Abstract
The activities of 228Th, 230Th, 234Th, 226Ra, 228Ra, 210Po, and 210Pb have been reported in the East Sea (Japan Sea) over the past few decades. The activities of thorium isotopes over the entire depth of the East Sea ranged from 0.4 to 8.3 dpm 100 L−1 for 228Th, 0.06 to 0.37 dpm 1000 L−1 for 230Th, and 0.4 to 2.1 dpm L−1 for 234Th. Thorium isotopes in the East Sea were used for determining the collection efficiency of sediment traps (using 230Th) and the annual vertical flux of particulate organic carbon (using 234Th). The activities of radium isotopes over the entire depth of the East Sea ranged from 0.3 to 11 dpm 100 L−1 for 228Ra and 6.4 to 16 dpm 100 L−1 for 226Ra. Radium isotopes in the East Sea were used for determining the vertical eddy diffusion coefficient (using 228Ra) and the residence time of deep water (using 226Ra). The activities of 210Pb over the entire depth ranged from 4.4 to 27 dpm 100 L−1, and the activities for 210Po over the entire depth ranged from 1.5 to 11 dpm 100 L−1. The 210Pb and 210Po in the East Sea were used for estimating the residence time of trace elements in the dissolved, colloid, and particulate phases. In summary, U-series radioisotopes have provided useful information on various physical and biogeochemical processes in the East Sea.
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References
Bacon M, Spencer D, Brewer P (1976) 210Pb/226Ra and 210Po/210Pb disequilibria in seawater and suspended particulate matter. Earth Planet Sci Lett 32(2):277–296
Bacon MP, Belastock RA, Tecotzky M, Turekian KK, Spencer DW (1988) Lead-210 and polonium-210 in ocean water profiles of the continental shelf and slope south of New England. Cont Shelf Res 8(5):841–853
Baskaran M, Santschi P, Benoit G, Honeyman B (1992) Scavenging of thorium isotopes by colloids in seawater of the Gulf of Mexico. Geochim Cosmochim Acta 56(9):3375–3388
Broecker W (1963) Radioisotopes and large-scale oceanic mixing. In Hill MN (ed) The sea: ideas and observations on progress in the study of the seas 2:88–108
Buesseler KO (1998) The decoupling of production and particulate export in the surface ocean. Global Biogeochem Cycles 12(2):297–310
Chen JH, Lawrence Edwards R, Wasserburg GJ (1986) 238U, 234U and 232Th in seawater. Earth Planet Sci Lett 80(3–4):241–251
Cherry R, Fowler S, Beasley T, Heyraud M (1975) Polonium-210: its vertical oceanic transport by zooplankton metabolic activity. Mar Chem 3(2):105–110
Chung Y (1987) 210Pb in the western Indian Ocean: distribution, disequilibrium, and partitioning between dissolved and particulate phases. Earth Planet Sci Lett 85(1):28–40
Chung Y, Craig H (1983) 210Pb in the Pacific: the GEOSECS measurements of particulate and dissolved concentrations. Earth Planet Sci Lett 65(2):406–432
Chung Y, Finkel R (1988) 210Po in the western Indian Ocean: distributions, disequilibria and partitioning between the dissolved and particulate phases. Earth Planet Sci Lett 88(3):232–240
Chung Y, Wu T (2005) Large 210Po deficiency in the northern South China Sea. Cont Shelf Res 25(10):1209–1224
Coale KH, Bruland KW (1985) 234Th:238U disequilibria within the California current. Limnol Oceanogr 30(1):22–33
Cochran J (1992) The oceanic chemistry of the uranium- and thorium-series nuclides. In Ivanovich M, Harmon RS (eds) Uranium-Series disequilibrium: applications to earth, marine, and environmental sciences, pp 334–395
Cochran JK, Bacon MP, Krishnaswami S, Turekian KK (1983) 210Po and 210Pb distributions in the central and eastern Indian Ocean. Earth Planet Sci Lett 65(2):433–452
Cochran JK, Barnes C, Achman D, Hirschberg DJ (1995) Thorium-234/uranium-238 disequilibrium as an indicator of scavenging rates and particulate organic carbon fluxes in the Northeast Water Polynya. Greenland. J Geophys Res 100(C3):4399–4410
Fowler SW, Knauer GA (1986) Role of large particles in the transport of elements and organic compounds through the oceanic water column. Prog Oceanogr 16(3):147–194
Goldberg ED, Koide M (1962) Geochronological studies of deep sea sediments by the ionium/thorium method. Geochim Cosmochim Acta 26(3):417–450
Guo L, Santschi PH, Baskaran M (1997) Interactions of thorium isotopes with colloidal organic matter in oceanic environments. Colloids Surf A 120(1):255–271
Harada K, Tsunogai S (1986) 226Ra in the Japan Sea and the residence time of the Japan Sea water. Earth Planet Sci Lett 77(2):236–244
Hong GH, Baskaran M, Lee HK, Kim SH (2008a) Sinking fluxes of particulate U-Th radionuclides in the East Sea (Sea of Japan). J Oceanogr 64(2):267–276
Hong GH, Kim YI, Baskaran M, Kim SH, Chung CS (2008b) Distribution of 210Po and export of organic carbon from the euphotic zone in the southwestern East Sea (Sea of Japan). J Oceanogr 64(2):277–292
Kim D, Choi MS, Oh HY, Song YH, Noh JH, Kim KH (2011a) Seasonal export fluxes of particulate organic carbon from 234Th/238U disequilibrium measurements in the Ulleung Basin (Tsushima Basin) of the East Sea (Sea of Japan). J Oceanogr 67(5):577–588
Kim G (2001) Large deficiency of polonium in the oligotrophic ocean’s interior. Earth Planet Sci Lett 192(1):15–21
Kim G, Hwang DW (2002) Tidal pumping of groundwater into the coastal ocean revealed from submarine 222Rn and CH4 monitoring. Geophys Res Lett 29(14):23-1–23-4
Kim G, Kim JS, Hwang DW (2011b) Submarine groundwater discharge from oceanic islands standing in oligotrophic oceans: implications for global biological production and organic carbon fluxes. Limnol Oceanogr 56(2):673–682
Kim G, Ryu JW, Yang HS, Yun ST (2005) Submarine groundwater discharge (SGD) into the Yellow Sea revealed by 228Ra and 226Ra isotopes: implications for global silicate fluxes. Earth Planet Sci Lett 237(1):156–166
Kim TH, Kim G (2012) Important role of colloids in the cycling of 210Pb and 210Po in the ocean: results from the East/Japan Sea. Geochim Cosmochim Acta 95:134–142
Koczy F (1963) Age determination in sediments by natural radioactivity. In Hill MN (ed) The sea: ideas and observations on progress in the study of the seas 3:816–831
Li YH, Feely HW, Santschi PH (1979) 228Th-228Ra radioactive disequilibrium in the New York Bight and its implications for coastal pollution. Earth Planet Sci Lett 42(1):13–26
Masqué P, Sanchez-Cabeza J, Bruach J, Palacios E, Canals M (2002) Balance and residence times of 210Pb and 210Po in surface waters of the northwestern Mediterranean Sea. Cont Shelf Res 22(15):2127–2146
Moon DS, Kim KH, Noh I (2000) The vertical fluxes of particles and radionuclides in the East Sea. J Korean Soc Oceanogr 35(1):16–33
Moore WS, Sarmiento JL, Key RM (2008) Submarine groundwater discharge revealed by 228Ra distribution in the upper Atlantic Ocean. Nat Geosci 1(5):309–311
Moran SB, Buesseler KO (1992) Short residence time of colloids in the upper ocean estimated from 238U-234Th disequilibria. Nature 359(6392):221–223
Moran SB, Shen CC, Weinstein SE, Hettinger LH, Hoff JH, Edmonds HN, Edwards RL (2001) Constraints on deep water age and particle flux in the Equatorial and South Atlantic Ocean based on seawater 231Pa and 230Th data. Geophys Res Lett 28(18):3437–3440
Murray JW, Downs JN, Strom S, Wei CL, Jannasch HW (1989) Nutrient assimilation, export production and 234Th scavenging in the eastern equatorial Pacific. Deep-Sea Res 36(10):1471–1489
Nozaki Y (1974) Radium-226, Lead-210 and polonium-210 in sea water and their use in oceanography, Ph.D. thesis, Hokkaido Univ., p 148
Nozaki Y, Ikuta N, Yashima M (1990) Unusually large 210Po deficiencies relative to 210Pb in the Kuroshio Current of the East China and Philippine Seas. J Geophys Res 95(C4):5321–5329
Nozaki Y, Thomson J, Turekian KK (1976) The distribution of 210Pb and 210Po in the surface waters of the Pacific Ocean. Earth Planet Sci Lett 32(2):304–312
Nozaki Y, Yamada M (1987) Thorium and protactinium isotope distribution in waters of the Japan Sea. Deep-Sea Res 34(8):1417–1430
Nozaki Y, Zhang J, Takeda A (1997) 210Pb and 210Po in the equatorial Pacific and the Bering Sea: the effects of biological productivity and boundary scavenging. Deep-Sea Res II 44(9):2203–2220
Okubo T (1980) Radium-228 in the Japan Sea. J Ocean Soc Japan 36(5):263–268
Owens SA, Buesseler KO, Sims KWW (2011) Re-evaluating the 238U-salinity relationship in seawater: implications for the 238U–234Th disequilibrium method. Mar Chem 127(1):31–39
Roether W, Kromer B (1978) Field determination of air-sea gas exchange by continuous of radon-222. Pure appl Geophys 116(2–3):476–485
Settle D, Patterson C, Turekian K, Cochran J (1982) Lead precipitation fluxes at tropical oceanic sites determined from 210Pb measurements. J Geophys Res Oceans (1978–2012) 87(C2):1239–1245
Stewart GM, Fisher NS (2003) Experimental studies on the accumulation of polonium-210 by marine phytoplankton. Limnol Oceanogr 48(3):1193–1201
Trimble SM, Baskaran M, Porcelli D (2004) Scavenging of thorium isotopes in the Canada Basin of the Arctic Ocean. Earth Planet Sci Lett 222:915–932
Tsunogai S, Harada K (1980) 226Ra and 210Pb in the western North Pacific. In: Goldberg E, Horibe Y, Saruhashi K (eds) Isotope marine chemistry, pp 165–191
Turekian KK, Graustein WC, Cochran JK (1989) Lead-210 in the SEAREX program: an aerosol tracer across the Pacific. In: Riley JP, Chester R, Duce RA (eds) Chemical oceanography, vol 10, pp 51–81
Yang H, Kim S, Lee J (1995) Effect of eddy on the cycle of 210Po and 234Th in the central region of Korean East Sea. J Korean Soc Oceanogr 30(4):279–287
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Kim, TH., Kim, J., Kim, G. (2016). Uranium Series Radionuclides. In: Chang, KI., et al. Oceanography of the East Sea (Japan Sea). Springer, Cham. https://doi.org/10.1007/978-3-319-22720-7_8
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DOI: https://doi.org/10.1007/978-3-319-22720-7_8
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