecchione, Appl. Phys. B 119(3), 4445–4452 (2015)
J. Singh, R. Kumar, S. Awasthi, V. Singh, A.K. Rai, Food Chem. 221, 1778–1783 (2017)
J. Hermann, E. Axente, F. Pelascini, V. Craciun, Anal. Chem. 91(3), 2544–2550 (2019)
A. Ojeda-G-P, C.W. Schneider, M. Döbeli, T. Lippert, A. Wokaun, J. Appl. Phys. 121, 135306 (2017)
A. Chehrghani, M.J. Torkamany, Opt. Laser Eng. 51, 61–68 (2013)
B.D. Ngom, S. Lafane, S. Abdelli-Messaci, T. Kerdja, M. Maaza, Appl. Phys. A Mater. Sci. Process. 122, 1–7 (2016)
C.R. Menegatti, G. Nicolodelli, G.S. Senesi et al., Appl. Phys. B 125, 74 (2019)
L. Liu, M. Chen, Opt. Laser Eng. 49, 1124–1231 (2011)
S.A. Irimiciuc, G. Bulai, S. Gurlui, M. Agop, Powder Technol. 339, 273–280 (2018)
S. Irimiciuc, G. Bulai, M. Agop, S. Gurlui, Appl. Phys. A Mater. Sci. Process. 615, 1–15 (2018)
D.W. Hahn, N. Omenetto, Appl. Spectrosc. 64, 335A–366A (2010)
N. Glumac, G. Elliot, Opt. Laser Eng. 45, 27–35 (2009)
M. Hauer, D.J. Funk, T. Lippert, A. Wokaun, Opt. Laser Eng. 43, 545–556 (2005)
K.K. Anoop, M.P. Polek, R. Bruzzese, S. Amoruso, S.S. Harilal, J. Appl. Phys. 117, 083108 (2015)
S.A. Irimiciuc, I. Mihaila, M. Agop, Phys. Plasmas 21, 093509 (2014)
P.K. Diwakar, S.S. Harilal, A. Hassanein, M.C. Phillips, Expansion dynamics of ultrafast laser produced plasmas in the presence of ambient argon. J. Appl. Phys. 116, 133301 (2014)
S. Irimiciuc, R. Boidin, G. Bulai, S. Gurlui, P. Nemec, V. Nazabal, C. Focsa, Appl. Surf. Sci. 418, 594–600 (2017)
D.B. Geohegan, MRS Proc. 285, 27 (1992)
D.B. Geohegan, A.A. Puretzky, G. Duscher, S.J. Pennycook, Appl. Phys. Lett. 72, 2987–2989 (1998)
S.A. Irimiciuc, S. Gurlui, P. Nica, C. Focsa, M. Agop, J. Appl. Phys. 12, 083301 (2017)
G. Cristoforetti, S. Legnaioli, L. Pardini, V. Palleschi, A. Salvetti, E. Tognoni, Spectrochim. Acta Part B At. Spectrosc. 61, 340–350 (2006)
J. Singh, S. Thakur, Laser induced breakdown spectroscopy (Elsevier, Amsterdam, 2007)
G. Colonna, L.D. Pietanza, M. Capitelli, Spectrochim. Acta Part B At. Spectrosc. 56, 587–589 (2001)
G. Colonna, D. D’Ammando, L.D. Pietanza, M. Capitelli, Plasma Phys. Control. Fusion 57, 014009 (2015)
C.P. Cristescu, Nonlinear dynamics and Chaos. Theoretical fundamental and applications (Romanian Academy Publishing, Bucharest, 2008)
B. Mandelbrot, The fractal geometry of nature (WH Freeman Publisher, New York, 1993)
L. Nottale, Scale relativity and fractal space-time: an approach to unifying relativity and quantum mechanics (Imperial College Press, London, 2011)
I. Merches, M. Agop, Differentiability and fractality in dynamics of physical systems (World Scientific Publisher, Singapore, 2016)
M. Agop, V.P. Paun, On the new paradigm of fractal theory. Fundamental and applications (Romanian Academy Publishing House, Bucharest, 2017)
M. Agop, I. Merches, Operational procedures describing physical systems (CRC Press Taylor and Francis Group, London, 2019)
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This work has been funded by the National Authority for Scientific Research and Innovation in the framework of Nucleus Program—16N/2019
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Irimiciuc, S.A., Gurlui, S. & Agop, M. Particle distribution in transient plasmas generated by ns-laser ablation on ternary metallic alloys. Appl. Phys. B 125, 190 (2019). https://doi.org/10.1007/s00340-019-7302-0
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DOI: https://doi.org/10.1007/s00340-019-7302-0