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Magnetic Interactions and Magnetocaloric Effect in (La0.5Pr0.5)0.6Ba0.4MnO3: Effect of A-Site Codoping

Abstract

The structural, magnetic, and magnetocaloric properties of polycrystalline (La0.5Pr0.5)0.6Ba0.4MnO3 (LPBMO), fabricated by a conventional solid-state reaction method, are reported herein. LPBMO undergoes a second-order paramagnetic–ferromagnetic phase transition around a Curie temperature TC ∼ 277 K. The maximum magnetic entropy change −ΔSMmax is ∼ 3.22 J kg−1 K−1 for a magnetic field change of 5 T. Based on the modified Arrott plot and the iterative Kouvel–Fisher methods, a set of critical exponents (β = 0.514 ± 0.010, γ = 1.164 ± 0.013, and Δ  = 3.265 ± 0.023) have been determined. These values are close to those expected for the mean-field model with long-range interactions below TC and for the three-dimensional (3D) Ising model with short-range interactions above TC. The effect of A-site codoping (La, Pr) on the magnetic and magnetocaloric properties of LPBMO has been analyzed and discussed.

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Correspondence to Nguyen Thi My Duc or Ngo Thu Huong or Manh-Huong Phan.

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Duc, N.T.M., Hung, C., Huong, N.T. et al. Magnetic Interactions and Magnetocaloric Effect in (La0.5Pr0.5)0.6Ba0.4MnO3: Effect of A-Site Codoping. Journal of Elec Materi 49, 2596–2607 (2020). https://doi.org/10.1007/s11664-020-07974-6

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Keywords

  • Perovskite
  • manganite
  • magnetocaloric effect
  • magnetic refrigeration
  • critical behavior
  • critical exponents