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NON-PROPORTIONALITY AND ENERGY RESOLUTION OF SCINTILLATION DETECTORS

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Radiation Detectors for Medical Applications

Part of the book series: NATO Security through Science Series ((NASTB))

Abstract

The application of scintillation detectors in nuclear medicine utilizing gamma spectrometry methods, as PET and SPECT detectors, and gamma cameras, requires a high energy resolution of the detectors. The limitations of energy resolution are discussed with a special emphasis on non-proportional response of scintillators to gamma rays and electrons, which is of crucial importance to an intrinsic resolution of the crystals. An importance of the scattering of secondary electrons (δ-rays) on intrinsic resolution is pointed out. Examples of the study carried out with different crystals and particularly those used in nuclear medicine are presented.

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REFERENCES

  1. G.F. Knoll, “Radiation Detection and Measurements”, Third Edition, John Willey and Son, New York, 2000

    Google Scholar 

  2. M. Moszynski, “Inorganic scintillation detectors in γ-ray spectrometry”, Nucl. Instr. Meth., A505, 101–110, (2003)

    Google Scholar 

  3. M. Moszynski, “Energy resolution of scintillation detectors”, SPIE Proceedings, in press

    Google Scholar 

  4. P. Dorenbos, J.T.M. de Haas, C.W.E. van Eijk, “Non-proportionality in the Scintillation Response and the Energy Resolution Obtainable with Scintillation Crystals”, IEEE Trans. Nucl. Sci, 42, 2190–2202, (1995)

    Article  CAS  Google Scholar 

  5. M. Moszyński, J. Zalipska, M. Balcerzyk, M. Kapusta, W. Mengeshe, J.D. Valentine, “Intrinsic energy resolution of NaI(Tl)”, Nucl. Instr. Meth., A484, 259–269, (2002)

    Google Scholar 

  6. G.G. Kelly, P.R. Bell, R.C. Davis and N.A. Lazar, “Intrinsic energy resolution”, IRE Trans, on Nucl, Sci., NS3, 57–58, (1956)

    Article  Google Scholar 

  7. P. Iredale, “The effect of the non-proportional response of NaI(Tl) crystals to electrons upon the resolution for γ-rays”, Nucl. Instr. Meth., 11, 340–346, (1961)

    Article  CAS  Google Scholar 

  8. C.D. Zerby, A. Meyer, R.B. Murray, “Intrinsic line broadening in NaI(Tl) gamma-ray spectrometers”, Nucl. Instr. Meth., 12, 115–123, (1961)

    Article  Google Scholar 

  9. G.H. Narayan and J.R. Prescott, “The contribution of the NaI(Tl) crystal to the total line width of NaI(Tl) scintillation counters”, IEEE Trans. Nucl. Sci, NS-15, 162–166, (1968)

    Article  Google Scholar 

  10. J.R. Prescott and G.H. Narayan, “Electron response and intrinsic line-widths in NaI(Tl) Crystals”, Nucl. Instr. Meth., 75, 51–55, (1969)

    Article  CAS  Google Scholar 

  11. P. Dorenbos, J.T.M. de Hass, C.W.E. van Eijk, C.L. Melcher, and J.S. Schweitzer, “Nonlinear response in the scintillation yield of Lu2SiO5:Ce, IEEE Trans, on Nucl. Sci., 41,1052–1061, (1994)

    Article  Google Scholar 

  12. P. Dorenbos, J.T.M. de Hass and C.W.E. van Eijk, “Non-proportional response in the light yield of inorganic scintillators”, 1994 IEEE Nucl. Sci. Symp. Norfolk, USA, Conference Records, p. 304–6

    Google Scholar 

  13. T.D. Taulbee, B.D. Rooney, W. Mengesha, and J.D. Velentine, “The Measured Electron Response Nonproportionalities of CaF2, BGO, and LSO”, IEEE Trans. Nucl. Sci., 44, 489–493, (1997)

    Article  CAS  Google Scholar 

  14. J.D. Valentine and B.D. Rooney, “Design of a Compton spectrometer for studying scintillator nonlinearity and intrinsic resolution”, Nucl. Instr. and Meth., A353, 37–40, (1994)

    Google Scholar 

  15. B.D. Rooney and J.D. Valentine, “Benchmarking the Compton Coincidence Technique for measuring electron response nonproportionality in inorganic scintillators”, IEEE Trans. Nucl. Sci., 43, 1271–1276, (1996)

    Article  CAS  Google Scholar 

  16. B.D. Rooney and J. D. Valentine, “Scintillator light yield nonproportionality: calculating photon response using measured electron response”, IEEE Trans. Nucl. Sci., 44, 509–16, (1997)

    Article  CAS  Google Scholar 

  17. W. Mengesha, T.D. Taulbee, B.D. Rooney and J.D. Valentine, “Light Yield Nonproportionality of CsI(Tl), CsI(Na), and YAP”, IEEE Trans. Nucl. Sci., 45, 456–460, (1998)

    Article  CAS  Google Scholar 

  18. J.D. Valentine, B.D. Rooney, and J. Li, “The Light Yield Nonproportionality Component of Scintillator Energy Resolution”, IEEE Trans. Nucl. Sci., 45, 512–517, (1998)

    Article  CAS  Google Scholar 

  19. M. Kapusta, M. Balcerzyk, M. Moszyński, J. Pawelke. “A high-energy resolution observed from a YAP:Ce scintillator”, Nucl. Instr. Meth., A421, 610–13, (1999)

    Google Scholar 

  20. M. Balcerzyk, M. Moszyński, M. Kapusta, “Energy resolution of contemporary scintillators. Quest for high resolution, proportional detector”, Proc. of Fifth Int. Conf. on Inorganic Scintillators and Their Application, Moscow, August 16–20. (1999), p. 167

    Google Scholar 

  21. M. Balcerzyk, M. Moszyński, M. Kapusta, D. Wolski, J. Pawelke, C.L. Melcher, “YSO, LSO, GSO and LGSO. A Study of Energy Resolution and Non-Proportionality”, IEEE Trans. Nucl. Sci., 47, 1319–1323, (2000)

    Article  CAS  Google Scholar 

  22. M. Moszyński, M. Kapusta, D. Wolski, M. Szawlowski, W. Klamra, “Energy Resolution of Scintillation Detectors Readout with Large Area Avalanche Photodiodes and Photomultipliers”, IEEE Trans. Nucl. Sci., 45, 472–77, (1998)

    Article  Google Scholar 

  23. M. Moszyński, M. Kapusta, J. Zalipska, M. Balcerzyk, D. Wolski, M. Szawlowski and W. Klamra, “Low energy gamma-ray scintillation detection with large area avalanche photodiodes”, IEEE Trans. Nucl. Sci., 46, 243, (1999)

    Article  Google Scholar 

  24. W. Mengesha, J.D. Valentine, “Benchmarking NaI(Tl) Electron Energy Resolution Measurements”, IEEE Trans. Nucl. Sci., 49, 2420–2426, (2002)

    Article  CAS  Google Scholar 

  25. M. Moszynski, M. Balcerzyk, W Czarnacki, M. Kapusta, W. Klamra, A. Syntfeld, M. Szawlowski, “Intrinsic Resolution and Light Yield Non-proportionality of BGO”, IEEE Trans. Nucl. Sci., 51, 1074, (2004)

    Article  CAS  Google Scholar 

  26. E. Breitenberger, “Scintillation spectrometers statistics”, Progress in Nucl. Phys. 4, 56–94, (1956)

    Google Scholar 

  27. D. Engelkemeir, “Nonlinear response of NaI(Tl) to photons”, Rev. Sci. Instr., 27, 589–591, (1956)

    Article  CAS  Google Scholar 

  28. R.B. Murray and A. Meyer, “Scintillation Response of Activated Inorganic Crystals to Various Charged Particles”, Phys. Rev., 112, 815–826, (1961)

    Article  Google Scholar 

  29. H. Leutz, C. D’Ambrosio, “On the scintillation response of NaI(Tl)-crystals”, IEEE Trans. Nucl. Sci., 44, 190–193, (1997)

    Article  CAS  Google Scholar 

  30. P.A. Rodnyi, “Physical processes in inorganic scintillators”, CRC Press, New York, 1997

    Google Scholar 

  31. M. Moszyński, M. Balcerzyk, M. Kapusta, A. Syntfeld, D. Wolski, G. Pausch, J. Stein, P. Schotanus, “CdWO4 Crystal in Gamma-ray Spectrometry”, IEEE Trans. Nucl. Sci., in press

    Google Scholar 

  32. M. Moszyński, M. Balcerzyk, W. Czarnacki,_A. Nassalski, T. Szczęśniak,_M. Moszyński, H. Kraus, V. B. Mikhailik, I.M. Solskii, “Characterization of CaWO4 scintillator at room and liquid nitrogen temperatures”, Nucl. Instr. Meth., in press

    Google Scholar 

  33. M. Moszyński, W. Czarnacki, M. Kapusta, M. Szawlowski, W. Klamra, P. Schotanus, “Energy resolution and light yield non-proportionality of pure NaI scintillator studied with large area avalanche photodiodes at liquid nitrogen temperature”, Nucl. Instr. Meth., A., A486, 13–17, (2002)

    Article  Google Scholar 

  34. M. Moszyński, W. Czarnacki, W. Klamra, M. Szawlowski, P. Schotanus, M. Kapusta, “Intrinsic Energy Resolution of pure NaI Studied with Large Area Avalanche Photodiodes at Liquid Nitrogen Temperature”, Nucl. Instr. Meth., A., A505, 63–67, (2003)

    Article  CAS  Google Scholar 

  35. M. Moszynski, M. Balcerzyk, W. Czarnacki, M. Kapusta, W. Klamra, P. Schotanus, A. Syntfeld, M. Szawlowski, “Study of Pure NaI at Room and Liquid Nitrogen Temperatures”, IEEE Trans. Nucl Sci., 50, 767–773, (2003)

    Article  CAS  Google Scholar 

  36. M. Moszyński, M. Balcerzyk, W. Czarnacki, M. Kapusta, W. Klamra, P. Schotanus, A. Syntfeld, M. Szawlowski, “Energy Resolution and Non-proportionality of the Light Yield of Pure CsI at Liquid Nitrogen Temperature”, Nucl. Instr. Meth., A537, 357–362, (2005)

    Google Scholar 

  37. M. Kapusta, P Szupryczyński, C. Melcher, M. Moszynski, M. Balcerzyk, A. A. Carey, W. Czarnacki, A. Spurrier, A. Syntfeld, “Non-proportionality and Thermoluminescence of LSO:Ce”, IEEE Trans. Nucl. Sci., in press

    Google Scholar 

  38. M. Balcerzyk, M. Moszyński, Z. Galazka, M. Kapusta, A. Syntfeld and J-L. Lefaucheur, “Perspectives for high resolution and high light output LuAP:Ce crystals”, IEEE Trans. Nucl. Sci., in press

    Google Scholar 

  39. M. Moszyński, D. Wolski, T. Ludziejewski, M. Kapusta, A. Lempicki, C. Brecher, D. Wisniewski, AJ. Wojtowicz, “Properties of LuAP:Ce scintillator”, Nucl. Instr. Meth. A385, 123–31, (1997)

    Google Scholar 

  40. E.V.D. van Loef, P. Dorenbos, C.W.E. van Eijk, “High-energy resolution scintillator Ce3+ activated LaCl3”, Appl. Phys. Lett., 77, 1467–1468, (2000)

    Article  Google Scholar 

  41. E.V.D. van Loef, P. Dorenbos, C.W.E. van Eijk, K. Kramer, H.U. Gudel, “High-energy-resolution scintillator: Ce3+ activated LaBr3”, Appl. Phys. Lett., 79, 1573–1575, (2001)

    Article  CAS  Google Scholar 

  42. A. Kuhn, S. Surti, J.S. Karp, P.S. Raby, K.S. Shah, A.E. Perkins, G. Muehllehner, “Design of a Lanthanum Bromide Detector for Time-of-Flight PET”, IEEE Trans. Nucl. Sci., 51, 2550–2557, (2004)

    Article  CAS  Google Scholar 

  43. M. Balcerzyk, M. Moszyński, M. Kapusta, “Comparison of LaCl3:Ce and NaI(Tl) scintillators in γ-ray spectrometry”, Nucl. Instr. Meth., A537, 50–56, (2005)

    Google Scholar 

  44. P. Dorenbos, J.T.M. de Haas, C.W.E. van Eijk, “Gamma ray spectroscopy with a Ø19 × 19 mm3 LaBr3:0.5%Ce3+ scintillator”, IEEE Trans. Nucl. Sci., 486, 1289–1296, (2004)

    Article  CAS  Google Scholar 

  45. P. Dorenbos, “Thoughts on non-proportionality”, Non-proportionality Workshop, Portland, USA, October 2003

    Google Scholar 

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Moszyński, M. (2006). NON-PROPORTIONALITY AND ENERGY RESOLUTION OF SCINTILLATION DETECTORS. In: Tavernier, S., Gektin, A., Grinyov, B., Moses, W.W. (eds) Radiation Detectors for Medical Applications. NATO Security through Science Series. Springer, Dordrecht . https://doi.org/10.1007/1-4020-5093-3_13

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  • DOI: https://doi.org/10.1007/1-4020-5093-3_13

  • Publisher Name: Springer, Dordrecht

  • Print ISBN: 978-1-4020-5091-6

  • Online ISBN: 978-1-4020-5093-0

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