Magnetic domain behaviour of MgFe₂O₄-CoFe₂O₄ system

Abstract

Ferrites with the composition Mg_1−x CO _x Fe₂O₄(0<x≤0·33) were synthesized by solid state reaction between MgO,α-Fe₂O₃ and CoFe₂O₄ at 1300°C. The compounds were analyzed from the results of x-ray diffraction, magnetic hysteresis and initial susceptibility (χ) studies. All the compounds of the series were found to be monophasic with no appreciable change in their lattice parameter. The saturation magnetization and coercive field (H _c ) values increased with increasing cobalt ferrite content. Similarly, the shapes of theχ-T curves and temperature variations ofH _c values indicated that the magnetic behaviour changes from multi-domain to single domain with increasing cobalt content. The results are similar to those observed for the (MgFe₂O₄)_1−x (Co₃O₄) system.