Abstract
The application of scintillation detectors in nuclear medicine utilizing gamma spectrometry methods, as PET and SPECT detectors, and gamma cameras, requires a high energy resolution of the detectors. The limitations of energy resolution are discussed with a special emphasis on non-proportional response of scintillators to gamma rays and electrons, which is of crucial importance to an intrinsic resolution of the crystals. An importance of the scattering of secondary electrons (δ-rays) on intrinsic resolution is pointed out. Examples of the study carried out with different crystals and particularly those used in nuclear medicine are presented.
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REFERENCES
G.F. Knoll, “Radiation Detection and Measurements”, Third Edition, John Willey and Son, New York, 2000
M. Moszynski, “Inorganic scintillation detectors in γ-ray spectrometry”, Nucl. Instr. Meth., A505, 101–110, (2003)
M. Moszynski, “Energy resolution of scintillation detectors”, SPIE Proceedings, in press
P. Dorenbos, J.T.M. de Haas, C.W.E. van Eijk, “Non-proportionality in the Scintillation Response and the Energy Resolution Obtainable with Scintillation Crystals”, IEEE Trans. Nucl. Sci, 42, 2190–2202, (1995)
M. Moszyński, J. Zalipska, M. Balcerzyk, M. Kapusta, W. Mengeshe, J.D. Valentine, “Intrinsic energy resolution of NaI(Tl)”, Nucl. Instr. Meth., A484, 259–269, (2002)
G.G. Kelly, P.R. Bell, R.C. Davis and N.A. Lazar, “Intrinsic energy resolution”, IRE Trans, on Nucl, Sci., NS3, 57–58, (1956)
P. Iredale, “The effect of the non-proportional response of NaI(Tl) crystals to electrons upon the resolution for γ-rays”, Nucl. Instr. Meth., 11, 340–346, (1961)
C.D. Zerby, A. Meyer, R.B. Murray, “Intrinsic line broadening in NaI(Tl) gamma-ray spectrometers”, Nucl. Instr. Meth., 12, 115–123, (1961)
G.H. Narayan and J.R. Prescott, “The contribution of the NaI(Tl) crystal to the total line width of NaI(Tl) scintillation counters”, IEEE Trans. Nucl. Sci, NS-15, 162–166, (1968)
J.R. Prescott and G.H. Narayan, “Electron response and intrinsic line-widths in NaI(Tl) Crystals”, Nucl. Instr. Meth., 75, 51–55, (1969)
P. Dorenbos, J.T.M. de Hass, C.W.E. van Eijk, C.L. Melcher, and J.S. Schweitzer, “Nonlinear response in the scintillation yield of Lu2SiO5:Ce, IEEE Trans, on Nucl. Sci., 41,1052–1061, (1994)
P. Dorenbos, J.T.M. de Hass and C.W.E. van Eijk, “Non-proportional response in the light yield of inorganic scintillators”, 1994 IEEE Nucl. Sci. Symp. Norfolk, USA, Conference Records, p. 304–6
T.D. Taulbee, B.D. Rooney, W. Mengesha, and J.D. Velentine, “The Measured Electron Response Nonproportionalities of CaF2, BGO, and LSO”, IEEE Trans. Nucl. Sci., 44, 489–493, (1997)
J.D. Valentine and B.D. Rooney, “Design of a Compton spectrometer for studying scintillator nonlinearity and intrinsic resolution”, Nucl. Instr. and Meth., A353, 37–40, (1994)
B.D. Rooney and J.D. Valentine, “Benchmarking the Compton Coincidence Technique for measuring electron response nonproportionality in inorganic scintillators”, IEEE Trans. Nucl. Sci., 43, 1271–1276, (1996)
B.D. Rooney and J. D. Valentine, “Scintillator light yield nonproportionality: calculating photon response using measured electron response”, IEEE Trans. Nucl. Sci., 44, 509–16, (1997)
W. Mengesha, T.D. Taulbee, B.D. Rooney and J.D. Valentine, “Light Yield Nonproportionality of CsI(Tl), CsI(Na), and YAP”, IEEE Trans. Nucl. Sci., 45, 456–460, (1998)
J.D. Valentine, B.D. Rooney, and J. Li, “The Light Yield Nonproportionality Component of Scintillator Energy Resolution”, IEEE Trans. Nucl. Sci., 45, 512–517, (1998)
M. Kapusta, M. Balcerzyk, M. Moszyński, J. Pawelke. “A high-energy resolution observed from a YAP:Ce scintillator”, Nucl. Instr. Meth., A421, 610–13, (1999)
M. Balcerzyk, M. Moszyński, M. Kapusta, “Energy resolution of contemporary scintillators. Quest for high resolution, proportional detector”, Proc. of Fifth Int. Conf. on Inorganic Scintillators and Their Application, Moscow, August 16–20. (1999), p. 167
M. Balcerzyk, M. Moszyński, M. Kapusta, D. Wolski, J. Pawelke, C.L. Melcher, “YSO, LSO, GSO and LGSO. A Study of Energy Resolution and Non-Proportionality”, IEEE Trans. Nucl. Sci., 47, 1319–1323, (2000)
M. Moszyński, M. Kapusta, D. Wolski, M. Szawlowski, W. Klamra, “Energy Resolution of Scintillation Detectors Readout with Large Area Avalanche Photodiodes and Photomultipliers”, IEEE Trans. Nucl. Sci., 45, 472–77, (1998)
M. Moszyński, M. Kapusta, J. Zalipska, M. Balcerzyk, D. Wolski, M. Szawlowski and W. Klamra, “Low energy gamma-ray scintillation detection with large area avalanche photodiodes”, IEEE Trans. Nucl. Sci., 46, 243, (1999)
W. Mengesha, J.D. Valentine, “Benchmarking NaI(Tl) Electron Energy Resolution Measurements”, IEEE Trans. Nucl. Sci., 49, 2420–2426, (2002)
M. Moszynski, M. Balcerzyk, W Czarnacki, M. Kapusta, W. Klamra, A. Syntfeld, M. Szawlowski, “Intrinsic Resolution and Light Yield Non-proportionality of BGO”, IEEE Trans. Nucl. Sci., 51, 1074, (2004)
E. Breitenberger, “Scintillation spectrometers statistics”, Progress in Nucl. Phys. 4, 56–94, (1956)
D. Engelkemeir, “Nonlinear response of NaI(Tl) to photons”, Rev. Sci. Instr., 27, 589–591, (1956)
R.B. Murray and A. Meyer, “Scintillation Response of Activated Inorganic Crystals to Various Charged Particles”, Phys. Rev., 112, 815–826, (1961)
H. Leutz, C. D’Ambrosio, “On the scintillation response of NaI(Tl)-crystals”, IEEE Trans. Nucl. Sci., 44, 190–193, (1997)
P.A. Rodnyi, “Physical processes in inorganic scintillators”, CRC Press, New York, 1997
M. Moszyński, M. Balcerzyk, M. Kapusta, A. Syntfeld, D. Wolski, G. Pausch, J. Stein, P. Schotanus, “CdWO4 Crystal in Gamma-ray Spectrometry”, IEEE Trans. Nucl. Sci., in press
M. Moszyński, M. Balcerzyk, W. Czarnacki,_A. Nassalski, T. Szczęśniak,_M. Moszyński, H. Kraus, V. B. Mikhailik, I.M. Solskii, “Characterization of CaWO4 scintillator at room and liquid nitrogen temperatures”, Nucl. Instr. Meth., in press
M. Moszyński, W. Czarnacki, M. Kapusta, M. Szawlowski, W. Klamra, P. Schotanus, “Energy resolution and light yield non-proportionality of pure NaI scintillator studied with large area avalanche photodiodes at liquid nitrogen temperature”, Nucl. Instr. Meth., A., A486, 13–17, (2002)
M. Moszyński, W. Czarnacki, W. Klamra, M. Szawlowski, P. Schotanus, M. Kapusta, “Intrinsic Energy Resolution of pure NaI Studied with Large Area Avalanche Photodiodes at Liquid Nitrogen Temperature”, Nucl. Instr. Meth., A., A505, 63–67, (2003)
M. Moszynski, M. Balcerzyk, W. Czarnacki, M. Kapusta, W. Klamra, P. Schotanus, A. Syntfeld, M. Szawlowski, “Study of Pure NaI at Room and Liquid Nitrogen Temperatures”, IEEE Trans. Nucl Sci., 50, 767–773, (2003)
M. Moszyński, M. Balcerzyk, W. Czarnacki, M. Kapusta, W. Klamra, P. Schotanus, A. Syntfeld, M. Szawlowski, “Energy Resolution and Non-proportionality of the Light Yield of Pure CsI at Liquid Nitrogen Temperature”, Nucl. Instr. Meth., A537, 357–362, (2005)
M. Kapusta, P Szupryczyński, C. Melcher, M. Moszynski, M. Balcerzyk, A. A. Carey, W. Czarnacki, A. Spurrier, A. Syntfeld, “Non-proportionality and Thermoluminescence of LSO:Ce”, IEEE Trans. Nucl. Sci., in press
M. Balcerzyk, M. Moszyński, Z. Galazka, M. Kapusta, A. Syntfeld and J-L. Lefaucheur, “Perspectives for high resolution and high light output LuAP:Ce crystals”, IEEE Trans. Nucl. Sci., in press
M. Moszyński, D. Wolski, T. Ludziejewski, M. Kapusta, A. Lempicki, C. Brecher, D. Wisniewski, AJ. Wojtowicz, “Properties of LuAP:Ce scintillator”, Nucl. Instr. Meth. A385, 123–31, (1997)
E.V.D. van Loef, P. Dorenbos, C.W.E. van Eijk, “High-energy resolution scintillator Ce3+ activated LaCl3”, Appl. Phys. Lett., 77, 1467–1468, (2000)
E.V.D. van Loef, P. Dorenbos, C.W.E. van Eijk, K. Kramer, H.U. Gudel, “High-energy-resolution scintillator: Ce3+ activated LaBr3”, Appl. Phys. Lett., 79, 1573–1575, (2001)
A. Kuhn, S. Surti, J.S. Karp, P.S. Raby, K.S. Shah, A.E. Perkins, G. Muehllehner, “Design of a Lanthanum Bromide Detector for Time-of-Flight PET”, IEEE Trans. Nucl. Sci., 51, 2550–2557, (2004)
M. Balcerzyk, M. Moszyński, M. Kapusta, “Comparison of LaCl3:Ce and NaI(Tl) scintillators in γ-ray spectrometry”, Nucl. Instr. Meth., A537, 50–56, (2005)
P. Dorenbos, J.T.M. de Haas, C.W.E. van Eijk, “Gamma ray spectroscopy with a Ø19 × 19 mm3 LaBr3:0.5%Ce3+ scintillator”, IEEE Trans. Nucl. Sci., 486, 1289–1296, (2004)
P. Dorenbos, “Thoughts on non-proportionality”, Non-proportionality Workshop, Portland, USA, October 2003
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Moszyński, M. (2006). NON-PROPORTIONALITY AND ENERGY RESOLUTION OF SCINTILLATION DETECTORS. In: Tavernier, S., Gektin, A., Grinyov, B., Moses, W.W. (eds) Radiation Detectors for Medical Applications. NATO Security through Science Series. Springer, Dordrecht . https://doi.org/10.1007/1-4020-5093-3_13
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DOI: https://doi.org/10.1007/1-4020-5093-3_13
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